Pt1 enhanced C-H activation synergistic with Ptn catalysis for glycerol cascade oxidation to glyceric acid
The selective oxidation of glycerol to glyceric acid is an important value-added cascade catalytic process. Here the authors report a cascade synergistic catalysis strategy by atomic and low-coordinated cluster Pt on well-defined Cu-CuZrOx to simultaneously achieve high activity and selectivity.
Main Authors: | , , , , , , , , , , , |
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Format: | Article |
Language: | English |
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Nature Portfolio
2022-09-01
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Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-022-33038-w |
_version_ | 1811267540131774464 |
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author | Zhe An Zilong Zhang Zeyu Huang Hongbo Han Binbin Song Jian Zhang Qi Ping Yanru Zhu Hongyan Song Bin Wang Lirong Zheng Jing He |
author_facet | Zhe An Zilong Zhang Zeyu Huang Hongbo Han Binbin Song Jian Zhang Qi Ping Yanru Zhu Hongyan Song Bin Wang Lirong Zheng Jing He |
author_sort | Zhe An |
collection | DOAJ |
description | The selective oxidation of glycerol to glyceric acid is an important value-added cascade catalytic process. Here the authors report a cascade synergistic catalysis strategy by atomic and low-coordinated cluster Pt on well-defined Cu-CuZrOx to simultaneously achieve high activity and selectivity. |
first_indexed | 2024-04-12T21:04:20Z |
format | Article |
id | doaj.art-08c9b7d9cb424e2b9dc6113397ae79b3 |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-04-12T21:04:20Z |
publishDate | 2022-09-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-08c9b7d9cb424e2b9dc6113397ae79b32022-12-22T03:16:45ZengNature PortfolioNature Communications2041-17232022-09-0113111310.1038/s41467-022-33038-wPt1 enhanced C-H activation synergistic with Ptn catalysis for glycerol cascade oxidation to glyceric acidZhe An0Zilong Zhang1Zeyu Huang2Hongbo Han3Binbin Song4Jian Zhang5Qi Ping6Yanru Zhu7Hongyan Song8Bin Wang9Lirong Zheng10Jing He11State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyBeijing Research Institute of Chemical Industry, Sinopec GroupTechnology Institute of High Energy Physics, Chinese Academy of SciencesState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical TechnologyThe selective oxidation of glycerol to glyceric acid is an important value-added cascade catalytic process. Here the authors report a cascade synergistic catalysis strategy by atomic and low-coordinated cluster Pt on well-defined Cu-CuZrOx to simultaneously achieve high activity and selectivity.https://doi.org/10.1038/s41467-022-33038-w |
spellingShingle | Zhe An Zilong Zhang Zeyu Huang Hongbo Han Binbin Song Jian Zhang Qi Ping Yanru Zhu Hongyan Song Bin Wang Lirong Zheng Jing He Pt1 enhanced C-H activation synergistic with Ptn catalysis for glycerol cascade oxidation to glyceric acid Nature Communications |
title | Pt1 enhanced C-H activation synergistic with Ptn catalysis for glycerol cascade oxidation to glyceric acid |
title_full | Pt1 enhanced C-H activation synergistic with Ptn catalysis for glycerol cascade oxidation to glyceric acid |
title_fullStr | Pt1 enhanced C-H activation synergistic with Ptn catalysis for glycerol cascade oxidation to glyceric acid |
title_full_unstemmed | Pt1 enhanced C-H activation synergistic with Ptn catalysis for glycerol cascade oxidation to glyceric acid |
title_short | Pt1 enhanced C-H activation synergistic with Ptn catalysis for glycerol cascade oxidation to glyceric acid |
title_sort | pt1 enhanced c h activation synergistic with ptn catalysis for glycerol cascade oxidation to glyceric acid |
url | https://doi.org/10.1038/s41467-022-33038-w |
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