Anthropogenic sulfur dioxide emissions: 1850–2005

Sulfur aerosols impact human health, ecosystems, agriculture, and global and regional climate. A new annual estimate of anthropogenic global and regional sulfur dioxide emissions has been constructed spanning the period 1850–2005 using a bottom-up mass balance method, calibrated to country-level inv...

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Main Authors: S. J. Smith, J. van Aardenne, Z. Klimont, R. J. Andres, A. Volke, S. Delgado Arias
Format: Article
Language:English
Published: Copernicus Publications 2011-02-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/11/1101/2011/acp-11-1101-2011.pdf
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author S. J. Smith
J. van Aardenne
Z. Klimont
R. J. Andres
A. Volke
S. Delgado Arias
author_facet S. J. Smith
J. van Aardenne
Z. Klimont
R. J. Andres
A. Volke
S. Delgado Arias
author_sort S. J. Smith
collection DOAJ
description Sulfur aerosols impact human health, ecosystems, agriculture, and global and regional climate. A new annual estimate of anthropogenic global and regional sulfur dioxide emissions has been constructed spanning the period 1850–2005 using a bottom-up mass balance method, calibrated to country-level inventory data. Global emissions peaked in the early 1970s and decreased until 2000, with an increase in recent years due to increased emissions in China, international shipping, and developing countries in general. An uncertainty analysis was conducted including both random and systemic uncertainties. The overall global uncertainty in sulfur dioxide emissions is relatively small, but regional uncertainties ranged up to 30%. The largest contributors to uncertainty at present are emissions from China and international shipping. Emissions were distributed on a 0.5° grid by sector for use in coordinated climate model experiments.
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spelling doaj.art-0508da0b75094535b4664b5ff8eee9ee2022-12-22T00:38:26ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242011-02-011131101111610.5194/acp-11-1101-2011Anthropogenic sulfur dioxide emissions: 1850–2005S. J. SmithJ. van AardenneZ. KlimontR. J. AndresA. VolkeS. Delgado AriasSulfur aerosols impact human health, ecosystems, agriculture, and global and regional climate. A new annual estimate of anthropogenic global and regional sulfur dioxide emissions has been constructed spanning the period 1850–2005 using a bottom-up mass balance method, calibrated to country-level inventory data. Global emissions peaked in the early 1970s and decreased until 2000, with an increase in recent years due to increased emissions in China, international shipping, and developing countries in general. An uncertainty analysis was conducted including both random and systemic uncertainties. The overall global uncertainty in sulfur dioxide emissions is relatively small, but regional uncertainties ranged up to 30%. The largest contributors to uncertainty at present are emissions from China and international shipping. Emissions were distributed on a 0.5° grid by sector for use in coordinated climate model experiments.http://www.atmos-chem-phys.net/11/1101/2011/acp-11-1101-2011.pdf
spellingShingle S. J. Smith
J. van Aardenne
Z. Klimont
R. J. Andres
A. Volke
S. Delgado Arias
Anthropogenic sulfur dioxide emissions: 1850–2005
Atmospheric Chemistry and Physics
title Anthropogenic sulfur dioxide emissions: 1850–2005
title_full Anthropogenic sulfur dioxide emissions: 1850–2005
title_fullStr Anthropogenic sulfur dioxide emissions: 1850–2005
title_full_unstemmed Anthropogenic sulfur dioxide emissions: 1850–2005
title_short Anthropogenic sulfur dioxide emissions: 1850–2005
title_sort anthropogenic sulfur dioxide emissions 1850 2005
url http://www.atmos-chem-phys.net/11/1101/2011/acp-11-1101-2011.pdf
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AT zklimont anthropogenicsulfurdioxideemissions18502005
AT rjandres anthropogenicsulfurdioxideemissions18502005
AT avolke anthropogenicsulfurdioxideemissions18502005
AT sdelgadoarias anthropogenicsulfurdioxideemissions18502005