Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation

Mesoporous silica KCC-1 was successfully synthesized by microemulsion system coupled with microwave-assisted hydrothermal method. Mesoporous silica KCC-1 exhibited spherical morphology surrounded with dendritic fiber with the particle size of 200–400 nm and BET surface area of 773 m2/g. Mesoporous s...

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Main Authors: M. Y. S., Hamid, M. L., Firmansyah, S., Triwahyono, A. A., Jalil, R. R., Mukti, E., Febriyanti, V., Suendo, Setiabudi, H. D., M., Mohamed, W., Nabgan
Format: Article
Language:English
Published: Elsevier Ltd 2017
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/16548/1/fkksa-2017-setiabudi-Oxygen%20vacancy-rich1.pdf
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author M. Y. S., Hamid
M. L., Firmansyah
S., Triwahyono
A. A., Jalil
R. R., Mukti
E., Febriyanti
V., Suendo
Setiabudi, H. D.
M., Mohamed
W., Nabgan
author_facet M. Y. S., Hamid
M. L., Firmansyah
S., Triwahyono
A. A., Jalil
R. R., Mukti
E., Febriyanti
V., Suendo
Setiabudi, H. D.
M., Mohamed
W., Nabgan
author_sort M. Y. S., Hamid
collection UMP
description Mesoporous silica KCC-1 was successfully synthesized by microemulsion system coupled with microwave-assisted hydrothermal method. Mesoporous silica KCC-1 exhibited spherical morphology surrounded with dendritic fiber with the particle size of 200–400 nm and BET surface area of 773 m2/g. Mesoporous silica KCC-1 has significantly higher number of basicity and oxygen vacancy than those of MCM-41 and SiO2 which directly correlated with the catalytic performance of the catalyst. The activity of mesoporous silica KCC-1 in CO2 methanation is five-fold higher than MCM-41 with the yield of CH4 reached 38.9% at 723 K.
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spelling UMPir165482017-06-16T07:15:01Z http://umpir.ump.edu.my/id/eprint/16548/ Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation M. Y. S., Hamid M. L., Firmansyah S., Triwahyono A. A., Jalil R. R., Mukti E., Febriyanti V., Suendo Setiabudi, H. D. M., Mohamed W., Nabgan TP Chemical technology Mesoporous silica KCC-1 was successfully synthesized by microemulsion system coupled with microwave-assisted hydrothermal method. Mesoporous silica KCC-1 exhibited spherical morphology surrounded with dendritic fiber with the particle size of 200–400 nm and BET surface area of 773 m2/g. Mesoporous silica KCC-1 has significantly higher number of basicity and oxygen vacancy than those of MCM-41 and SiO2 which directly correlated with the catalytic performance of the catalyst. The activity of mesoporous silica KCC-1 in CO2 methanation is five-fold higher than MCM-41 with the yield of CH4 reached 38.9% at 723 K. Elsevier Ltd 2017 Article PeerReviewed application/pdf en http://umpir.ump.edu.my/id/eprint/16548/1/fkksa-2017-setiabudi-Oxygen%20vacancy-rich1.pdf M. Y. S., Hamid and M. L., Firmansyah and S., Triwahyono and A. A., Jalil and R. R., Mukti and E., Febriyanti and V., Suendo and Setiabudi, H. D. and M., Mohamed and W., Nabgan (2017) Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation. Applied Catalysis A: General, 532. pp. 86-94. ISSN 0926-860X. (Published) https://doi.org/10.1016/j.apcata.2016.12.023 DOI: 10.1016/j.apcata.2016.12.023
spellingShingle TP Chemical technology
M. Y. S., Hamid
M. L., Firmansyah
S., Triwahyono
A. A., Jalil
R. R., Mukti
E., Febriyanti
V., Suendo
Setiabudi, H. D.
M., Mohamed
W., Nabgan
Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation
title Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation
title_full Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation
title_fullStr Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation
title_full_unstemmed Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation
title_short Oxygen Vacancy-rich Mesoporous Silica KCC-1 for CO2 Methanation
title_sort oxygen vacancy rich mesoporous silica kcc 1 for co2 methanation
topic TP Chemical technology
url http://umpir.ump.edu.my/id/eprint/16548/1/fkksa-2017-setiabudi-Oxygen%20vacancy-rich1.pdf
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