Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductors

We compare the upper critical field of bulk single-crystalline samples of the two intrinsic transition metal dichalcogenide superconductors, 2H-NbSe _2 and 2H-NbS _2 , in high magnetic fields where their layer structure is aligned strictly parallel and perpendicular to the field, using magnetic torq...

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Main Authors: Chang-woo Cho, Cheuk Yin Ng, Chi Ho Wong, Mahmoud Abdel-Hafiez, Alexander N Vasiliev, Dmitriy A Chareev, A G Lebed, Rolf Lortz
Format: Article
Language:English
Published: IOP Publishing 2022-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/ac8114
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author Chang-woo Cho
Cheuk Yin Ng
Chi Ho Wong
Mahmoud Abdel-Hafiez
Alexander N Vasiliev
Dmitriy A Chareev
A G Lebed
Rolf Lortz
author_facet Chang-woo Cho
Cheuk Yin Ng
Chi Ho Wong
Mahmoud Abdel-Hafiez
Alexander N Vasiliev
Dmitriy A Chareev
A G Lebed
Rolf Lortz
author_sort Chang-woo Cho
collection DOAJ
description We compare the upper critical field of bulk single-crystalline samples of the two intrinsic transition metal dichalcogenide superconductors, 2H-NbSe _2 and 2H-NbS _2 , in high magnetic fields where their layer structure is aligned strictly parallel and perpendicular to the field, using magnetic torque experiments and a high-precision piezo-rotary positioner. While both superconductors show that orbital effects still have a significant impact when the layer structure is aligned parallel to the field, the upper critical field of NbS _2 rises above the Pauli limiting field and forms a Fulde–Ferrell–Larkin–Ovchinnikov (FFLO) state, while orbital effects suppress superconductivity in NbSe _2 just below the Pauli limit, which excludes the formation of the FFLO state. From the out-of-plane anisotropies, the coherence length perpendicular to the layers of 31 Å in NbSe _2 is much larger than the interlayer distance, leading to a significant orbital effect suppressing superconductivity before the Pauli limit is reached, in contrast to the more 2D NbS _2 .
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spelling doaj.art-0a55270c94634aefaf5559854a7f69b22023-08-09T14:26:01ZengIOP PublishingNew Journal of Physics1367-26302022-01-0124808300110.1088/1367-2630/ac8114Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductorsChang-woo Cho0https://orcid.org/0000-0002-5190-7070Cheuk Yin Ng1Chi Ho Wong2Mahmoud Abdel-Hafiez3https://orcid.org/0000-0002-1802-5279Alexander N Vasiliev4Dmitriy A Chareev5A G Lebed6Rolf Lortz7https://orcid.org/0000-0002-4075-9375Department of Physics, The Hong Kong University of Science and Technology , Clear Water Bay, Kowloon, Hong Kong Special Administrative Region of ChinaDepartment of Physics, The Hong Kong University of Science and Technology , Clear Water Bay, Kowloon, Hong Kong Special Administrative Region of ChinaDepartment of Industrial and Systems Engineering, The Hong Kong Polytechnic University , 11 Yuk Choi Rd, Hung Hom, Kowloon, H ong Kong Special Administrative Region of ChinaDepartment of Physics and Astronomy, Uppsala University , Uppsala SE-75120, Sweden; Lyman Laboratory of Physics, Harvard University , Cambridge, MA 02138, United States of AmericaDepartment of Low Temperature Physics and Superconductivity, Lomonosov Moscow State University , Moscow 119991, Russia; Quantum Functional Materials Laboratory, National University of Science and Technology ‘MISiS’, Moscow 119049 , Russia; Ural Federal University , Ekaterinburg 620002, RussiaQuantum Functional Materials Laboratory, National University of Science and Technology ‘MISiS’, Moscow 119049 , Russia; Ural Federal University , Ekaterinburg 620002, Russia; Institute of Experimental Mineralogy , RAS, Chernogolovka, Moscow Region 142432, RussiaDepartment of Physics, University of Arizona , 1118 E. 4th Street, Tucson, AZ 85721, United States of America; Landau Institute for Theoretical Physics , RAS, 2 Kosygina Street, Moscow 117334, RussiaDepartment of Physics, The Hong Kong University of Science and Technology , Clear Water Bay, Kowloon, Hong Kong Special Administrative Region of ChinaWe compare the upper critical field of bulk single-crystalline samples of the two intrinsic transition metal dichalcogenide superconductors, 2H-NbSe _2 and 2H-NbS _2 , in high magnetic fields where their layer structure is aligned strictly parallel and perpendicular to the field, using magnetic torque experiments and a high-precision piezo-rotary positioner. While both superconductors show that orbital effects still have a significant impact when the layer structure is aligned parallel to the field, the upper critical field of NbS _2 rises above the Pauli limiting field and forms a Fulde–Ferrell–Larkin–Ovchinnikov (FFLO) state, while orbital effects suppress superconductivity in NbSe _2 just below the Pauli limit, which excludes the formation of the FFLO state. From the out-of-plane anisotropies, the coherence length perpendicular to the layers of 31 Å in NbSe _2 is much larger than the interlayer distance, leading to a significant orbital effect suppressing superconductivity before the Pauli limit is reached, in contrast to the more 2D NbS _2 .https://doi.org/10.1088/1367-2630/ac8114superconductivityFulde–Ferrell–Larkin–Ovchinnikov statetransition metal dichalcogenideNbSe2NbS2
spellingShingle Chang-woo Cho
Cheuk Yin Ng
Chi Ho Wong
Mahmoud Abdel-Hafiez
Alexander N Vasiliev
Dmitriy A Chareev
A G Lebed
Rolf Lortz
Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductors
New Journal of Physics
superconductivity
Fulde–Ferrell–Larkin–Ovchinnikov state
transition metal dichalcogenide
NbSe2
NbS2
title Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductors
title_full Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductors
title_fullStr Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductors
title_full_unstemmed Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductors
title_short Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductors
title_sort competition between orbital effects pauli limiting and fulde ferrell larkin ovchinnikov states in 2d transition metal dichalcogenide superconductors
topic superconductivity
Fulde–Ferrell–Larkin–Ovchinnikov state
transition metal dichalcogenide
NbSe2
NbS2
url https://doi.org/10.1088/1367-2630/ac8114
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