A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water
<p>We present the laboratory results of immersion freezing efficiencies of cellulose particles at supercooled temperature (<span class="inline-formula"><i>T</i>)</span> conditions. Three types of chemically homogeneous cellulose samples are used as surrogates...
| Main Authors: | , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Copernicus Publications
2019-04-01
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| Series: | Atmospheric Chemistry and Physics |
| Online Access: | https://www.atmos-chem-phys.net/19/4823/2019/acp-19-4823-2019.pdf |
| _version_ | 1828528969435054080 |
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| author | N. Hiranuma K. Adachi D. M. Bell D. M. Bell F. Belosi H. Beydoun B. Bhaduri B. Bhaduri H. Bingemer C. Budke H.-C. Clemen F. Conen K. M. Cory J. Curtius P. J. DeMott O. Eppers S. Grawe S. Hartmann N. Hoffmann K. Höhler E. Jantsch A. Kiselev T. Koop G. Kulkarni A. Mayer M. Murakami M. Murakami B. J. Murray A. Nicosia A. Nicosia M. D. Petters M. Piazza M. Polen N. Reicher Y. Rudich A. Saito G. Santachiara T. Schiebel G. P. Schill J. Schneider L. Segev E. Stopelli E. Stopelli R. C. Sullivan K. Suski K. Suski M. Szakáll T. Tajiri H. Taylor Y. Tobo Y. Tobo R. Ullrich D. Weber H. Wex T. F. Whale C. L. Whiteside K. Yamashita K. Yamashita A. Zelenyuk O. Möhler |
| author_facet | N. Hiranuma K. Adachi D. M. Bell D. M. Bell F. Belosi H. Beydoun B. Bhaduri B. Bhaduri H. Bingemer C. Budke H.-C. Clemen F. Conen K. M. Cory J. Curtius P. J. DeMott O. Eppers S. Grawe S. Hartmann N. Hoffmann K. Höhler E. Jantsch A. Kiselev T. Koop G. Kulkarni A. Mayer M. Murakami M. Murakami B. J. Murray A. Nicosia A. Nicosia M. D. Petters M. Piazza M. Polen N. Reicher Y. Rudich A. Saito G. Santachiara T. Schiebel G. P. Schill J. Schneider L. Segev E. Stopelli E. Stopelli R. C. Sullivan K. Suski K. Suski M. Szakáll T. Tajiri H. Taylor Y. Tobo Y. Tobo R. Ullrich D. Weber H. Wex T. F. Whale C. L. Whiteside K. Yamashita K. Yamashita A. Zelenyuk O. Möhler |
| author_sort | N. Hiranuma |
| collection | DOAJ |
| description | <p>We present the laboratory results of immersion freezing efficiencies of
cellulose particles at supercooled temperature (<span class="inline-formula"><i>T</i>)</span> conditions. Three types of
chemically homogeneous cellulose samples are used as surrogates that
represent supermicron and submicron ice-nucleating plant structural
polymers. These samples include microcrystalline cellulose (MCC), fibrous
cellulose (FC) and nanocrystalline cellulose (NCC). Our immersion freezing
dataset includes data from various ice nucleation measurement techniques
available at 17 different institutions, including nine dry dispersion
and 11 aqueous suspension techniques. With a total of 20 methods, we
performed systematic accuracy and precision analysis of measurements from
all 20 measurement techniques by evaluating <span class="inline-formula"><i>T</i></span>-binned (1 <span class="inline-formula"><sup>∘</sup></span>C)
data over a wide <span class="inline-formula"><i>T</i></span> range (<span class="inline-formula">−</span>36 <span class="inline-formula"><sup>∘</sup></span>C <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M7" display="inline" overflow="scroll" dspmath="mathml"><mrow><mo><</mo><mi>T</mi><mo><</mo><mo>-</mo><mn mathvariant="normal">4</mn></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="46pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="3b7a6b6ea4e55ac45ae2885dad986a21"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-19-4823-2019-ie00001.svg" width="46pt" height="10pt" src="acp-19-4823-2019-ie00001.png"/></svg:svg></span></span> <span class="inline-formula"><sup>∘</sup></span>C). Specifically, we intercompared the geometric surface
area-based ice nucleation active surface site (INAS) density data derived from
our measurements as a function of <span class="inline-formula"><i>T</i></span>, <span class="inline-formula"><i>n</i><sub>s,geo</sub>(<i>T</i>)</span>. Additionally, we also
compared the <span class="inline-formula"><i>n</i><sub>s,geo</sub>(<i>T</i>)</span> values and the freezing spectral slope parameter
(<span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M12" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="normal">Δ</mi><mi mathvariant="normal">log</mi><mo>(</mo><msub><mi>n</mi><mrow><mi mathvariant="normal">s</mi><mo>,</mo><mi mathvariant="normal">geo</mi></mrow></msub><mo>)</mo><mo>/</mo><mi mathvariant="normal">Δ</mi><mi>T</mi><mo>)</mo></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="83pt" height="16pt" class="svg-formula" dspmath="mathimg" md5hash="8ec71e136abcca72f65a4b88c200015b"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-19-4823-2019-ie00002.svg" width="83pt" height="16pt" src="acp-19-4823-2019-ie00002.png"/></svg:svg></span></span> from our measurements to previous
literature results. Results show all three cellulose materials are
