Classification of second harmonic generation effect in magnetically ordered materials

Abstract The relationship between magnetic order and the second harmonic generation (SHG) effect is a fundamental area of study in condensed matter physics with significant practical implications. In order to gain a clearer understanding of this intricate relation, this study presents a comprehensiv...

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Main Authors: Rui-Chun Xiao, Ding-Fu Shao, Wei Gan, Huan-Wen Wang, Hui Han, Z. G. Sheng, Changjin Zhang, Hua Jiang, Hui Li
Format: Article
Language:English
Published: Nature Portfolio 2023-10-01
Series:npj Quantum Materials
Online Access:https://doi.org/10.1038/s41535-023-00594-3
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author Rui-Chun Xiao
Ding-Fu Shao
Wei Gan
Huan-Wen Wang
Hui Han
Z. G. Sheng
Changjin Zhang
Hua Jiang
Hui Li
author_facet Rui-Chun Xiao
Ding-Fu Shao
Wei Gan
Huan-Wen Wang
Hui Han
Z. G. Sheng
Changjin Zhang
Hua Jiang
Hui Li
author_sort Rui-Chun Xiao
collection DOAJ
description Abstract The relationship between magnetic order and the second harmonic generation (SHG) effect is a fundamental area of study in condensed matter physics with significant practical implications. In order to gain a clearer understanding of this intricate relation, this study presents a comprehensive classification scheme for the SHG effect in magnetically ordered materials. This framework offers a straightforward approach to connecting magnetic order and the SHG effect. The characteristics of the SHG tensors in all magnetic point groups are studied using the isomorphic group method, followed by a comprehensive SHG effect classification scheme that includes seven types based on the symmetries of the magnetic phases and their corresponding parent phases. In addition, a tensor dictionary containing the SHG and linear magneto-optic (LMO) effect is established. Furthermore, an extensive SHG database of magnetically ordered materials is also built up. This classification strategy exposes an anomalous SHG effect with even characteristics (i.e., invariant) under time-reversal symmetry, which is solely contributed by magnetic structure. Moreover, the proposed classification scheme facilitates the determination of magnetic structures through the SHG effect.
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spelling doaj.art-07497ae78fdb491abbfe6956611cac5b2023-11-19T12:17:03ZengNature Portfolionpj Quantum Materials2397-46482023-10-01811910.1038/s41535-023-00594-3Classification of second harmonic generation effect in magnetically ordered materialsRui-Chun Xiao0Ding-Fu Shao1Wei Gan2Huan-Wen Wang3Hui Han4Z. G. Sheng5Changjin Zhang6Hua Jiang7Hui Li8Institute of Physical Science and Information Technology, Anhui UniversityKey Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of SciencesInstitute of Physical Science and Information Technology, Anhui UniversitySchool of Physics, University of Electronic Science and Technology of ChinaInstitute of Physical Science and Information Technology, Anhui UniversityHigh Magnetic Field Laboratory, Chinese Academy of SciencesInstitute of Physical Science and Information Technology, Anhui UniversityInstitute for Advanced Study, Soochow UniversityInstitute of Physical Science and Information Technology, Anhui UniversityAbstract The relationship between magnetic order and the second harmonic generation (SHG) effect is a fundamental area of study in condensed matter physics with significant practical implications. In order to gain a clearer understanding of this intricate relation, this study presents a comprehensive classification scheme for the SHG effect in magnetically ordered materials. This framework offers a straightforward approach to connecting magnetic order and the SHG effect. The characteristics of the SHG tensors in all magnetic point groups are studied using the isomorphic group method, followed by a comprehensive SHG effect classification scheme that includes seven types based on the symmetries of the magnetic phases and their corresponding parent phases. In addition, a tensor dictionary containing the SHG and linear magneto-optic (LMO) effect is established. Furthermore, an extensive SHG database of magnetically ordered materials is also built up. This classification strategy exposes an anomalous SHG effect with even characteristics (i.e., invariant) under time-reversal symmetry, which is solely contributed by magnetic structure. Moreover, the proposed classification scheme facilitates the determination of magnetic structures through the SHG effect.https://doi.org/10.1038/s41535-023-00594-3
spellingShingle Rui-Chun Xiao
Ding-Fu Shao
Wei Gan
Huan-Wen Wang
Hui Han
Z. G. Sheng
Changjin Zhang
Hua Jiang
Hui Li
Classification of second harmonic generation effect in magnetically ordered materials
npj Quantum Materials
title Classification of second harmonic generation effect in magnetically ordered materials
title_full Classification of second harmonic generation effect in magnetically ordered materials
title_fullStr Classification of second harmonic generation effect in magnetically ordered materials
title_full_unstemmed Classification of second harmonic generation effect in magnetically ordered materials
title_short Classification of second harmonic generation effect in magnetically ordered materials
title_sort classification of second harmonic generation effect in magnetically ordered materials
url https://doi.org/10.1038/s41535-023-00594-3
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