Design of All‐Oxide Multilayers with High‐Temperature Stability Toward Future Thermophotovoltaic Applications

Abstract Thermophotovoltaic (TPV) technology converts heat into electricity using thermal radiation. Increasing operating temperature is a highly effective approach to improving the efficiency of TPV systems. However, most reported TPV selective emitters degrade rapidly via. oxidation as operating t...

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Main Authors: Jiawei Song, Zihao He, Chao Shen, Jie Zhu, Zhimin Qi, Xing Sun, Yizhi Zhang, Juncheng Liu, Xinghang Zhang, Xiulin Ruan, Peter Bermel, Haiyan Wang
Format: Article
Language:English
Published: Wiley-VCH 2024-02-01
Series:Advanced Materials Interfaces
Subjects:
Online Access:https://doi.org/10.1002/admi.202300733
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author Jiawei Song
Zihao He
Chao Shen
Jie Zhu
Zhimin Qi
Xing Sun
Yizhi Zhang
Juncheng Liu
Xinghang Zhang
Xiulin Ruan
Peter Bermel
Haiyan Wang
author_facet Jiawei Song
Zihao He
Chao Shen
Jie Zhu
Zhimin Qi
Xing Sun
Yizhi Zhang
Juncheng Liu
Xinghang Zhang
Xiulin Ruan
Peter Bermel
Haiyan Wang
author_sort Jiawei Song
collection DOAJ
description Abstract Thermophotovoltaic (TPV) technology converts heat into electricity using thermal radiation. Increasing operating temperature is a highly effective approach to improving the efficiency of TPV systems. However, most reported TPV selective emitters degrade rapidly via. oxidation as operating temperatures increase. To address this issue, replacing nanostructured oxide‐metal films with oxide–oxide films is a promising way to greatly limit oxidation, even under high‐temperature conditions. This study introduces new all‐oxide photonic crystal designs for high‐temperature stable TPV systems, overcoming limitations of metal phases and offering promising material choices. The designs utilize both yttria‐stabilized zirconia (YSZ)/MgO and CeO2/MgO combinations with a multilayer structure and stable high‐quality growth. Both designsexhibit positive optical dielectric constants with tunable reflectivity, measured via optical characterization. Thermal stability testing using in situ heating X‐ray diffraction (XRD) suggests high‐temperature stability (up to 1000 °C) of both YSZ/MgO and CeO2/MgO systems. The results demonstrate a new and promising approach to improve the high‐temperature stability of TPV systems, which can be extended to a wide range of material selection and potential designs.
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spelling doaj.art-094b3dc2ff2749c8ae708a6d52a856742024-02-16T04:36:59ZengWiley-VCHAdvanced Materials Interfaces2196-73502024-02-01115n/an/a10.1002/admi.202300733Design of All‐Oxide Multilayers with High‐Temperature Stability Toward Future Thermophotovoltaic ApplicationsJiawei Song0Zihao He1Chao Shen2Jie Zhu3Zhimin Qi4Xing Sun5Yizhi Zhang6Juncheng Liu7Xinghang Zhang8Xiulin Ruan9Peter Bermel10Haiyan Wang11School of Materials EngineeringPurdue UniversityWest Lafayette IN 47907 USABirck Nanotechnology Center and School of Electrical and Computer Engineering Purdue University West Lafayette IN 47907 USASchool of Materials EngineeringPurdue UniversityWest Lafayette IN 47907 USABirck Nanotechnology Center and School of Electrical and Computer Engineering Purdue University West Lafayette IN 47907 USASchool of Materials EngineeringPurdue UniversityWest Lafayette IN 47907 USASchool of Materials EngineeringPurdue UniversityWest Lafayette IN 47907 USASchool of Materials EngineeringPurdue UniversityWest Lafayette IN 47907 USASchool of Materials EngineeringPurdue UniversityWest Lafayette IN 47907 USASchool of Materials EngineeringPurdue UniversityWest Lafayette IN 47907 USASchool of Mechanical Engineering Purdue University West Lafayette IN 47907 USABirck Nanotechnology Center and School of Electrical and Computer Engineering Purdue University West Lafayette IN 47907 USASchool of Materials EngineeringPurdue UniversityWest Lafayette IN 47907 USAAbstract Thermophotovoltaic (TPV) technology converts heat into electricity using thermal radiation. Increasing operating temperature is a highly effective approach to improving the efficiency of TPV systems. However, most reported TPV selective emitters degrade rapidly via. oxidation as operating temperatures increase. To address this issue, replacing nanostructured oxide‐metal films with oxide–oxide films is a promising way to greatly limit oxidation, even under high‐temperature conditions. This study introduces new all‐oxide photonic crystal designs for high‐temperature stable TPV systems, overcoming limitations of metal phases and offering promising material choices. The designs utilize both yttria‐stabilized zirconia (YSZ)/MgO and CeO2/MgO combinations with a multilayer structure and stable high‐quality growth. Both designsexhibit positive optical dielectric constants with tunable reflectivity, measured via optical characterization. Thermal stability testing using in situ heating X‐ray diffraction (XRD) suggests high‐temperature stability (up to 1000 °C) of both YSZ/MgO and CeO2/MgO systems. The results demonstrate a new and promising approach to improve the high‐temperature stability of TPV systems, which can be extended to a wide range of material selection and potential designs.https://doi.org/10.1002/admi.202300733all‐oxide designmultilayerthermal stabilitythermophotovoltaic
spellingShingle Jiawei Song
Zihao He
Chao Shen
Jie Zhu
Zhimin Qi
Xing Sun
Yizhi Zhang
Juncheng Liu
Xinghang Zhang
Xiulin Ruan
Peter Bermel
Haiyan Wang
Design of All‐Oxide Multilayers with High‐Temperature Stability Toward Future Thermophotovoltaic Applications
Advanced Materials Interfaces
all‐oxide design
multilayer
thermal stability
thermophotovoltaic
title Design of All‐Oxide Multilayers with High‐Temperature Stability Toward Future Thermophotovoltaic Applications
title_full Design of All‐Oxide Multilayers with High‐Temperature Stability Toward Future Thermophotovoltaic Applications
title_fullStr Design of All‐Oxide Multilayers with High‐Temperature Stability Toward Future Thermophotovoltaic Applications
title_full_unstemmed Design of All‐Oxide Multilayers with High‐Temperature Stability Toward Future Thermophotovoltaic Applications
title_short Design of All‐Oxide Multilayers with High‐Temperature Stability Toward Future Thermophotovoltaic Applications
title_sort design of all oxide multilayers with high temperature stability toward future thermophotovoltaic applications
topic all‐oxide design
multilayer
thermal stability
thermophotovoltaic
url https://doi.org/10.1002/admi.202300733
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