Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment, North China

Intensive farming is a primary cause of increased sediment and associated nitrogen (N) and phosphorus (P) loads in surface water systems. Determining their contributing sources, pathways and loads present major challenges in the high-intensity agricultural catchments. Herein, we quantify the sedimen...

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Main Authors: Hanqing Yu, Joseph Adu-Gyamfi, Suarau Odutola Oshunsanya, Adrian Chappell, Wenxiang Liu, Yu Zheng, Tingting Xue, Lee Heng
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2023-09-01
Series:International Soil and Water Conservation Research
Online Access:http://www.sciencedirect.com/science/article/pii/S2095633922000843
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author Hanqing Yu
Joseph Adu-Gyamfi
Suarau Odutola Oshunsanya
Adrian Chappell
Wenxiang Liu
Yu Zheng
Tingting Xue
Lee Heng
author_facet Hanqing Yu
Joseph Adu-Gyamfi
Suarau Odutola Oshunsanya
Adrian Chappell
Wenxiang Liu
Yu Zheng
Tingting Xue
Lee Heng
author_sort Hanqing Yu
collection DOAJ
description Intensive farming is a primary cause of increased sediment and associated nitrogen (N) and phosphorus (P) loads in surface water systems. Determining their contributing sources, pathways and loads present major challenges in the high-intensity agricultural catchments. Herein, we quantify the sediment sources and magnitude of sediment total N and total P from different sources using a novel application of compound-specific stable isotope (CSSI) and fallout radionuclides (FRNs) of 137Cs and 210Pbex in an intensive agricultural catchment in North China. Sediment sources from surface and sub-surface soils were estimated from FRNs fingerprint and accounted for 62 ± 7% and 38 ± 7% respectively, while surface soil from land uses that originated from hillslope were identified by CSSI fingerprint. Using a novel application of FRNs and CSSI sediment fingerprinting techniques, the dominant sediment source was derived from maize farmland (44 ± 0.1%), followed by channel bank (38 ± 7%). The sedimentation rate (13.55 ± 0.30 t ha−1 yr−1) was quantified by the 137Cs cores (0–60 cm) at the outlet of this catchment. The total N and total P in sediment were both mostly derived from maize farmland and least from channel banks. The channel banks are significant sediment sources but contribute little to the input of sediment N and P for eutrophication. It implies that chemically-applied farmlands are the main hotspots for catchment erosion control and pollution prevention. The novel application of FRNs and CSSI techniques cost-effectively quantified sediment N and P loads from different sources with a single visit to the catchment, enabling rapid assessment for optimizing soil conservation strategies and land management practices. Keywords: Sediment sources, Land use, N and P loads, Compound-specific stable isotope, Fallout radionuclides.
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spelling doaj.art-0a00c3863ba244b386fea95826404a6b2024-03-03T09:15:05ZengKeAi Communications Co., Ltd.International Soil and Water Conservation Research2095-63392023-09-01113494506Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment, North ChinaHanqing Yu0Joseph Adu-Gyamfi1Suarau Odutola Oshunsanya2Adrian Chappell3Wenxiang Liu4Yu Zheng5Tingting Xue6Lee Heng7Agricultural Clean Watershed Research Group, Institute of Environment and Sustainable Development in Agriculture, Chinese Academy of Agricultural Sciences (CAAS), Haidian District, 100081, Beijing, China; Corresponding author.International Atomic Energy Agency, Vienna, AustriaAgricultural Clean Watershed Research Group, Institute of Environment and Sustainable Development in Agriculture, Chinese Academy of Agricultural Sciences (CAAS), Haidian District, 100081, Beijing, China; Department of Agronomy, University of Ibadan, NigeriaSchool of Earth and Environmental Sciences, Cardiff University, Cardiff, UKAgricultural Clean Watershed Research Group, Institute of Environment and Sustainable Development in Agriculture, Chinese Academy of Agricultural Sciences (CAAS), Haidian District, 100081, Beijing, China; Chongqing Branch Institute, Changjiang River Scientific Research Institute, Chongqing, 400026, ChinaAgricultural Clean Watershed Research Group, Institute of Environment and Sustainable Development in Agriculture, Chinese Academy of Agricultural Sciences (CAAS), Haidian District, 100081, Beijing, ChinaAgricultural Clean Watershed Research Group, Institute of Environment and Sustainable Development in Agriculture, Chinese Academy of Agricultural Sciences (CAAS), Haidian District, 100081, Beijing, ChinaInternational Atomic Energy Agency, Vienna, AustriaIntensive farming is a primary cause of increased sediment and associated nitrogen (N) and phosphorus (P) loads in surface water systems. Determining their contributing sources, pathways and loads present major challenges in the high-intensity agricultural catchments. Herein, we quantify the sediment sources and magnitude of sediment total N and total P from different sources using a novel application of compound-specific stable isotope (CSSI) and fallout radionuclides (FRNs) of 137Cs and 210Pbex in an intensive agricultural catchment in North China. Sediment sources from surface and sub-surface soils were estimated from FRNs fingerprint and accounted for 62 ± 7% and 38 ± 7% respectively, while surface soil from land uses that originated from hillslope were identified by CSSI fingerprint. Using a novel application of FRNs and CSSI sediment fingerprinting techniques, the dominant sediment source was derived from maize farmland (44 ± 0.1%), followed by channel bank (38 ± 7%). The sedimentation rate (13.55 ± 0.30 t ha−1 yr−1) was quantified by the 137Cs cores (0–60 cm) at the outlet of this catchment. The total N and total P in sediment were both mostly derived from maize farmland and least from channel banks. The channel banks are significant sediment sources but contribute little to the input of sediment N and P for eutrophication. It implies that chemically-applied farmlands are the main hotspots for catchment erosion control and pollution prevention. The novel application of FRNs and CSSI techniques cost-effectively quantified sediment N and P loads from different sources with a single visit to the catchment, enabling rapid assessment for optimizing soil conservation strategies and land management practices. Keywords: Sediment sources, Land use, N and P loads, Compound-specific stable isotope, Fallout radionuclides.http://www.sciencedirect.com/science/article/pii/S2095633922000843
spellingShingle Hanqing Yu
Joseph Adu-Gyamfi
Suarau Odutola Oshunsanya
Adrian Chappell
Wenxiang Liu
Yu Zheng
Tingting Xue
Lee Heng
Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment, North China
International Soil and Water Conservation Research
title Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment, North China
title_full Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment, North China
title_fullStr Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment, North China
title_full_unstemmed Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment, North China
title_short Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment, North China
title_sort novel sediment source fingerprinting quantifying erosion induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment north china
url http://www.sciencedirect.com/science/article/pii/S2095633922000843
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