reasonably ice active. The freezing efficiencies of NCC samples agree
reasonably well, whereas the diversity for the other two samples spans
<span class="inline-formula">≈</span> 10 <span class="inline-formula"><sup>∘</sup></span>C. Despite given uncertainties within each
instrument technique, the overall trend of the <span class="inline-formula"><i>n</i><sub>s,geo</sub>(<i>T</i>)</span> spectrum traced
by the <span class="inline-formula"><i>T</i></span>-binned average of measurements suggests that predominantly
supermicron-sized cellulose particles (MCC and FC) generally act as more
efficient ice-nucleating particles (INPs) than NCC with about 1 order of
magnitude higher <span class="inline-formula"><i>n</i><sub>s,geo</sub>(<i>T</i>)</span>.</p> |
| first_indexed | 2024-12-11T22:00:25Z |
| format | Article |
| id | doaj.art-08f06bde9b57423cbfa05e229f398727 |
| institution | Directory Open Access Journal |
| issn | 1680-7316 1680-7324 |
| language | English |
| last_indexed | 2024-12-11T22:00:25Z |
| publishDate | 2019-04-01 |
| publisher | Copernicus Publications |
| record_format | Article |
| series | Atmospheric Chemistry and Physics |
| spelling | doaj.art-08f06bde9b57423cbfa05e229f3987272022-12-22T00:49:07ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242019-04-01194823484910.5194/acp-19-4823-2019A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in waterN. Hiranuma0K. Adachi1D. M. Bell2D. M. Bell3F. Belosi4H. Beydoun5B. Bhaduri6B. Bhaduri7H. Bingemer8C. Budke9H.-C. Clemen10F. Conen11K. M. Cory12J. Curtius13P. J. DeMott14O. Eppers15S. Grawe16S. Hartmann17N. Hoffmann18K. Höhler19E. Jantsch20A. Kiselev21T. Koop22G. Kulkarni23A. Mayer24M. Murakami25M. Murakami26B. J. Murray27A. Nicosia28A. Nicosia29M. D. Petters30M. Piazza31M. Polen32N. Reicher33Y. Rudich34A. Saito35G. Santachiara36T. Schiebel37G. P. Schill38J. Schneider39L. Segev40E. Stopelli41E. Stopelli42R. C. Sullivan43K. Suski44K. Suski45M. Szakáll46T. Tajiri47H. Taylor48Y. Tobo49Y. Tobo50R. Ullrich51D. Weber52H. Wex53T. F. Whale54C. L. Whiteside55K. Yamashita56K. Yamashita57A. Zelenyuk58O. Möhler59Department of Life, Earth and Environmental Sciences, West Texas A&M University, Canyon, TX, USAMeteorological Research Institute (MRI), Tsukuba, JapanPacific Northwest National Laboratory, Richland, WA, USAnow at: Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen, SwitzerlandInstitute of Atmospheric Sciences and Climate, National Research Council, Bologna, ItalyCenter for Atmospheric Particle Studies, Carnegie Mellon University, Pittsburgh, PA, USADepartment of Earth and Planetary Sciences, Weizmann Institute, Rehovot, Israelnow at: Department of Soil and Water Sciences, Hebrew University of Jerusalem, IsraelInstitute for Atmospheric and Environmental Science, Goethe University of Frankfurt, Frankfurt am Main, GermanyFaculty of Chemistry, Bielefeld University, Bielefeld, GermanyMax-Planck-Institut für Chemie, Particle Chemistry Department, Mainz, GermanyEnvironmental Geosciences, University of Basel, Basel, SwitzerlandDepartment of Life, Earth and Environmental Sciences, West Texas A&M University, Canyon, TX, USAInstitute for Atmospheric and Environmental Science, Goethe University of Frankfurt, Frankfurt am Main, GermanyDepartment of Atmospheric Science, Colorado State University, Fort Collins, CO, USAInstitute for Atmospheric Physics, University of Mainz, Mainz, GermanyLeibniz Institute for Tropospheric Research, Leipzig, GermanyLeibniz Institute for Tropospheric Research, Leipzig, GermanyInstitute for Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, GermanyInstitute for Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, GermanyFaculty of Chemistry, Bielefeld University, Bielefeld, GermanyInstitute for Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, GermanyFaculty of Chemistry, Bielefeld University, Bielefeld, GermanyPacific Northwest National Laboratory, Richland, WA, USAInstitute for Atmospheric Physics, University of Mainz, Mainz, GermanyMeteorological Research Institute (MRI), Tsukuba, Japannow at: Institute for Space-Earth Environmental Research, Nagoya University, Nagoya, JapanInstitute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, UKInstitute of Atmospheric Sciences and Climate, National Research Council, Bologna, Italynow at: Laboratoire de Météorologie Physique (Lamp-CNRS) Aubiere, FranceDepartment of Marine, Earth, and Atmospheric Sciences, North Carolina State University Raleigh, Raleigh, NC, USAInstitute of Atmospheric Sciences and Climate, National Research Council, Bologna, ItalyCenter for Atmospheric Particle Studies, Carnegie Mellon University, Pittsburgh, PA, USADepartment of Earth and Planetary Sciences, Weizmann Institute, Rehovot, IsraelDepartment of Earth and Planetary Sciences, Weizmann Institute, Rehovot, IsraelMeteorological Research Institute (MRI), Tsukuba, JapanInstitute of Atmospheric Sciences and Climate, National Research Council, Bologna, ItalyInstitute for Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, GermanyDepartment