Outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalyst
Although multinuclear, supramolecular photocatalysts show promise in their ability to separate the processes required for lightdriven energy production into light absorption, charge separation and fuel production by individual parts of the molecule, mechanistic understanding of the performance limit...
| Main Authors: | , , , , , , |
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| Format: | Article |
| Language: | English |
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Nature Portfolio
2022-05-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-022-30147-4 |
| _version_ | 1811235389836361728 |
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| author | Linda Zedler Pascal Wintergerst Alexander K. Mengele Carolin Müller Chunyu Li Benjamin Dietzek-Ivanšić Sven Rau |
| author_facet | Linda Zedler Pascal Wintergerst Alexander K. Mengele Carolin Müller Chunyu Li Benjamin Dietzek-Ivanšić Sven Rau |
| author_sort | Linda Zedler |
| collection | DOAJ |
| description | Although multinuclear, supramolecular photocatalysts show promise in their ability to separate the processes required for lightdriven energy production into light absorption, charge separation and fuel production by individual parts of the molecule, mechanistic understanding of the performance limiting processes are lacking. Here the authors synthesize two new dinuclear catalysts and compare them to a benchmark through detailed spectroscopic studies, obtaining significant chemical insight. |
| first_indexed | 2024-04-12T11:50:05Z |
| format | Article |
| id | doaj.art-055004a4482e43e7b67b54ca8edfb9df |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-04-12T11:50:05Z |
| publishDate | 2022-05-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-055004a4482e43e7b67b54ca8edfb9df2022-12-22T03:34:11ZengNature PortfolioNature Communications2041-17232022-05-0113111310.1038/s41467-022-30147-4Outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalystLinda Zedler0Pascal Wintergerst1Alexander K. Mengele2Carolin Müller3Chunyu Li4Benjamin Dietzek-Ivanšić5Sven Rau6Institute of Physical Chemistry, Friedrich Schiller University JenaInstitute of Inorganic Chemistry I, Materials and Catalysis, Ulm UniversityInstitute of Inorganic Chemistry I, Materials and Catalysis, Ulm UniversityInstitute of Physical Chemistry, Friedrich Schiller University JenaInstitute of Physical Chemistry, Friedrich Schiller University JenaInstitute of Physical Chemistry, Friedrich Schiller University JenaInstitute of Inorganic Chemistry I, Materials and Catalysis, Ulm UniversityAlthough multinuclear, supramolecular photocatalysts show promise in their ability to separate the processes required for lightdriven energy production into light absorption, charge separation and fuel production by individual parts of the molecule, mechanistic understanding of the performance limiting processes are lacking. Here the authors synthesize two new dinuclear catalysts and compare them to a benchmark through detailed spectroscopic studies, obtaining significant chemical insight.https://doi.org/10.1038/s41467-022-30147-4 |
| spellingShingle | Linda Zedler Pascal Wintergerst Alexander K. Mengele Carolin Müller Chunyu Li Benjamin Dietzek-Ivanšić Sven Rau Outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalyst Nature Communications |
| title | Outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalyst |
| title_full | Outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalyst |
| title_fullStr | Outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalyst |
| title_full_unstemmed | Outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalyst |
| title_short | Outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalyst |
| title_sort | outpacing conventional nicotinamide hydrogenation catalysis by a strongly communicating heterodinuclear photocatalyst |
| url | https://doi.org/10.1038/s41467-022-30147-4 |
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