Evaluation of radionuclide contamination of soil, coal ash and zeolitic materials from Figueira Thermoelectric Power Plant

Neutron activation analysis and gamma-ray spectrometry was used to determine 238U, 226Ra, 228Ra, 210Pb, 232Th and 40K contents in feed pulverized coal, bottom ash, fly ash from cyclone and baghouse filters, zeolites synthesized from the ashes and two different soil samples. All the samples used in...

Full description

Bibliographic Details
Main Authors: Denise Alves Fungaro, Paulo Sergio Silva, Felipe Campello, Caio Silva Miranda, Juliana Izidoro
Format: Article
Language:English
Published: Brazilian Radiation Protection Society (Sociedade Brasileira de Proteção Radiológica, SBPR) 2019-02-01
Series:Brazilian Journal of Radiation Sciences
Subjects:
Online Access:https://bjrs.org.br/revista/index.php/REVISTA/article/view/606
_version_ 1811338298302398464
author Denise Alves Fungaro
Denise Alves Fungaro
Paulo Sergio Silva
Felipe Campello
Caio Silva Miranda
Juliana Izidoro
author_facet Denise Alves Fungaro
Denise Alves Fungaro
Paulo Sergio Silva
Felipe Campello
Caio Silva Miranda
Juliana Izidoro
author_sort Denise Alves Fungaro
collection DOAJ
description Neutron activation analysis and gamma-ray spectrometry was used to determine 238U, 226Ra, 228Ra, 210Pb, 232Th and 40K contents in feed pulverized coal, bottom ash, fly ash from cyclone and baghouse filters, zeolites synthesized from the ashes and two different soil samples. All the samples used in the study was collected at Figueira thermoelectric power plant, located in the city of Figueira, Paraná State, which coal presents a significant amount of uranium concentration. The natural radionuclide concentrations in pulverized coal were 4216 Bq kg–1 for 238U, 180 Bq kg–1 for 226Ra, 27 Bq kg–1 for 228Ra, 28 Bq kg–1 for 232Th and 192 Bq kg–1 for 40K. The ashes fraction presented concentrations ranging from 683.5 to 1479 Bq kg–1 for 238U, from 484 to 1086 Bq kg–1 for 226Ra, from 291 to 1891 Bq kg–1 for 210Pb, from 67 to 111 Bq kg–1for 228Ra, from 80 to 87 Bq kg–1 for 232Th and from 489 to 718 Bq kg–1 for 40K. Similar ranges were observed for zeolites. The activity concentration of 238U was higher than worldwide average concentration for all samples. The concentration of the uranium series found in the ashes were lower than the values observed in similar studies carried out 10 years ago and under the limit adopted by the Brazilian guideline (CNEN-NN-4.01). Nevertheless, the concentrations of this specific area are higher than others coal mines and thermoelectric power plants in and out of Brazil, so it is advisable to evaluate the environmental impact of the installation.
first_indexed 2024-04-13T18:08:52Z
format Article
id doaj.art-037caff571c94aa19ce4835797df2be4
institution Directory Open Access Journal
issn 2319-0612
language English
last_indexed 2024-04-13T18:08:52Z
publishDate 2019-02-01
publisher Brazilian Radiation Protection Society (Sociedade Brasileira de Proteção Radiológica, SBPR)
record_format Article
series Brazilian Journal of Radiation Sciences
spelling doaj.art-037caff571c94aa19ce4835797df2be42022-12-22T02:35:58ZengBrazilian Radiation Protection Society (Sociedade Brasileira de Proteção Radiológica, SBPR)Brazilian Journal of Radiation Sciences2319-06122019-02-0172A10.15392/bjrs.v7i2A.606Evaluation of radionuclide contamination of soil, coal ash and zeolitic materials from Figueira Thermoelectric Power PlantDenise Alves Fungaro0Denise Alves Fungaro1Paulo Sergio Silva2Felipe Campello3Caio Silva Miranda4Juliana Izidoro5Nuclear and Energy Research InstituteNuclear and Energy Research InstituteNuclear and Energy Research InstituteNuclear