of Atmospheric Science, Colorado State University, Fort Collins, CO, USAMax-Planck-Institut für Chemie, Particle Chemistry Department, Mainz, GermanyDepartment of Earth and Planetary Sciences, Weizmann Institute, Rehovot, IsraelEnvironmental Geosciences, University of Basel, Basel, Switzerlandnow at: Water Resources and Drinking Water Department, Eawag, Dübendorf, SwitzerlandCenter for Atmospheric Particle Studies, Carnegie Mellon University, Pittsburgh, PA, USAPacific Northwest National Laboratory, Richland, WA, USADepartment of Atmospheric Science, Colorado State University, Fort Collins, CO, USAInstitute for Atmospheric Physics, University of Mainz, Mainz, GermanyMeteorological Research Institute (MRI), Tsukuba, JapanDepartment of Marine, Earth, and Atmospheric Sciences, North Carolina State University Raleigh, Raleigh, NC, USANational Institute of Polar Research, Tachikawa, Tokyo, JapanDepartment of Polar Science, School of Multidisciplinary Sciences, SOKENDAI (The Graduate University for Advanced Studies), Tachikawa, Tokyo, JapanInstitute for Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, GermanyInstitute for Atmospheric and Environmental Science, Goethe University of Frankfurt, Frankfurt am Main, GermanyLeibniz Institute for Tropospheric Research, Leipzig, GermanyInstitute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, UKDepartment of Life, Earth and Environmental Sciences, West Texas A&M University, Canyon, TX, USAMeteorological Research Institute (MRI), Tsukuba, Japannow at: Snow and Ice Research Center, National Research Institute for Earth Science and Disaster, Nagaoka, JapanPacific Northwest National Laboratory, Richland, WA, USAInstitute for Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, Germany<p>We present the laboratory results of immersion freezing efficiencies of cellulose particles at supercooled temperature (<span class="inline-formula"><i>T</i>)</span> conditions. Three types of chemically homogeneous cellulose samples are used as surrogates that represent supermicron and submicron ice-nucleating plant structural polymers. These samples include microcrystalline cellulose (MCC), fibrous cellulose (FC) and nanocrystalline cellulose (NCC). Our immersion freezing dataset includes data from various ice nucleation measurement techniques available at 17 different institutions, including nine dry dispersion and 11 aqueous suspension techniques. With a total of 20 methods, we performed systematic accuracy and precision analysis of measurements from all 20 measurement techniques by evaluating <span class="inline-formula"><i>T</i></span>-binned (1 <span class="inline-formula"><sup>∘</sup></span>C) data over a wide <span class="inline-formula"><i>T</i></span> range (<span class="inline-formula">−</span>36 <span class="inline-formula"><sup>∘</sup></span>C <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M7" display="inline" overflow="scroll" dspmath="mathml"><mrow><mo><</mo><mi>T</mi><mo><</mo><mo>-</mo><mn mathvariant="normal">4</mn></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="46pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="3b7a6b6ea4e55ac45ae2885dad986a21"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-19-4823-2019-ie00001.svg" width="46pt" height="10pt" src="acp-19-4823-2019-ie00001.png"/></svg:svg></span></span> <span class="inline-formula"><sup>∘</sup></span>C). Specifically, we intercompared the geometric surface area-based ice nucleation active surface site (INAS) density data derived from our measurements as a function of <span class="inline-formula"><i>T</i></span>, <span class="inline-formula"><i>n</i><sub>s,geo</sub>(<i>T</i>)</span>. Additionally, we also compared the <span class="inline-formula"><i>n</i><sub>s,geo</sub>(<i>T</i>)</span> values and the freezing spectral slope parameter (<span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M12" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="normal">Δ</mi><mi mathvariant="normal">log</mi><mo>(</mo><msub><mi>n</mi><mrow><mi mathvariant="normal">s</mi><mo>,</mo><mi mathvariant="normal">geo</mi></mrow></msub><mo>)</mo><mo>/</mo><mi mathvariant="normal">Δ</mi><mi>T</mi><mo>)</mo></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="83pt" height="16pt" class="svg-formula" dspmath="mathimg" md5hash="8ec71e136abcca72f65a4b88c200015b"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-19-4823-2019-ie00002.svg" width="83pt" height="16pt" src="acp-19-4823-2019-ie00002.png"/></svg:svg></span></span> from our measurements to previous literature results. Results show all three cellulose materials are reasonably ice active. The freezing efficiencies of NCC samples agree reasonably well, whereas the diversity for the other two samples spans <span class="inline-formula">≈</span> 10 <span class="inline-formula"><sup>∘</sup></span>C. Despite given uncertainties within each instrument technique, the overall trend of the <span class="inline-formula"><i>n</i><sub>s,geo</sub>(<i>T</i>)</span> spectrum traced by the <span class="inline-formula"><i>T</i></span>-binned average of measurements suggests that predominantly supermicron-sized cellulose particles (MCC and FC) generally act as more efficient ice-nucleating particles (INPs) than NCC with about 1 order of magnitude higher <span class="inline-formula"><i>n</i><sub>s,geo</sub>(<i>T</i>)</span>.</p>https://www.atmos-chem-phys.net/19/4823/2019/acp-19-4823-2019.pdf |
