Strong correlation between uniaxial magnetic anisotropic constant and in-plane tensile strain in Mn4N epitaxial films

Ferrimagnetic Mn4N is a promising candidate for current-induced domain wall motion assisted by spin-transfer and spin–orbit torques. Mn4N can be doped to have perpendicular magnetic anisotropy (PMA) and a small spontaneous magnetization. However, the origin of the PMA of Mn4N has yet to be fully und...

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Main Authors: Taku Hirose, Taro Komori, Toshiki Gushi, Akihito Anzai, Kaoru Toko, Takashi Suemasu
Format: Article
Language:English
Published: AIP Publishing LLC 2020-02-01
Series:AIP Advances
Online Access:http://dx.doi.org/10.1063/1.5141818
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author Taku Hirose
Taro Komori
Toshiki Gushi
Akihito Anzai
Kaoru Toko
Takashi Suemasu
author_facet Taku Hirose
Taro Komori
Toshiki Gushi
Akihito Anzai
Kaoru Toko
Takashi Suemasu
author_sort Taku Hirose
collection DOAJ
description Ferrimagnetic Mn4N is a promising candidate for current-induced domain wall motion assisted by spin-transfer and spin–orbit torques. Mn4N can be doped to have perpendicular magnetic anisotropy (PMA) and a small spontaneous magnetization. However, the origin of the PMA of Mn4N has yet to be fully understood. Here, we investigated the relationship between the ratios of the perpendicular lattice constant c to the in-plane lattice constant a of Mn4N epitaxial thin films (c/a) and the uniaxial magnetic anisotropic constant (Ku) in Mn4N thin films grown on MgO(001), SrTiO3(001), and LaAlO3(001) substrates. The lattice mismatches between Mn4N and these substrates are approximately −6%, −0.1%, and +2%, respectively. All the Mn4N thin films had PMA and in-plane tensile distortion (c/a < 1) regardless of the Mn4N thickness and substrate. Although the magnitude of c/a depended on several factors, such as the Mn4N layer thickness and substrate, we found a strong correlation between c/a and Ku; Ku increased markedly when c/a deviated from 1. This result indicates that the origin of PMA is tensile distortion in Mn4N films; hence, it might be possible to control the magnitude of Ku by tuning c/a through the Mn4N layer thickness and the substrate.
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spelling doaj.art-0877b7b40df9434b9936c127fcd0683f2022-12-22T01:59:54ZengAIP Publishing LLCAIP Advances2158-32262020-02-01102025117025117-610.1063/1.5141818Strong correlation between uniaxial magnetic anisotropic constant and in-plane tensile strain in Mn4N epitaxial filmsTaku Hirose0Taro Komori1Toshiki Gushi2Akihito Anzai3Kaoru Toko4Takashi Suemasu5Institute of Applied Physics, Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanInstitute of Applied Physics, Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanInstitute of Applied Physics, Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanInstitute of Applied Physics, Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanInstitute of Applied Physics, Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanInstitute of Applied Physics, Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanFerrimagnetic Mn4N is a promising candidate for current-induced domain wall motion assisted by spin-transfer and spin–orbit torques. Mn4N can be doped to have perpendicular magnetic anisotropy (PMA) and a small spontaneous magnetization. However, the origin of the PMA of Mn4N has yet to be fully understood. Here, we investigated the relationship between the ratios of the perpendicular lattice constant c to the in-plane lattice constant a of Mn4N epitaxial thin films (c/a) and the uniaxial magnetic anisotropic constant (Ku) in Mn4N thin films grown on MgO(001), SrTiO3(001), and LaAlO3(001) substrates. The lattice mismatches between Mn4N and these substrates are approximately −6%, −0.1%, and +2%, respectively. All the Mn4N thin films had PMA and in-plane tensile distortion (c/a < 1) regardless of the Mn4N thickness and substrate. Although the magnitude of c/a depended on several factors, such as the Mn4N layer thickness and substrate, we found a strong correlation between c/a and Ku; Ku increased markedly when c/a deviated from 1. This result indicates that the origin of PMA is tensile distortion in Mn4N films; hence, it might be possible to control the magnitude of Ku by tuning c/a through the Mn4N layer thickness and the substrate.http://dx.doi.org/10.1063/1.5141818
spellingShingle Taku Hirose
Taro Komori
Toshiki Gushi
Akihito Anzai
Kaoru Toko
Takashi Suemasu
Strong correlation between uniaxial magnetic anisotropic constant and in-plane tensile strain in Mn4N epitaxial films
AIP Advances
title Strong correlation between uniaxial magnetic anisotropic constant and in-plane tensile strain in Mn4N epitaxial films
title_full Strong correlation between uniaxial magnetic anisotropic constant and in-plane tensile strain in Mn4N epitaxial films
title_fullStr Strong correlation between uniaxial magnetic anisotropic constant and in-plane tensile strain in Mn4N epitaxial films
title_full_unstemmed Strong correlation between uniaxial magnetic anisotropic constant and in-plane tensile strain in Mn4N epitaxial films
title_short Strong correlation between uniaxial magnetic anisotropic constant and in-plane tensile strain in Mn4N epitaxial films
title_sort strong correlation between uniaxial magnetic anisotropic constant and in plane tensile strain in mn4n epitaxial films
url http://dx.doi.org/10.1063/1.5141818
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