Optically Induced Nonlinear Cubic Crystal System for 3D Quasi‐Phase Matching

Quasi‐phase matching (QPM) is a technique in nonlinear optics for achieving efficient energy exchange among optical waves at different frequencies, by spatially modulating the quadratic nonlinearity (χ (2)) of the medium. To realize the full potential of QPM, 3D spatial modulation of χ (2) is requir...

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Main Authors: Yesheng Chen, Chen Yang, Shan Liu, Sen Wang, Ningning Wang, Yongxing Liu, Yan Sheng, Ruwei Zhao, Tianxiang Xu, Wieslaw Krolikowski
Format: Article
Language:English
Published: Wiley-VCH 2022-04-01
Series:Advanced Photonics Research
Subjects:
Online Access:https://doi.org/10.1002/adpr.202100268
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author Yesheng Chen
Chen Yang
Shan Liu
Sen Wang
Ningning Wang
Yongxing Liu
Yan Sheng
Ruwei Zhao
Tianxiang Xu
Wieslaw Krolikowski
author_facet Yesheng Chen
Chen Yang
Shan Liu
Sen Wang
Ningning Wang
Yongxing Liu
Yan Sheng
Ruwei Zhao
Tianxiang Xu
Wieslaw Krolikowski
author_sort Yesheng Chen
collection DOAJ
description Quasi‐phase matching (QPM) is a technique in nonlinear optics for achieving efficient energy exchange among optical waves at different frequencies, by spatially modulating the quadratic nonlinearity (χ (2)) of the medium. To realize the full potential of QPM, 3D spatial modulation of χ (2) is required. This has become experimentally feasible recently thanks to the invention of femtosecond laser‐based nonlinearity engineering in ferroelectric crystals. Herein, the first experimental demonstration of QPM second harmonic generation (SHG) in a nonlinear cubic crystal system is presented, in which χ (2) modulations form simple cubic, body‐centered cubic, face‐centered cubic, and diamond cubic lattices, respectively. The experimental results indicate that these nonlinear cubic structures share the same primary reciprocal lattice vectors (RLVs), but possess different Fourier coefficients (in conventional cells), leading to SHG with similar angular resonances but various intensity distributions in the far field. This work contributes to a comprehensive understanding of nonlinear optical processes in 3D periodic media, and thus sheds light on the development of high‐performance QPM devices.
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spelling doaj.art-011065a2ab2f4d2f9f6facae4de948032022-12-22T01:46:26ZengWiley-VCHAdvanced Photonics Research2699-92932022-04-0134n/an/a10.1002/adpr.202100268Optically Induced Nonlinear Cubic Crystal System for 3D Quasi‐Phase MatchingYesheng Chen0Chen Yang1Shan Liu2Sen Wang3Ningning Wang4Yongxing Liu5Yan Sheng6Ruwei Zhao7Tianxiang Xu8Wieslaw Krolikowski9Laboratory of Infrared Materials and Devices Research Institute of Advanced Technologies Ningbo University Ningbo 315211 P. R. ChinaLaboratory of Infrared Materials and Devices Research Institute of Advanced Technologies Ningbo University Ningbo 315211 P. R. ChinaLaser Physics Center Research School of Physics Australian National University Canberra ACT 2601 AustraliaLaboratory of Infrared Materials and Devices Research Institute of Advanced Technologies Ningbo University Ningbo 315211 P. R. ChinaLaboratory of Infrared Materials and Devices Research Institute of Advanced Technologies Ningbo University Ningbo 315211 P. R. ChinaLaboratory of Infrared Materials and Devices Research Institute of Advanced Technologies Ningbo University Ningbo 315211 P. R. ChinaLaboratory of Infrared Materials and Devices Research Institute of Advanced Technologies Ningbo University Ningbo 315211 P. R. ChinaLaboratory of Infrared Materials and Devices Research Institute of Advanced Technologies Ningbo University Ningbo 315211 P. R. ChinaLaboratory of Infrared Materials and Devices Research Institute of Advanced Technologies Ningbo University Ningbo 315211 P. R. ChinaLaser Physics Center Research School of Physics Australian National University Canberra ACT 2601 AustraliaQuasi‐phase matching (QPM) is a technique in nonlinear optics for achieving efficient energy exchange among optical waves at different frequencies, by spatially modulating the quadratic nonlinearity (χ (2)) of the medium. To realize the full potential of QPM, 3D spatial modulation of χ (2) is required. This has become experimentally feasible recently thanks to the invention of femtosecond laser‐based nonlinearity engineering in ferroelectric crystals. Herein, the first experimental demonstration of QPM second harmonic generation (SHG) in a nonlinear cubic crystal system is presented, in which χ (2) modulations form simple cubic, body‐centered cubic, face‐centered cubic, and diamond cubic lattices, respectively. The experimental results indicate that these nonlinear cubic structures share the same primary reciprocal lattice vectors (RLVs), but possess different Fourier coefficients (in conventional cells), leading to SHG with similar angular resonances but various intensity distributions in the far field. This work contributes to a comprehensive understanding of nonlinear optical processes in 3D periodic media, and thus sheds light on the development of high‐performance QPM devices.https://doi.org/10.1002/adpr.202100268laser frequency conversionnonlinear photonic crystalsquasi-phase matchingsecond harmonic generation
spellingShingle Yesheng Chen
Chen Yang
Shan Liu
Sen Wang
Ningning Wang
Yongxing Liu
Yan Sheng
Ruwei Zhao
Tianxiang Xu
Wieslaw Krolikowski
Optically Induced Nonlinear Cubic Crystal System for 3D Quasi‐Phase Matching
Advanced Photonics Research
laser frequency conversion
nonlinear photonic crystals
quasi-phase matching
second harmonic generation
title Optically Induced Nonlinear Cubic Crystal System for 3D Quasi‐Phase Matching
title_full Optically Induced Nonlinear Cubic Crystal System for 3D Quasi‐Phase Matching
title_fullStr Optically Induced Nonlinear Cubic Crystal System for 3D Quasi‐Phase Matching
title_full_unstemmed Optically Induced Nonlinear Cubic Crystal System for 3D Quasi‐Phase Matching
title_short Optically Induced Nonlinear Cubic Crystal System for 3D Quasi‐Phase Matching
title_sort optically induced nonlinear cubic crystal system for 3d quasi phase matching
topic laser frequency conversion
nonlinear photonic crystals
quasi-phase matching
second harmonic generation
url https://doi.org/10.1002/adpr.202100268
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