and Energy Research InstituteNuclear and Energy Research InstituteNuclear and Energy Research Institute Neutron activation analysis and gamma-ray spectrometry was used to determine 238U, 226Ra, 228Ra, 210Pb, 232Th and 40K contents in feed pulverized coal, bottom ash, fly ash from cyclone and baghouse filters, zeolites synthesized from the ashes and two different soil samples. All the samples used in the study was collected at Figueira thermoelectric power plant, located in the city of Figueira, Paraná State, which coal presents a significant amount of uranium concentration. The natural radionuclide concentrations in pulverized coal were 4216 Bq kg–1 for 238U, 180 Bq kg–1 for 226Ra, 27 Bq kg–1 for 228Ra, 28 Bq kg–1 for 232Th and 192 Bq kg–1 for 40K. The ashes fraction presented concentrations ranging from 683.5 to 1479 Bq kg–1 for 238U, from 484 to 1086 Bq kg–1 for 226Ra, from 291 to 1891 Bq kg–1 for 210Pb, from 67 to 111 Bq kg–1for 228Ra, from 80 to 87 Bq kg–1 for 232Th and from 489 to 718 Bq kg–1 for 40K. Similar ranges were observed for zeolites. The activity concentration of 238U was higher than worldwide average concentration for all samples. The concentration of the uranium series found in the ashes were lower than the values observed in similar studies carried out 10 years ago and under the limit adopted by the Brazilian guideline (CNEN-NN-4.01). Nevertheless, the concentrations of this specific area are higher than others coal mines and thermoelectric power plants in and out of Brazil, so it is advisable to evaluate the environmental impact of the installation. https://bjrs.org.br/revista/index.php/REVISTA/article/view/606soilcoalcoal ash
spellingShingle Denise Alves Fungaro
Denise Alves Fungaro
Paulo Sergio Silva
Felipe Campello
Caio Silva Miranda
Juliana Izidoro
Evaluation of radionuclide contamination of soil, coal ash and zeolitic materials from Figueira Thermoelectric Power Plant
Brazilian Journal of Radiation Sciences
soil
coal
coal ash
title Evaluation of radionuclide contamination of soil, coal ash and zeolitic materials from Figueira Thermoelectric Power Plant
title_full Evaluation of radionuclide contamination of soil, coal ash and zeolitic materials from Figueira Thermoelectric Power Plant
title_fullStr Evaluation of radionuclide contamination of soil, coal ash and zeolitic materials from Figueira Thermoelectric Power Plant
title_full_unstemmed Evaluation of radionuclide contamination of soil, coal ash and zeolitic materials from Figueira Thermoelectric Power Plant
title_short Evaluation of radionuclide contamination of soil, coal ash and zeolitic materials from Figueira Thermoelectric Power Plant
title_sort evaluation of radionuclide contamination of soil coal ash and zeolitic materials from figueira thermoelectric power plant
topic soil
coal
coal ash
url https://bjrs.org.br/revista/index.php/REVISTA/article/view/606
work_keys_str_mv AT denisealvesfungaro evaluationofradionuclidecontaminationofsoilcoalashandzeoliticmaterialsfromfigueirathermoelectricpowerplant
AT denisealvesfungaro evaluationofradionuclidecontaminationofsoilcoalashandzeoliticmaterialsfromfigueirathermoelectricpowerplant
AT paulosergiosilva evaluationofradionuclidecontaminationofsoilcoalashandzeoliticmaterialsfromfigueirathermoelectricpowerplant
AT felipecampello evaluationofradionuclidecontaminationofsoilcoalashandzeoliticmaterialsfromfigueirathermoelectricpowerplant
AT caiosilvamiranda evaluationofradionuclidecontaminationofsoilcoalashandzeoliticmaterialsfromfigueirathermoelectricpowerplant
AT julianaizidoro evaluationofradionuclidecontaminationofsoilcoalashandzeoliticmaterialsfromfigueirathermoelectricpowerplant