Solvothermal synthesis-driven quaternary Ni-rich cathode for stability-improved Li-ion batteries

Recently, Ni-rich ternary transition metal oxides (Li(NiCoMn)O2, NCM) containing more than 80% Ni have been extensively studied as high-capacity cathodes. Herein, we synthesized a quaternary cathode, Ni-rich Al-doped NCM, using a facile solvothermal method without an additional Al doping process. Co...

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Main Authors: Sung-Beom Kim, So-Yeon Ahn, Ji-Hwan Kim, Jae-Sung Jang, Kyung-Won Park
Format: Article
Language:English
Published: Elsevier 2023-01-01
Series:Electrochemistry Communications
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S1388248122002284
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author Sung-Beom Kim
So-Yeon Ahn
Ji-Hwan Kim
Jae-Sung Jang
Kyung-Won Park
author_facet Sung-Beom Kim
So-Yeon Ahn
Ji-Hwan Kim
Jae-Sung Jang
Kyung-Won Park
author_sort Sung-Beom Kim
collection DOAJ
description Recently, Ni-rich ternary transition metal oxides (Li(NiCoMn)O2, NCM) containing more than 80% Ni have been extensively studied as high-capacity cathodes. Herein, we synthesized a quaternary cathode, Ni-rich Al-doped NCM, using a facile solvothermal method without an additional Al doping process. Compared to an undoped NCM cathode, the quaternary Ni-rich cathode exhibited improved lithium-ion battery performance (retentions of 82.0% and 65.8% after 100 and 250 cycles, respectively). In particular, the superior stability of the quaternary Ni-rich cathode may result from the stable cathode structure resulting from Al doping.
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spelling doaj.art-086ad98f82d4443a83639b76cb4356be2023-01-08T04:13:47ZengElsevierElectrochemistry Communications1388-24812023-01-01146107426Solvothermal synthesis-driven quaternary Ni-rich cathode for stability-improved Li-ion batteriesSung-Beom Kim0So-Yeon Ahn1Ji-Hwan Kim2Jae-Sung Jang3Kyung-Won Park4Department of Chemical Engineering, Soongsil University, Seoul 06978, Republic of KoreaDepartment of Chemical Engineering, Soongsil University, Seoul 06978, Republic of KoreaDepartment of Chemical Engineering, Soongsil University, Seoul 06978, Republic of KoreaDepartment of Chemical Engineering, Soongsil University, Seoul 06978, Republic of KoreaCorresponding author.; Department of Chemical Engineering, Soongsil University, Seoul 06978, Republic of KoreaRecently, Ni-rich ternary transition metal oxides (Li(NiCoMn)O2, NCM) containing more than 80% Ni have been extensively studied as high-capacity cathodes. Herein, we synthesized a quaternary cathode, Ni-rich Al-doped NCM, using a facile solvothermal method without an additional Al doping process. Compared to an undoped NCM cathode, the quaternary Ni-rich cathode exhibited improved lithium-ion battery performance (retentions of 82.0% and 65.8% after 100 and 250 cycles, respectively). In particular, the superior stability of the quaternary Ni-rich cathode may result from the stable cathode structure resulting from Al doping.http://www.sciencedirect.com/science/article/pii/S1388248122002284Lithium-ion batteriesQuaternary Ni-rich cathodeAluminum dopingSolvothermal synthesis
spellingShingle Sung-Beom Kim
So-Yeon Ahn
Ji-Hwan Kim
Jae-Sung Jang
Kyung-Won Park
Solvothermal synthesis-driven quaternary Ni-rich cathode for stability-improved Li-ion batteries
Electrochemistry Communications
Lithium-ion batteries
Quaternary Ni-rich cathode
Aluminum doping
Solvothermal synthesis
title Solvothermal synthesis-driven quaternary Ni-rich cathode for stability-improved Li-ion batteries
title_full Solvothermal synthesis-driven quaternary Ni-rich cathode for stability-improved Li-ion batteries
title_fullStr Solvothermal synthesis-driven quaternary Ni-rich cathode for stability-improved Li-ion batteries
title_full_unstemmed Solvothermal synthesis-driven quaternary Ni-rich cathode for stability-improved Li-ion batteries
title_short Solvothermal synthesis-driven quaternary Ni-rich cathode for stability-improved Li-ion batteries
title_sort solvothermal synthesis driven quaternary ni rich cathode for stability improved li ion batteries
topic Lithium-ion batteries
Quaternary Ni-rich cathode
Aluminum doping
Solvothermal synthesis
url http://www.sciencedirect.com/science/article/pii/S1388248122002284
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AT jihwankim solvothermalsynthesisdrivenquaternarynirichcathodeforstabilityimprovedliionbatteries
AT jaesungjang solvothermalsynthesisdrivenquaternarynirichcathodeforstabilityimprovedliionbatteries
AT kyungwonpark solvothermalsynthesisdrivenquaternarynirichcathodeforstabilityimprovedliionbatteries