Atmospheric aerosol characterization with a ground-based SPEX spectropolarimetric instrument

Characterization of atmospheric aerosols is important for understanding their impact on health and climate. A wealth of aerosol parameters can be retrieved from multi-angle, multi-wavelength radiance and polarization measurements of the clear sky. We developed a ground-based SPEX instrument (groundS...

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Main Authors: G. van Harten, J. de Boer, J. H. H. Rietjens, A. Di Noia, F. Snik, H. Volten, J. M. Smit, O. P. Hasekamp, J. S. Henzing, C. U. Keller
Format: Article
Language:English
Published: Copernicus Publications 2014-12-01
Series:Atmospheric Measurement Techniques
Online Access:http://www.atmos-meas-tech.net/7/4341/2014/amt-7-4341-2014.pdf
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author G. van Harten
J. de Boer
J. H. H. Rietjens
A. Di Noia
F. Snik
H. Volten
J. M. Smit
O. P. Hasekamp
J. S. Henzing
C. U. Keller
author_facet G. van Harten
J. de Boer
J. H. H. Rietjens
A. Di Noia
F. Snik
H. Volten
J. M. Smit
O. P. Hasekamp
J. S. Henzing
C. U. Keller
author_sort G. van Harten
collection DOAJ
description Characterization of atmospheric aerosols is important for understanding their impact on health and climate. A wealth of aerosol parameters can be retrieved from multi-angle, multi-wavelength radiance and polarization measurements of the clear sky. We developed a ground-based SPEX instrument (groundSPEX) for accurate spectropolarimetry, based on the passive, robust, athermal, and snapshot spectral polarization modulation technique, and is hence ideal for field deployment. It samples the scattering phase function in the principal plane in an automated fashion, using a motorized pan/tilt unit and automatic exposure time detection. Extensive radiometric and polarimetric calibrations were performed, yielding values for both random noise and systematic uncertainties. The absolute polarimetric accuracy at low degrees of polarization is established to be ~5 &times; 10<sup>&minus;3</sup>. About 70 measurement sequences have been performed throughout four clear-sky days at Cabauw, the Netherlands. Several aerosol parameters were retrieved: aerosol optical thickness, effective radius, and complex refractive index for fine and coarse mode. The results are in good agreement with the colocated AERONET products, with a correlation coefficient of &rho; = 0.932 for the total aerosol optical thickness at 550 nm.
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spelling doaj.art-0856ec8d19ac40cba9ddfe29fd9057472022-12-21T17:57:07ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482014-12-017124341435110.5194/amt-7-4341-2014Atmospheric aerosol characterization with a ground-based SPEX spectropolarimetric instrumentG. van Harten0J. de Boer1J. H. H. Rietjens2A. Di Noia3F. Snik4H. Volten5J. M. Smit6O. P. Hasekamp7J. S. Henzing8C. U. Keller9Leiden Observatory, Leiden University, Leiden, the NetherlandsLeiden Observatory, Leiden University, Leiden, the NetherlandsSRON Netherlands Institute for Space Research, Utrecht, the NetherlandsSRON Netherlands Institute for Space Research, Utrecht, the NetherlandsLeiden Observatory, Leiden University, Leiden, the NetherlandsCentre for Environmental Quality, National Institute for Public Health and the Environment (RIVM), Bilthoven, the NetherlandsSRON Netherlands Institute for Space Research, Utrecht, the NetherlandsSRON Netherlands Institute for Space Research, Utrecht, the NetherlandsNetherlands Institute for Applied Scientific Research – TNO, Utrecht, the NetherlandsLeiden Observatory, Leiden University, Leiden, the NetherlandsCharacterization of atmospheric aerosols is important for understanding their impact on health and climate. A wealth of aerosol parameters can be retrieved from multi-angle, multi-wavelength radiance and polarization measurements of the clear sky. We developed a ground-based SPEX instrument (groundSPEX) for accurate spectropolarimetry, based on the passive, robust, athermal, and snapshot spectral polarization modulation technique, and is hence ideal for field deployment. It samples the scattering phase function in the principal plane in an automated fashion, using a motorized pan/tilt unit and automatic exposure time detection. Extensive radiometric and polarimetric calibrations were performed, yielding values for both random noise and systematic uncertainties. The absolute polarimetric accuracy at low degrees of polarization is established to be ~5 &times; 10<sup>&minus;3</sup>. About 70 measurement sequences have been performed throughout four clear-sky days at Cabauw, the Netherlands. Several aerosol parameters were retrieved: aerosol optical thickness, effective radius, and complex refractive index for fine and coarse mode. The results are in good agreement with the colocated AERONET products, with a correlation coefficient of &rho; = 0.932 for the total aerosol optical thickness at 550 nm.http://www.atmos-meas-tech.net/7/4341/2014/amt-7-4341-2014.pdf
spellingShingle G. van Harten
J. de Boer
J. H. H. Rietjens
A. Di Noia
F. Snik
H. Volten
J. M. Smit
O. P. Hasekamp
J. S. Henzing
C. U. Keller
Atmospheric aerosol characterization with a ground-based SPEX spectropolarimetric instrument
Atmospheric Measurement Techniques
title Atmospheric aerosol characterization with a ground-based SPEX spectropolarimetric instrument
title_full Atmospheric aerosol characterization with a ground-based SPEX spectropolarimetric instrument
title_fullStr Atmospheric aerosol characterization with a ground-based SPEX spectropolarimetric instrument
title_full_unstemmed Atmospheric aerosol characterization with a ground-based SPEX spectropolarimetric instrument
title_short Atmospheric aerosol characterization with a ground-based SPEX spectropolarimetric instrument
title_sort atmospheric aerosol characterization with a ground based spex spectropolarimetric instrument
url http://www.atmos-meas-tech.net/7/4341/2014/amt-7-4341-2014.pdf
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