Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers

A flexible perovskite solar yarn with an impressive active lifetime (>216 h) and an exceptional photon conversion efficiency is prepared under ordinary conditions. The champion device demonstrates an average linear mass density of 0.89 mg cm−1 and can be bent over a loop diameter of 2.5 mm, with...

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Main Authors: Li, Qian, Balilonda, Andrew, Ali, Aizaz, Rajan, Jose, Zabihi, Fatemeh, Yang, Shengyuan, Ramakrishna, Seeram, Zhu, Meifang
Format: Article
Language:English
Published: Wiley 2020
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/30805/7/Flexible%20Solar%20Yarns%20with%20151.pdf
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author Li, Qian
Balilonda, Andrew
Ali, Aizaz
Rajan, Jose
Zabihi, Fatemeh
Yang, Shengyuan
Ramakrishna, Seeram
Zhu, Meifang
author_facet Li, Qian
Balilonda, Andrew
Ali, Aizaz
Rajan, Jose
Zabihi, Fatemeh
Yang, Shengyuan
Ramakrishna, Seeram
Zhu, Meifang
author_sort Li, Qian
collection UMP
description A flexible perovskite solar yarn with an impressive active lifetime (>216 h) and an exceptional photon conversion efficiency is prepared under ordinary conditions. The champion device demonstrates an average linear mass density of 0.89 mg cm−1 and can be bent over a loop diameter of 2.5 mm, with a negligible efficiency loss. Photoactive nanofibers composed of a polyvinylpyrrolidone (PVP) central strain and a perovskite phase on the surface (with average grain size of 275 ± 14.3 nm), are prepared by electrospinning, at 18 kV, relative humidity of 75%, and a temperature of 25 °C. This bilayered configuration promises superior mechanical strength and flexibility, together with an excellent photovoltaic character, compared with their dip coated counterparts. Photoactive perovskite nanofibers are incorporated into a plied-solar yarn, with an organic hole-conductive layer, poly(3-hexylthiophene-2,5-diyl)-coated on silver yarn electrode, and a composite electron conductive layer, phenyl-C61-butyric acid methyl ester (PC61BM)-SnO2 coated on a carbon yarn. An individual double-twisted solar yarns yields 15.7% champion power conversion efficiency, while a 30.5 mm × 30.5 mm active area of plain-woven fabric generates a maximum power density of 1.26 mW cm−2 under one sun (1000 W m−2) solar illumination.
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spelling UMPir308052021-03-01T06:31:18Z http://umpir.ump.edu.my/id/eprint/30805/ Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers Li, Qian Balilonda, Andrew Ali, Aizaz Rajan, Jose Zabihi, Fatemeh Yang, Shengyuan Ramakrishna, Seeram Zhu, Meifang QC Physics QD Chemistry TK Electrical engineering. Electronics Nuclear engineering A flexible perovskite solar yarn with an impressive active lifetime (>216 h) and an exceptional photon conversion efficiency is prepared under ordinary conditions. The champion device demonstrates an average linear mass density of 0.89 mg cm−1 and can be bent over a loop diameter of 2.5 mm, with a negligible efficiency loss. Photoactive nanofibers composed of a polyvinylpyrrolidone (PVP) central strain and a perovskite phase on the surface (with average grain size of 275 ± 14.3 nm), are prepared by electrospinning, at 18 kV, relative humidity of 75%, and a temperature of 25 °C. This bilayered configuration promises superior mechanical strength and flexibility, together with an excellent photovoltaic character, compared with their dip coated counterparts. Photoactive perovskite nanofibers are incorporated into a plied-solar yarn, with an organic hole-conductive layer, poly(3-hexylthiophene-2,5-diyl)-coated on silver yarn electrode, and a composite electron conductive layer, phenyl-C61-butyric acid methyl ester (PC61BM)-SnO2 coated on a carbon yarn. An individual double-twisted solar yarns yields 15.7% champion power conversion efficiency, while a 30.5 mm × 30.5 mm active area of plain-woven fabric generates a maximum power density of 1.26 mW cm−2 under one sun (1000 W m−2) solar illumination. Wiley 2020-09-01 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/30805/7/Flexible%20Solar%20Yarns%20with%20151.pdf Li, Qian and Balilonda, Andrew and Ali, Aizaz and Rajan, Jose and Zabihi, Fatemeh and Yang, Shengyuan and Ramakrishna, Seeram and Zhu, Meifang (2020) Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers. Solar RRL, 4 (9). pp. 1-12. ISSN 2367-198X. (Published) http://doi.org/10.1002/solr.202000269 http://doi.org/10.1002/solr.202000269
spellingShingle QC Physics
QD Chemistry
TK Electrical engineering. Electronics Nuclear engineering
Li, Qian
Balilonda, Andrew
Ali, Aizaz
Rajan, Jose
Zabihi, Fatemeh
Yang, Shengyuan
Ramakrishna, Seeram
Zhu, Meifang
Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers
title Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers
title_full Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers
title_fullStr Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers
title_full_unstemmed Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers
title_short Flexible Solar Yarns with 15.7% Power Conversion Efficiency, Based on Electrospun Perovskite Composite Nanofibers
title_sort flexible solar yarns with 15 7 power conversion efficiency based on electrospun perovskite composite nanofibers
topic QC Physics
QD Chemistry
TK Electrical engineering. Electronics Nuclear engineering
url http://umpir.ump.edu.my/id/eprint/30805/7/Flexible%20Solar%20Yarns%20with%20151.pdf
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