A Facile Preparation of Multicolor Carbon Dots

Abstract Carbon dots (CDs) have raised broad interest because of their great potential in the fluorescence related fields, such as photocatalysis and bioimaging. CDs exhibit different optical properties when dissolved in various solvents. However, the effects of solvents during the process of prepar...

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Main Authors: Risheng Yu, Sen Liang, Yi Ru, Lu Li, Zhikun Wang, Junlang Chen, Liang Chen
Format: Article
Language:English
Published: SpringerOpen 2022-03-01
Series:Nanoscale Research Letters
Subjects:
Online Access:https://doi.org/10.1186/s11671-022-03661-z
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author Risheng Yu
Sen Liang
Yi Ru
Lu Li
Zhikun Wang
Junlang Chen
Liang Chen
author_facet Risheng Yu
Sen Liang
Yi Ru
Lu Li
Zhikun Wang
Junlang Chen
Liang Chen
author_sort Risheng Yu
collection DOAJ
description Abstract Carbon dots (CDs) have raised broad interest because of their great potential in the fluorescence related fields, such as photocatalysis and bioimaging. CDs exhibit different optical properties when dissolved in various solvents. However, the effects of solvents during the process of preparation on the fluorescence emission of CDs are still unclear. In this work, CDs were prepared by a simple one-pot solvothermal route. Typical critic acid and thiourea were used as precursors. Through changing the volume ratio of water to N,N-dimethylformamide (DMF), we have obtained color tunable CDs, with the emission wavelength from 450 to 640 nm. TEM images, Raman and XPS spectra indicate that the particle size of CDs and the content of surface functional groups (C–N/C–S and C≡N bonds) increase with the increasing ratio of DMF to water, which results in the optimal emission wavelength red-shifted. The prepared multicolor CDs may have prospects in the lighting applications. Graphical abstract
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spelling doaj.art-09ea864bfccb4268911f34d6441268542023-09-03T05:01:59ZengSpringerOpenNanoscale Research Letters1556-276X2022-03-011711910.1186/s11671-022-03661-zA Facile Preparation of Multicolor Carbon DotsRisheng Yu0Sen Liang1Yi Ru2Lu Li3Zhikun Wang4Junlang Chen5Liang Chen6Department of Optical Engineering, Zhejiang Prov Key Lab Carbon Cycling Forest Ecosy, College of Environmental and Resource Sciences, Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F UniversityDepartment of Optical Engineering, Zhejiang Prov Key Lab Carbon Cycling Forest Ecosy, College of Environmental and Resource Sciences, Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F UniversityDepartment of Optical Engineering, Zhejiang Prov Key Lab Carbon Cycling Forest Ecosy, College of Environmental and Resource Sciences, Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F UniversityDepartment of Optical Engineering, Zhejiang Prov Key Lab Carbon Cycling Forest Ecosy, College of Environmental and Resource Sciences, Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F UniversityDepartment of Optical Engineering, Zhejiang Prov Key Lab Carbon Cycling Forest Ecosy, College of Environmental and Resource Sciences, Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F UniversityDepartment of Optical Engineering, Zhejiang Prov Key Lab Carbon Cycling Forest Ecosy, College of Environmental and Resource Sciences, Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F UniversityDepartment of Optical Engineering, Zhejiang Prov Key Lab Carbon Cycling Forest Ecosy, College of Environmental and Resource Sciences, Zhejiang Provincial Key Laboratory of Chemical Utilization of Forestry Biomass, Zhejiang A&F UniversityAbstract Carbon dots (CDs) have raised broad interest because of their great potential in the fluorescence related fields, such as photocatalysis and bioimaging. CDs exhibit different optical properties when dissolved in various solvents. However, the effects of solvents during the process of preparation on the fluorescence emission of CDs are still unclear. In this work, CDs were prepared by a simple one-pot solvothermal route. Typical critic acid and thiourea were used as precursors. Through changing the volume ratio of water to N,N-dimethylformamide (DMF), we have obtained color tunable CDs, with the emission wavelength from 450 to 640 nm. TEM images, Raman and XPS spectra indicate that the particle size of CDs and the content of surface functional groups (C–N/C–S and C≡N bonds) increase with the increasing ratio of DMF to water, which results in the optimal emission wavelength red-shifted. The prepared multicolor CDs may have prospects in the lighting applications. Graphical abstracthttps://doi.org/10.1186/s11671-022-03661-zMulticolor carbon dotsSolvothermal reactionTunable photoluminescence
spellingShingle Risheng Yu
Sen Liang
Yi Ru
Lu Li
Zhikun Wang
Junlang Chen
Liang Chen
A Facile Preparation of Multicolor Carbon Dots
Nanoscale Research Letters
Multicolor carbon dots
Solvothermal reaction
Tunable photoluminescence
title A Facile Preparation of Multicolor Carbon Dots
title_full A Facile Preparation of Multicolor Carbon Dots
title_fullStr A Facile Preparation of Multicolor Carbon Dots
title_full_unstemmed A Facile Preparation of Multicolor Carbon Dots
title_short A Facile Preparation of Multicolor Carbon Dots
title_sort facile preparation of multicolor carbon dots
topic Multicolor carbon dots
Solvothermal reaction
Tunable photoluminescence
url https://doi.org/10.1186/s11671-022-03661-z
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