Influence of intermediate layers in tubular carbon membrane for gas separation performance

The main objective of this study is to determine the best intermediate layer for tubular carbon membranes for H2 and He separation. Intermediate layer was applied to strengthen interfacial adhesion between selective carbon layers and tubular support. Three different intermediate layers (alumina powd...

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Main Authors: Norazlianie, Sazali, Wan Norharyati, Wan Salleh, A. F., Ismail, N. H., Ismail, N., Yusof, F., Aziz, Jamiluddin, Jaafar, K., Kadirgama
Format: Article
Language:English
Published: Elsevier 2019
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/23812/8/Influence%20of%20intermediate%20layers%20in%20tubular%20carbon%20membrane.pdf
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author Norazlianie, Sazali
Wan Norharyati, Wan Salleh
A. F., Ismail
N. H., Ismail
N., Yusof
F., Aziz
Jamiluddin, Jaafar
K., Kadirgama
author_facet Norazlianie, Sazali
Wan Norharyati, Wan Salleh
A. F., Ismail
N. H., Ismail
N., Yusof
F., Aziz
Jamiluddin, Jaafar
K., Kadirgama
author_sort Norazlianie, Sazali
collection UMP
description The main objective of this study is to determine the best intermediate layer for tubular carbon membranes for H2 and He separation. Intermediate layer was applied to strengthen interfacial adhesion between selective carbon layers and tubular support. Three different intermediate layers (alumina powder, carbon molecular sieve (CMS), and carbon pencil) had been evaluated to compare their influence towards the performance of gas separation of the carbon membrane. Tubular carbon membrane was fabricated from PI/NCC-based polymer blends which had been carbonized under Argon atmosphere at 800 °C with a heating rate of 3 °C/min. Based on the scanning electron microscopic (SEM) observations, carbon membrane with alumina powder as an intermediate layer had formed a smoother surface compared to other types of intermediate layers. A high performance of tubular carbon membrane was obtained by employing alumina powder as an intermediate layer, which exhibited the best selectivity of H2/N2 and He/N2 of 447.31 ± 1.45 and 471.72 ± 2.19, respectively.
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spelling UMPir238122020-04-30T01:52:57Z http://umpir.ump.edu.my/id/eprint/23812/ Influence of intermediate layers in tubular carbon membrane for gas separation performance Norazlianie, Sazali Wan Norharyati, Wan Salleh A. F., Ismail N. H., Ismail N., Yusof F., Aziz Jamiluddin, Jaafar K., Kadirgama H Social Sciences (General) QD Chemistry TP Chemical technology The main objective of this study is to determine the best intermediate layer for tubular carbon membranes for H2 and He separation. Intermediate layer was applied to strengthen interfacial adhesion between selective carbon layers and tubular support. Three different intermediate layers (alumina powder, carbon molecular sieve (CMS), and carbon pencil) had been evaluated to compare their influence towards the performance of gas separation of the carbon membrane. Tubular carbon membrane was fabricated from PI/NCC-based polymer blends which had been carbonized under Argon atmosphere at 800 °C with a heating rate of 3 °C/min. Based on the scanning electron microscopic (SEM) observations, carbon membrane with alumina powder as an intermediate layer had formed a smoother surface compared to other types of intermediate layers. A high performance of tubular carbon membrane was obtained by employing alumina powder as an intermediate layer, which exhibited the best selectivity of H2/N2 and He/N2 of 447.31 ± 1.45 and 471.72 ± 2.19, respectively. Elsevier 2019-07 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/23812/8/Influence%20of%20intermediate%20layers%20in%20tubular%20carbon%20membrane.pdf Norazlianie, Sazali and Wan Norharyati, Wan Salleh and A. F., Ismail and N. H., Ismail and N., Yusof and F., Aziz and Jamiluddin, Jaafar and K., Kadirgama (2019) Influence of intermediate layers in tubular carbon membrane for gas separation performance. International Journal of Hydrogen Energy, 44 (37). pp. 20914-20923. ISSN 0360-3199. (Published) https://doi.org/10.1016/j.ijhydene.2018.06.148 https://doi.org/10.1016/j.ijhydene.2018.06.148
spellingShingle H Social Sciences (General)
QD Chemistry
TP Chemical technology
Norazlianie, Sazali
Wan Norharyati, Wan Salleh
A. F., Ismail
N. H., Ismail
N., Yusof
F., Aziz
Jamiluddin, Jaafar
K., Kadirgama
Influence of intermediate layers in tubular carbon membrane for gas separation performance
title Influence of intermediate layers in tubular carbon membrane for gas separation performance
title_full Influence of intermediate layers in tubular carbon membrane for gas separation performance
title_fullStr Influence of intermediate layers in tubular carbon membrane for gas separation performance
title_full_unstemmed Influence of intermediate layers in tubular carbon membrane for gas separation performance
title_short Influence of intermediate layers in tubular carbon membrane for gas separation performance
title_sort influence of intermediate layers in tubular carbon membrane for gas separation performance
topic H Social Sciences (General)
QD Chemistry
TP Chemical technology
url http://umpir.ump.edu.my/id/eprint/23812/8/Influence%20of%20intermediate%20layers%20in%20tubular%20carbon%20membrane.pdf
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