Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and Storage

High-performance electrocatalysts are critical to support emerging electrochemical energy storage and conversion technologies. Graphite-derived materials, including fullerenes, carbon nanotubes, and graphene, have been recognized as promising electrocatalysts and electrocatalyst supports for the oxy...

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Main Authors: Shuaijie He, Mingjie Wu, Song Li, Zhiyi Jiang, Hanlie Hong, Sylvain G. Cloutier, Huaming Yang, Sasha Omanovic, Shuhui Sun, Gaixia Zhang
Format: Article
Language:English
Published: MDPI AG 2022-12-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/27/24/8644
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author Shuaijie He
Mingjie Wu
Song Li
Zhiyi Jiang
Hanlie Hong
Sylvain G. Cloutier
Huaming Yang
Sasha Omanovic
Shuhui Sun
Gaixia Zhang
author_facet Shuaijie He
Mingjie Wu
Song Li
Zhiyi Jiang
Hanlie Hong
Sylvain G. Cloutier
Huaming Yang
Sasha Omanovic
Shuhui Sun
Gaixia Zhang
author_sort Shuaijie He
collection DOAJ
description High-performance electrocatalysts are critical to support emerging electrochemical energy storage and conversion technologies. Graphite-derived materials, including fullerenes, carbon nanotubes, and graphene, have been recognized as promising electrocatalysts and electrocatalyst supports for the oxygen reduction reaction (ORR), oxygen evolution reaction (OER), hydrogen evolution reaction (HER), and carbon dioxide reduction reaction (CO<sub>2</sub>RR). Effective modification/functionalization of graphite-derived materials can promote higher electrocatalytic activity, stability, and durability. In this review, the mechanisms and evaluation parameters for the above-outlined electrochemical reactions are introduced first. Then, we emphasize the preparation methods for graphite-derived materials and modification strategies. We further highlight the importance of the structural changes of modified graphite-derived materials on electrocatalytic activity and stability. Finally, future directions and perspectives towards new and better graphite-derived materials are presented.
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spelling doaj.art-006dd7f719a24108a37d7a71d485d8f42023-11-24T16:54:58ZengMDPI AGMolecules1420-30492022-12-012724864410.3390/molecules27248644Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and StorageShuaijie He0Mingjie Wu1Song Li2Zhiyi Jiang3Hanlie Hong4Sylvain G. Cloutier5Huaming Yang6Sasha Omanovic7Shuhui Sun8Gaixia Zhang9Engineering Research Center of Nano-Geomaterials of Ministry of Education, China University of Geosciences, Wuhan 430074, ChinaDepartment of Chemical Engineering, McGill University, 3610 University Street, Montreal, QC H3A 0C5, CanadaEngineering Research Center of Nano-Geomaterials of Ministry of Education, China University of Geosciences, Wuhan 430074, ChinaEngineering Research Center of Nano-Geomaterials of Ministry of Education, China University of Geosciences, Wuhan 430074, ChinaEngineering Research Center of Nano-Geomaterials of Ministry of Education, China University of Geosciences, Wuhan 430074, ChinaDepartment of Electrical Engineering, École de Technologie Supérieure (ÉTS), Montreal, QC H3C 1K3, CanadaEngineering Research Center of Nano-Geomaterials of Ministry of Education, China University of Geosciences, Wuhan 430074, ChinaDepartment of Chemical Engineering, McGill University, 3610 University Street, Montreal, QC H3A 0C5, CanadaInstitut National de la Recherche Scientifique (INRS), Centre Énergie Matériaux Télécommunications, Varennes, QC J3X 1P7, CanadaDepartment of Electrical Engineering, École de Technologie Supérieure (ÉTS), Montreal, QC H3C 1K3, CanadaHigh-performance electrocatalysts are critical to support emerging electrochemical energy storage and conversion technologies. Graphite-derived materials, including fullerenes, carbon nanotubes, and graphene, have been recognized as promising electrocatalysts and electrocatalyst supports for the oxygen reduction reaction (ORR), oxygen evolution reaction (OER), hydrogen evolution reaction (HER), and carbon dioxide reduction reaction (CO<sub>2</sub>RR). Effective modification/functionalization of graphite-derived materials can promote higher electrocatalytic activity, stability, and durability. In this review, the mechanisms and evaluation parameters for the above-outlined electrochemical reactions are introduced first. Then, we emphasize the preparation methods for graphite-derived materials and modification strategies. We further highlight the importance of the structural changes of modified graphite-derived materials on electrocatalytic activity and stability. Finally, future directions and perspectives towards new and better graphite-derived materials are presented.https://www.mdpi.com/1420-3049/27/24/8644graphite-derived materialsfullerenescarbon nanotubesgrapheneelectrocatalysis
spellingShingle Shuaijie He
Mingjie Wu
Song Li
Zhiyi Jiang
Hanlie Hong
Sylvain G. Cloutier
Huaming Yang
Sasha Omanovic
Shuhui Sun
Gaixia Zhang
Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and Storage
Molecules
graphite-derived materials
fullerenes
carbon nanotubes
graphene
electrocatalysis
title Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and Storage
title_full Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and Storage
title_fullStr Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and Storage
title_full_unstemmed Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and Storage
title_short Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and Storage
title_sort research progress on graphite derived materials for electrocatalysis in energy conversion and storage
topic graphite-derived materials
fullerenes
carbon nanotubes
graphene
electrocatalysis
url https://www.mdpi.com/1420-3049/27/24/8644
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