CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition
Background/Objectives: The effects of Ce loading (1-7 wt%) on the properties of Ni/SBA-15 andCO2 dry reforming with methane was studied. Methods/StatisticalAnalysis: The physicochemical properties of the catalysts were analyzed by XRD, BET, TEM and FTIR. Catalytic performance of catalyst was perform...
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| Format: | Article |
| Language: | English |
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Informatics Publishing Limited
2017
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| Online Access: | http://umpir.ump.edu.my/id/eprint/18019/1/CO2%20Reforming%20of%20Methane%20over%20Ni-Ce-SBA-15-%20Effects%20of%20Ce%20Addition.pdf |
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| author | Nurul Aini, Razali Nurul Ainun Nabihah, AbGhazab Setiabudi, H. D. Chin, S. Y. |
| author_facet | Nurul Aini, Razali Nurul Ainun Nabihah, AbGhazab Setiabudi, H. D. Chin, S. Y. |
| author_sort | Nurul Aini, Razali |
| collection | UMP |
| description | Background/Objectives: The effects of Ce loading (1-7 wt%) on the properties of Ni/SBA-15 andCO2 dry reforming with methane was studied. Methods/StatisticalAnalysis: The physicochemical properties of the catalysts were analyzed by XRD, BET, TEM and FTIR. Catalytic performance of catalyst was performed using a fixed bed reactor at 700°C. Findings: NCS7 catalyst had the highest activity and good stability with CH4 conversion, CO2 conversion and H2/CO ratio of 94.9%, 95.1%, and 0.99, respectively. This can be attributed to the Ce ensuring a good Ni dispersion and inhibited the carbon deposition on the catalyst surfaces. Moreover, high Ce loading of NCS7 promoting the formation of a significant synergy effect between Ni active sites with SBA-15 for target reaction. Application/Improvements: The result presented is very promising to improve the GHGs conversion strategies for the production of useful chemical products. |
| first_indexed | 2024-03-06T12:16:27Z |
| format | Article |
| id | UMPir18019 |
| institution | Universiti Malaysia Pahang |
| language | English |
| last_indexed | 2024-03-06T12:16:27Z |
| publishDate | 2017 |
| publisher | Informatics Publishing Limited |
| record_format | dspace |
| spelling | UMPir180192018-07-16T08:39:56Z http://umpir.ump.edu.my/id/eprint/18019/ CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition Nurul Aini, Razali Nurul Ainun Nabihah, AbGhazab Setiabudi, H. D. Chin, S. Y. TP Chemical technology Background/Objectives: The effects of Ce loading (1-7 wt%) on the properties of Ni/SBA-15 andCO2 dry reforming with methane was studied. Methods/StatisticalAnalysis: The physicochemical properties of the catalysts were analyzed by XRD, BET, TEM and FTIR. Catalytic performance of catalyst was performed using a fixed bed reactor at 700°C. Findings: NCS7 catalyst had the highest activity and good stability with CH4 conversion, CO2 conversion and H2/CO ratio of 94.9%, 95.1%, and 0.99, respectively. This can be attributed to the Ce ensuring a good Ni dispersion and inhibited the carbon deposition on the catalyst surfaces. Moreover, high Ce loading of NCS7 promoting the formation of a significant synergy effect between Ni active sites with SBA-15 for target reaction. Application/Improvements: The result presented is very promising to improve the GHGs conversion strategies for the production of useful chemical products. Informatics Publishing Limited 2017 Article PeerReviewed application/pdf en cc_by http://umpir.ump.edu.my/id/eprint/18019/1/CO2%20Reforming%20of%20Methane%20over%20Ni-Ce-SBA-15-%20Effects%20of%20Ce%20Addition.pdf Nurul Aini, Razali and Nurul Ainun Nabihah, AbGhazab and Setiabudi, H. D. and Chin, S. Y. (2017) CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition. Indian Journal of Science and Technology, 10 (17). pp. 1-5. ISSN 0974-6846 (Print); 0974-5645 (Online). (Published) http://52.172.159.94/index.php/indjst/article/view/110380 DOI: 10.17485/ijst/2017/v10i17/110380 |
| spellingShingle | TP Chemical technology Nurul Aini, Razali Nurul Ainun Nabihah, AbGhazab Setiabudi, H. D. Chin, S. Y. CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition |
| title | CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition |
| title_full | CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition |
| title_fullStr | CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition |
| title_full_unstemmed | CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition |
| title_short | CO2 Reforming of Methane over Ni/Ce-SBA-15: Effects of Ce Addition |
| title_sort | co2 reforming of methane over ni ce sba 15 effects of ce addition |
| topic | TP Chemical technology |
| url | http://umpir.ump.edu.my/id/eprint/18019/1/CO2%20Reforming%20of%20Methane%20over%20Ni-Ce-SBA-15-%20Effects%20of%20Ce%20Addition.pdf |
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