Advancing the additive manufacturing of PLA-ZnO nanocomposites by fused filament fabrication

ABSTRACTPoly(lactic acid)-zinc oxide (PLA-ZnO) nanocomposites for fused filament fabrication have potential applications in the biomedical field as they combine the bio-compatibility of PLA with the antibacterial properties of ZnO. This work investigates the effects of masterbatch mixing strategy, Z...

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Main Authors: Wei Juene Chong, Dejana Pejak Simunec, Adrian Trinchi, Ilias (Louis) Kyratzis, Yuncang Li, Paul Wright, Shirley Shen, Antonella Sola, Cuie Wen
Format: Article
Language:English
Published: Taylor & Francis Group 2024-12-01
Series:Virtual and Physical Prototyping
Subjects:
Online Access:https://www.tandfonline.com/doi/10.1080/17452759.2023.2285418
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author Wei Juene Chong
Dejana Pejak Simunec
Adrian Trinchi
Ilias (Louis) Kyratzis
Yuncang Li
Paul Wright
Shirley Shen
Antonella Sola
Cuie Wen
author_facet Wei Juene Chong
Dejana Pejak Simunec
Adrian Trinchi
Ilias (Louis) Kyratzis
Yuncang Li
Paul Wright
Shirley Shen
Antonella Sola
Cuie Wen
author_sort Wei Juene Chong
collection DOAJ
description ABSTRACTPoly(lactic acid)-zinc oxide (PLA-ZnO) nanocomposites for fused filament fabrication have potential applications in the biomedical field as they combine the bio-compatibility of PLA with the antibacterial properties of ZnO. This work investigates the effects of masterbatch mixing strategy, ZnO concentration and ZnO surface treatment (silanisation) on the printability and the mechanical performance of the nanocomposites as a pre-requirement to the wider uptake of these materials. The results showed that the printability decreased as the filler loading increased. However, the surface treatment of the ZnO powder enhanced the matrix-filler interfacial interactions and reduced the thermal degradation of PLA. This ameliorated the printability and the tensile properties of the nanocomposites filled with up to 5 wt.% of ZnO. Moreover, despite the additional thermal treatment, melt-mixing prevented the degradative effect induced by the solvent used for solvent mixing. Future work will focus on assessing the antibacterial properties of the nanocomposite FFF parts.
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spelling doaj.art-09df6d0ba24d4b7e91dd89b33c1738732023-12-06T13:01:54ZengTaylor & Francis GroupVirtual and Physical Prototyping1745-27591745-27672024-12-0119110.1080/17452759.2023.2285418Advancing the additive manufacturing of PLA-ZnO nanocomposites by fused filament fabricationWei Juene Chong0Dejana Pejak Simunec1Adrian Trinchi2Ilias (Louis) Kyratzis3Yuncang Li4Paul Wright5Shirley Shen6Antonella Sola7Cuie Wen8School of Engineering, RMIT University, Melbourne, AustraliaCSIRO Manufacturing Business Unit, Clayton, AustraliaCSIRO Manufacturing Business Unit, Clayton, AustraliaCSIRO Manufacturing Business Unit, Clayton, AustraliaSchool of Engineering, RMIT University, Melbourne, AustraliaSchool of Health and Biomedical Sciences, RMIT University, Bundoora, Melbourne, AustraliaDSTG, Melbourne, AustraliaCSIRO Manufacturing Business Unit, Clayton, AustraliaSchool of Engineering, RMIT University, Melbourne, AustraliaABSTRACTPoly(lactic acid)-zinc oxide (PLA-ZnO) nanocomposites for fused filament fabrication have potential applications in the biomedical field as they combine the bio-compatibility of PLA with the antibacterial properties of ZnO. This work investigates the effects of masterbatch mixing strategy, ZnO concentration and ZnO surface treatment (silanisation) on the printability and the mechanical performance of the nanocomposites as a pre-requirement to the wider uptake of these materials. The results showed that the printability decreased as the filler loading increased. However, the surface treatment of the ZnO powder enhanced the matrix-filler interfacial interactions and reduced the thermal degradation of PLA. This ameliorated the printability and the tensile properties of the nanocomposites filled with up to 5 wt.% of ZnO. Moreover, despite the additional thermal treatment, melt-mixing prevented the degradative effect induced by the solvent used for solvent mixing. Future work will focus on assessing the antibacterial properties of the nanocomposite FFF parts.https://www.tandfonline.com/doi/10.1080/17452759.2023.2285418Additive manufacturingPLAZnOnanocompositefused filament fabricationfused deposition modelling
spellingShingle Wei Juene Chong
Dejana Pejak Simunec
Adrian Trinchi
Ilias (Louis) Kyratzis
Yuncang Li
Paul Wright
Shirley Shen
Antonella Sola
Cuie Wen
Advancing the additive manufacturing of PLA-ZnO nanocomposites by fused filament fabrication
Virtual and Physical Prototyping
Additive manufacturing
PLA
ZnO
nanocomposite
fused filament fabrication
fused deposition modelling
title Advancing the additive manufacturing of PLA-ZnO nanocomposites by fused filament fabrication
title_full Advancing the additive manufacturing of PLA-ZnO nanocomposites by fused filament fabrication
title_fullStr Advancing the additive manufacturing of PLA-ZnO nanocomposites by fused filament fabrication
title_full_unstemmed Advancing the additive manufacturing of PLA-ZnO nanocomposites by fused filament fabrication
title_short Advancing the additive manufacturing of PLA-ZnO nanocomposites by fused filament fabrication
title_sort advancing the additive manufacturing of pla zno nanocomposites by fused filament fabrication
topic Additive manufacturing
PLA
ZnO
nanocomposite
fused filament fabrication
fused deposition modelling
url https://www.tandfonline.com/doi/10.1080/17452759.2023.2285418
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