Investigation of Several Influential Factors on Organic Matter Decomposition in Lignite using Hydrogen Peroxide to Contribute to the Subsurface Cultivation and Gasification Method

Recently, the possibility of realizing a subsurface bio-reactor has been realized since microbial methanogenesis has been confirmed in diverse subsurface environments such as coalbeds or petroleum reservoirs. We propose a new gasification method for use in subsurface environments, known as the Subsu...

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Main Authors: Noritaka ARAMAKI, A.K.M. Badrul Alam, Shuji TAMAMURA, Akio UENO, Takuma MURAKAMI, Katsuhiko KANEKO
Format: Article
Language:English
Published: The Mining and Materials Processing Institute of Japan 2016-12-01
Series:Journal of MMIJ
Subjects:
Online Access:https://www.jstage.jst.go.jp/article/journalofmmij/132/12/132_190/_pdf/-char/en
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author Noritaka ARAMAKI
A.K.M. Badrul Alam
Shuji TAMAMURA
Akio UENO
Takuma MURAKAMI
Katsuhiko KANEKO
author_facet Noritaka ARAMAKI
A.K.M. Badrul Alam
Shuji TAMAMURA
Akio UENO
Takuma MURAKAMI
Katsuhiko KANEKO
author_sort Noritaka ARAMAKI
collection DOAJ
description Recently, the possibility of realizing a subsurface bio-reactor has been realized since microbial methanogenesis has been confirmed in diverse subsurface environments such as coalbeds or petroleum reservoirs. We propose a new gasification method for use in subsurface environments, known as the Subsurface Cultivation and Gasification (SCG). SCG was devised based on the production of biogenic methane gas in subsurface environments. This approach employed hydrogen peroxide to decompose organic matter rapidly. Conversion of organic matter from source rocks into biomethane with the help of microorganisms is expected to be highly profitable. In this study, a series of batch tests using a hydrogen peroxide (H2O2) solution were performed on lignite to estimate the potential of low-molecular-weight organic acid production. The effects of several factors on the production of low-molecular-weight organic acids have been considered, such as, concentration of H2O2, temperature, liquid-solid ratio, and specific subsurface area of lignite. It was found that the quantity of low-molecular-weight organic acids depended on temperature, liquid-solid ratio, and specific subsurface area of lignite; however, there isn't a unique relationship between them and the H2O2 concentration. Moreover, the mass of lignite reduced remarkably when batch tests were performed with a high concentration of H2O2. If H2O2 is to be injected into a target seam with the SCG method, we should estimate the optimum H2O2 concentration to produce low-molecular-weight organic acids with taking into consideration the mechanical stability of the target seam as well as the subsurface environmental chemical reaction with a geological improvement.
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spelling doaj.art-034b9e625d624d8a9e72c1fc23a02d5f2023-08-22T04:21:13ZengThe Mining and Materials Processing Institute of JapanJournal of MMIJ1881-61181884-04502016-12-011321219019810.2473/journalofmmij.132.190journalofmmijInvestigation of Several Influential Factors on Organic Matter Decomposition in Lignite using Hydrogen Peroxide to Contribute to the Subsurface Cultivation and Gasification MethodNoritaka ARAMAKI0A.K.M. Badrul Alam1Shuji TAMAMURA2Akio UENO3Takuma MURAKAMI4Katsuhiko KANEKO5Horonobe Research Institute for the Subsurface Environment, Northern Advancement Center for Science and TechnologyHoronobe Research Institute for the Subsurface Environment, Northern Advancement Center for Science and TechnologyHoronobe Research Institute for the Subsurface Environment, Northern Advancement Center for Science and TechnologyHoronobe Research Institute for the Subsurface Environment, Northern Advancement Center for Science and TechnologyHoronobe Research Institute for the Subsurface Environment, Northern Advancement Center for Science and TechnologyHoronobe Research Institute for the Subsurface Environment, Northern Advancement Center for Science and TechnologyRecently, the possibility of realizing a subsurface bio-reactor has been realized since microbial methanogenesis has been confirmed in diverse subsurface environments such as coalbeds or petroleum reservoirs. We propose a new gasification method for use in subsurface environments, known as the Subsurface Cultivation and Gasification (SCG). SCG was devised based on the production of biogenic methane gas in subsurface environments. This approach employed hydrogen peroxide to decompose organic matter rapidly. Conversion of organic matter from source rocks into biomethane with the help of microorganisms is expected to be highly profitable. In this study, a series of batch tests using a hydrogen peroxide (H2O2) solution were performed on lignite to estimate the potential of low-molecular-weight organic acid production. The effects of several factors on the production of low-molecular-weight organic acids have been considered, such as, concentration of H2O2, temperature, liquid-solid ratio, and specific subsurface area of lignite. It was found that the quantity of low-molecular-weight organic acids depended on temperature, liquid-solid ratio, and specific subsurface area of lignite; however, there isn't a unique relationship between them and the H2O2 concentration. Moreover, the mass of lignite reduced remarkably when batch tests were performed with a high concentration of H2O2. If H2O2 is to be injected into a target seam with the SCG method, we should estimate the optimum H2O2 concentration to produce low-molecular-weight organic acids with taking into consideration the mechanical stability of the target seam as well as the subsurface environmental chemical reaction with a geological improvement.https://www.jstage.jst.go.jp/article/journalofmmij/132/12/132_190/_pdf/-char/enligniteaccelerating decomposition of organic matterconcentration of hydrogen peroxidetemperaturespecific surface areas of lignitesubsurface cultivation and gasification
spellingShingle Noritaka ARAMAKI
A.K.M. Badrul Alam
Shuji TAMAMURA
Akio UENO
Takuma MURAKAMI
Katsuhiko KANEKO
Investigation of Several Influential Factors on Organic Matter Decomposition in Lignite using Hydrogen Peroxide to Contribute to the Subsurface Cultivation and Gasification Method
Journal of MMIJ
lignite
accelerating decomposition of organic matter
concentration of hydrogen peroxide
temperature
specific surface areas of lignite
subsurface cultivation and gasification
title Investigation of Several Influential Factors on Organic Matter Decomposition in Lignite using Hydrogen Peroxide to Contribute to the Subsurface Cultivation and Gasification Method
title_full Investigation of Several Influential Factors on Organic Matter Decomposition in Lignite using Hydrogen Peroxide to Contribute to the Subsurface Cultivation and Gasification Method
title_fullStr Investigation of Several Influential Factors on Organic Matter Decomposition in Lignite using Hydrogen Peroxide to Contribute to the Subsurface Cultivation and Gasification Method
title_full_unstemmed Investigation of Several Influential Factors on Organic Matter Decomposition in Lignite using Hydrogen Peroxide to Contribute to the Subsurface Cultivation and Gasification Method
title_short Investigation of Several Influential Factors on Organic Matter Decomposition in Lignite using Hydrogen Peroxide to Contribute to the Subsurface Cultivation and Gasification Method
title_sort investigation of several influential factors on organic matter decomposition in lignite using hydrogen peroxide to contribute to the subsurface cultivation and gasification method
topic lignite
accelerating decomposition of organic matter
concentration of hydrogen peroxide
temperature
specific surface areas of lignite
subsurface cultivation and gasification
url https://www.jstage.jst.go.jp/article/journalofmmij/132/12/132_190/_pdf/-char/en
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