| spellingShingle | N. Hiranuma K. Adachi D. M. Bell D. M. Bell F. Belosi H. Beydoun B. Bhaduri B. Bhaduri H. Bingemer C. Budke H.-C. Clemen F. Conen K. M. Cory J. Curtius P. J. DeMott O. Eppers S. Grawe S. Hartmann N. Hoffmann K. Höhler E. Jantsch A. Kiselev T. Koop G. Kulkarni A. Mayer M. Murakami M. Murakami B. J. Murray A. Nicosia A. Nicosia M. D. Petters M. Piazza M. Polen N. Reicher Y. Rudich A. Saito G. Santachiara T. Schiebel G. P. Schill J. Schneider L. Segev E. Stopelli E. Stopelli R. C. Sullivan K. Suski K. Suski M. Szakáll T. Tajiri H. Taylor Y. Tobo Y. Tobo R. Ullrich D. Weber H. Wex T. F. Whale C. L. Whiteside K. Yamashita K. Yamashita A. Zelenyuk O. Möhler A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water Atmospheric Chemistry and Physics |
| title | A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water |
| title_full | A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water |
| title_fullStr | A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water |
| title_full_unstemmed | A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water |
| title_short | A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water |
| title_sort | comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water |
| url | https://www.atmos-chem-phys.net/19/4823/2019/acp-19-4823-2019.pdf |
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AT jcurtius comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT pjdemott comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT oeppers comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT sgrawe comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT shartmann comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT nhoffmann comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT khohler comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT ejantsch comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT akiselev comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT tkoop comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT gkulkarni comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT amayer comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT mmurakami comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT mmurakami comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT bjmurray comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT anicosia comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT anicosia comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT mdpetters comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT mpiazza comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT mpolen comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT nreicher comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT yrudich comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT asaito comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT gsantachiara comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT tschiebel comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT gpschill comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT jschneider comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT lsegev comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT estopelli comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT estopelli comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT rcsullivan comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT ksuski comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT ksuski comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT mszakall comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT ttajiri comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT htaylor comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT ytobo comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT ytobo comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT rullrich comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT dweber comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT hwex comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT tfwhale comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT clwhiteside comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT kyamashita comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT kyamashita comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT azelenyuk comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater AT omohler comprehensivecharacterizationoficenucleationbythreedifferenttypesofcelluloseparticlesimmersedinwater |