Preparation of Polyamidoamine Dendrimer Modified Magnetic Nanoparticles and Its Application for Reliable Measurement of Sudan Red Contaminants in Natural Waters at Parts-Per-Billion Levels

The health threat from Sudan red dyes has been the subject of much attention in recent years and is crucial to design and establish reliable measurement technologies. In the present study, a new magnetic nanomaterial, polyamidoamine dendrimer-modified magnetic nanoparticles (Gn-MNPs), was synthesize...

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Main Authors: Yalin Wu, Huahua Bai, Qingxiang Zhou, Shuangying Li, Yayang Tong, Jinghan Guo, Boyao Zhou, Zhi Li, Yali Zhan, Menghua Liu, Yanhui Li, Tongxu Qu
Format: Article
Language:English
Published: Frontiers Media S.A. 2021-08-01
Series:Frontiers in Chemistry
Subjects:
Online Access:https://www.frontiersin.org/articles/10.3389/fchem.2021.708995/full
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author Yalin Wu
Yalin Wu
Huahua Bai
Qingxiang Zhou
Shuangying Li
Yayang Tong
Jinghan Guo
Boyao Zhou
Zhi Li
Yali Zhan
Menghua Liu
Yanhui Li
Tongxu Qu
author_facet Yalin Wu
Yalin Wu
Huahua Bai
Qingxiang Zhou
Shuangying Li
Yayang Tong
Jinghan Guo
Boyao Zhou
Zhi Li
Yali Zhan
Menghua Liu
Yanhui Li
Tongxu Qu
author_sort Yalin Wu
collection DOAJ
description The health threat from Sudan red dyes has been the subject of much attention in recent years and is crucial to design and establish reliable measurement technologies. In the present study, a new magnetic nanomaterial, polyamidoamine dendrimer-modified magnetic nanoparticles (Gn-MNPs), was synthesized and characterized. The nanomaterials had good adsorption capacity for Sudan dyes from natural waters. G1.5-MNPs possessed excellent adsorption capacity and a linear adsorption relationship over the range from 0.02 to 300 μg L−1 of Sudan dyes with relative coefficients all larger than 0.996. The sensitivity of the proposed method was excellent with detection limits over the range from 1.8 to 5.5 ng L−1 and the precision was less than 3.0%. G1.5-MNPs showed a remarkable application potential for the enrichment of trace environment pollutants in aqueous samples and the developed method based on this nanomaterial could be a robust and reliable alternative tool for routine monitoring of such pollutants.
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spelling doaj.art-04ab4b9af3844cf78ee1821c2adee8dd2022-12-21T23:33:13ZengFrontiers Media S.A.Frontiers in Chemistry2296-26462021-08-01910.3389/fchem.2021.708995708995Preparation of Polyamidoamine Dendrimer Modified Magnetic Nanoparticles and Its Application for Reliable Measurement of Sudan Red Contaminants in Natural Waters at Parts-Per-Billion LevelsYalin Wu0Yalin Wu1Huahua Bai2Qingxiang Zhou3Shuangying Li4Yayang Tong5Jinghan Guo6Boyao Zhou7Zhi Li8Yali Zhan9Menghua Liu10Yanhui Li11Tongxu Qu12State Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaBeijing Municipal Research Institute of Environmental Protection, Beijing, ChinaBeijing Municipal Research Institute of Environmental Protection, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaState Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing, ChinaThe health threat from Sudan red dyes has been the subject of much attention in recent years and is crucial to design and establish reliable measurement technologies. In the present study, a new magnetic nanomaterial, polyamidoamine dendrimer-modified magnetic nanoparticles (Gn-MNPs), was synthesized and characterized. The nanomaterials had good adsorption capacity for Sudan dyes from natural waters. G1.5-MNPs possessed excellent adsorption capacity and a linear adsorption relationship over the range from 0.02 to 300 μg L−1 of Sudan dyes with relative coefficients all larger than 0.996. The sensitivity of the proposed method was excellent with detection limits over the range from 1.8 to 5.5 ng L−1 and the precision was less than 3.0%. G1.5-MNPs showed a remarkable application potential for the enrichment of trace environment pollutants in aqueous samples and the developed method based on this nanomaterial could be a robust and reliable alternative tool for routine monitoring of such pollutants.https://www.frontiersin.org/articles/10.3389/fchem.2021.708995/fullSudan red dyesmagnetic solid phase extraction (MPSE)PAMAM dendrimerPAMAM dendrimer-modified magnetic nanoparticleshigh performance liquid phase chromatography
spellingShingle Yalin Wu
Yalin Wu
Huahua Bai
Qingxiang Zhou
Shuangying Li
Yayang Tong
Jinghan Guo
Boyao Zhou
Zhi Li
Yali Zhan
Menghua Liu
Yanhui Li
Tongxu Qu
Preparation of Polyamidoamine Dendrimer Modified Magnetic Nanoparticles and Its Application for Reliable Measurement of Sudan Red Contaminants in Natural Waters at Parts-Per-Billion Levels
Frontiers in Chemistry
Sudan red dyes
magnetic solid phase extraction (MPSE)
PAMAM dendrimer
PAMAM dendrimer-modified magnetic nanoparticles
high performance liquid phase chromatography
title Preparation of Polyamidoamine Dendrimer Modified Magnetic Nanoparticles and Its Application for Reliable Measurement of Sudan Red Contaminants in Natural Waters at Parts-Per-Billion Levels
title_full Preparation of Polyamidoamine Dendrimer Modified Magnetic Nanoparticles and Its Application for Reliable Measurement of Sudan Red Contaminants in Natural Waters at Parts-Per-Billion Levels
title_fullStr Preparation of Polyamidoamine Dendrimer Modified Magnetic Nanoparticles and Its Application for Reliable Measurement of Sudan Red Contaminants in Natural Waters at Parts-Per-Billion Levels
title_full_unstemmed Preparation of Polyamidoamine Dendrimer Modified Magnetic Nanoparticles and Its Application for Reliable Measurement of Sudan Red Contaminants in Natural Waters at Parts-Per-Billion Levels
title_short Preparation of Polyamidoamine Dendrimer Modified Magnetic Nanoparticles and Its Application for Reliable Measurement of Sudan Red Contaminants in Natural Waters at Parts-Per-Billion Levels
title_sort preparation of polyamidoamine dendrimer modified magnetic nanoparticles and its application for reliable measurement of sudan red contaminants in natural waters at parts per billion levels
topic Sudan red dyes
magnetic solid phase extraction (MPSE)
PAMAM dendrimer
PAMAM dendrimer-modified magnetic nanoparticles
high performance liquid phase chromatography
url https://www.frontiersin.org/articles/10.3389/fchem.2021.708995/full
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