Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe

Five one-year air quality simulations over a domain covering Europe have been performed using the CHIMERE chemistry transport model and the EMEP emission dataset for Europe. These five simulations differ only by the representation of the effective emission heights for anthropogenic emissions: one ha...

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Main Authors: S. Mailler, D. Khvorostyanov, L. Menut
Format: Article
Language:English
Published: Copernicus Publications 2013-06-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/13/5987/2013/acp-13-5987-2013.pdf
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author S. Mailler
D. Khvorostyanov
L. Menut
author_facet S. Mailler
D. Khvorostyanov
L. Menut
author_sort S. Mailler
collection DOAJ
description Five one-year air quality simulations over a domain covering Europe have been performed using the CHIMERE chemistry transport model and the EMEP emission dataset for Europe. These five simulations differ only by the representation of the effective emission heights for anthropogenic emissions: one has been run using the EMEP standard recommendations, three others with vertical injection profiles derived from the EMEP recommendations but multiplying the injection height by 0.75, 0.50 and 0.25, respectively, while the last one uses vertical profiles derived from the recent literature. It is shown that using injection heights lower than the EMEP recommendations leads to significantly improved simulation of background SO<sub>2</sub>, NO<sub>2</sub> and O<sub>3</sub> concentrations when compared to the Airbase station measurements.
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spelling doaj.art-0123cc26096c4628842b90eb8223a9e42022-12-22T00:57:45ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242013-06-0113125987599810.5194/acp-13-5987-2013Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over EuropeS. MaillerD. KhvorostyanovL. MenutFive one-year air quality simulations over a domain covering Europe have been performed using the CHIMERE chemistry transport model and the EMEP emission dataset for Europe. These five simulations differ only by the representation of the effective emission heights for anthropogenic emissions: one has been run using the EMEP standard recommendations, three others with vertical injection profiles derived from the EMEP recommendations but multiplying the injection height by 0.75, 0.50 and 0.25, respectively, while the last one uses vertical profiles derived from the recent literature. It is shown that using injection heights lower than the EMEP recommendations leads to significantly improved simulation of background SO<sub>2</sub>, NO<sub>2</sub> and O<sub>3</sub> concentrations when compared to the Airbase station measurements.http://www.atmos-chem-phys.net/13/5987/2013/acp-13-5987-2013.pdf
spellingShingle S. Mailler
D. Khvorostyanov
L. Menut
Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe
Atmospheric Chemistry and Physics
title Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe
title_full Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe
title_fullStr Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe
title_full_unstemmed Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe
title_short Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe
title_sort impact of the vertical emission profiles on background gas phase pollution simulated from the emep emissions over europe
url http://www.atmos-chem-phys.net/13/5987/2013/acp-13-5987-2013.pdf
work_keys_str_mv AT smailler impactoftheverticalemissionprofilesonbackgroundgasphasepollutionsimulatedfromtheemepemissionsovereurope
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AT lmenut impactoftheverticalemissionprofilesonbackgroundgasphasepollutionsimulatedfromtheemepemissionsovereurope