Single-order laser high harmonics in XUV for ultrafast photoelectron spectroscopy of molecular wavepacket dynamics
We present applications of extreme ultraviolet (XUV) single-order laser harmonics to gas-phase ultrafast photoelectron spectroscopy. Ultrashort XUV pulses at 80 nm are obtained as the 5th order harmonics of the fundamental laser at 400 nm by using Xe or Kr as the nonlinear medium and separated from...
Main Authors: | , |
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Format: | Article |
Language: | English |
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AIP Publishing LLC and ACA
2016-11-01
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Series: | Structural Dynamics |
Online Access: | http://dx.doi.org/10.1063/1.4964775 |
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author | Mizuho Fushitani Akiyoshi Hishikawa |
author_facet | Mizuho Fushitani Akiyoshi Hishikawa |
author_sort | Mizuho Fushitani |
collection | DOAJ |
description | We present applications of extreme ultraviolet (XUV) single-order laser harmonics to gas-phase ultrafast photoelectron spectroscopy. Ultrashort XUV pulses at 80 nm are obtained as the 5th order harmonics of the fundamental laser at 400 nm by using Xe or Kr as the nonlinear medium and separated from other harmonic orders by using an indium foil. The single-order laser harmonics is applied for real-time probing of vibrational wavepacket dynamics of I2 molecules in the bound and dissociating low-lying electronic states and electronic-vibrational wavepacket dynamics of highly excited Rydberg N2 molecules. |
first_indexed | 2024-12-20T09:48:18Z |
format | Article |
id | doaj.art-0785fcf8acc5467fb9447b86d763c3d1 |
institution | Directory Open Access Journal |
issn | 2329-7778 |
language | English |
last_indexed | 2024-12-20T09:48:18Z |
publishDate | 2016-11-01 |
publisher | AIP Publishing LLC and ACA |
record_format | Article |
series | Structural Dynamics |
spelling | doaj.art-0785fcf8acc5467fb9447b86d763c3d12022-12-21T19:44:40ZengAIP Publishing LLC and ACAStructural Dynamics2329-77782016-11-0136062602062602-1110.1063/1.4964775002694SDYSingle-order laser high harmonics in XUV for ultrafast photoelectron spectroscopy of molecular wavepacket dynamicsMizuho Fushitani0Akiyoshi Hishikawa1 Department of Chemistry, Nagoya University, Furo-cho, Chikusa, Nagoya, Aichi 464-8602, Japan Department of Chemistry, Nagoya University, Furo-cho, Chikusa, Nagoya, Aichi 464-8602, JapanWe present applications of extreme ultraviolet (XUV) single-order laser harmonics to gas-phase ultrafast photoelectron spectroscopy. Ultrashort XUV pulses at 80 nm are obtained as the 5th order harmonics of the fundamental laser at 400 nm by using Xe or Kr as the nonlinear medium and separated from other harmonic orders by using an indium foil. The single-order laser harmonics is applied for real-time probing of vibrational wavepacket dynamics of I2 molecules in the bound and dissociating low-lying electronic states and electronic-vibrational wavepacket dynamics of highly excited Rydberg N2 molecules.http://dx.doi.org/10.1063/1.4964775 |
spellingShingle | Mizuho Fushitani Akiyoshi Hishikawa Single-order laser high harmonics in XUV for ultrafast photoelectron spectroscopy of molecular wavepacket dynamics Structural Dynamics |
title | Single-order laser high harmonics in XUV for ultrafast photoelectron spectroscopy of molecular wavepacket dynamics |
title_full | Single-order laser high harmonics in XUV for ultrafast photoelectron spectroscopy of molecular wavepacket dynamics |
title_fullStr | Single-order laser high harmonics in XUV for ultrafast photoelectron spectroscopy of molecular wavepacket dynamics |
title_full_unstemmed | Single-order laser high harmonics in XUV for ultrafast photoelectron spectroscopy of molecular wavepacket dynamics |
title_short | Single-order laser high harmonics in XUV for ultrafast photoelectron spectroscopy of molecular wavepacket dynamics |
title_sort | single order laser high harmonics in xuv for ultrafast photoelectron spectroscopy of molecular wavepacket dynamics |
url | http://dx.doi.org/10.1063/1.4964775 |
work_keys_str_mv | AT mizuhofushitani singleorderlaserhighharmonicsinxuvforultrafastphotoelectronspectroscopyofmolecularwavepacketdynamics AT akiyoshihishikawa singleorderlaserhighharmonicsinxuvforultrafastphotoelectronspectroscopyofmolecularwavepacketdynamics |