Strong light–matter coupling in microcavities characterised by Rabi-splittings comparable to the Bragg stop-band widths

The vacuum Rabi splitting of polaritonic eigenmodes in semiconductor microcavities scales with the square root of the oscillator strength, as predicted by the coupled oscillator model and confirmed in many experiments. We show here that the square root law is no more applicable if the Rabi splitting...

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Main Authors: Junhui Cao, Simone De Liberato, Alexey V Kavokin
Format: Article
Language:English
Published: IOP Publishing 2021-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/ac3260
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author Junhui Cao
Simone De Liberato
Alexey V Kavokin
author_facet Junhui Cao
Simone De Liberato
Alexey V Kavokin
author_sort Junhui Cao
collection DOAJ
description The vacuum Rabi splitting of polaritonic eigenmodes in semiconductor microcavities scales with the square root of the oscillator strength, as predicted by the coupled oscillator model and confirmed in many experiments. We show here that the square root law is no more applicable if the Rabi splitting becomes comparable or larger than the stop-band width of the Bragg mirrors forming the cavity. Once the oscillator strength becomes large enough, the material hosting excitons hybridises with the quasi-continuum microcavity Bragg modes lying outside of the stop-band, thus forming a novel kind of polaritonic resonance. We study this physics considering both two- and three-dimensional excitonic materials embedded in the microcavity. We highlight the varied phenomenology of those polaritons and develop a theoretical understanding of their most peculiar features.
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spelling doaj.art-0a9f8ce51c5c4b11a76d89007c1ebc182023-08-08T15:40:37ZengIOP PublishingNew Journal of Physics1367-26302021-01-01231111301510.1088/1367-2630/ac3260Strong light–matter coupling in microcavities characterised by Rabi-splittings comparable to the Bragg stop-band widthsJunhui Cao0https://orcid.org/0000-0003-1101-9287Simone De Liberato1Alexey V Kavokin2Westlake University , 18 Shilongshan Road, Hangzhou 310024, Zhejiang Province, People’s Republic of China; Institute of Natural Sciences, Westlake Institute for Advanced Study , 18 Shilongshan Road, Hangzhou 310024, Zhejiang Province, People’s Republic of ChinaSchool of Physics and Astronomy, University of Southampton , Southampton, SO17 1BJ, United KingdomWestlake University , 18 Shilongshan Road, Hangzhou 310024, Zhejiang Province, People’s Republic of China; Institute of Natural Sciences, Westlake Institute for Advanced Study , 18 Shilongshan Road, Hangzhou 310024, Zhejiang Province, People’s Republic of ChinaThe vacuum Rabi splitting of polaritonic eigenmodes in semiconductor microcavities scales with the square root of the oscillator strength, as predicted by the coupled oscillator model and confirmed in many experiments. We show here that the square root law is no more applicable if the Rabi splitting becomes comparable or larger than the stop-band width of the Bragg mirrors forming the cavity. Once the oscillator strength becomes large enough, the material hosting excitons hybridises with the quasi-continuum microcavity Bragg modes lying outside of the stop-band, thus forming a novel kind of polaritonic resonance. We study this physics considering both two- and three-dimensional excitonic materials embedded in the microcavity. We highlight the varied phenomenology of those polaritons and develop a theoretical understanding of their most peculiar features.https://doi.org/10.1088/1367-2630/ac3260optical Rabi splittingorganic microcavitystrong light–matter coupling
spellingShingle Junhui Cao
Simone De Liberato
Alexey V Kavokin
Strong light–matter coupling in microcavities characterised by Rabi-splittings comparable to the Bragg stop-band widths
New Journal of Physics
optical Rabi splitting
organic microcavity
strong light–matter coupling
title Strong light–matter coupling in microcavities characterised by Rabi-splittings comparable to the Bragg stop-band widths
title_full Strong light–matter coupling in microcavities characterised by Rabi-splittings comparable to the Bragg stop-band widths
title_fullStr Strong light–matter coupling in microcavities characterised by Rabi-splittings comparable to the Bragg stop-band widths
title_full_unstemmed Strong light–matter coupling in microcavities characterised by Rabi-splittings comparable to the Bragg stop-band widths
title_short Strong light–matter coupling in microcavities characterised by Rabi-splittings comparable to the Bragg stop-band widths
title_sort strong light matter coupling in microcavities characterised by rabi splittings comparable to the bragg stop band widths
topic optical Rabi splitting
organic microcavity
strong light–matter coupling
url https://doi.org/10.1088/1367-2630/ac3260
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AT simonedeliberato stronglightmattercouplinginmicrocavitiescharacterisedbyrabisplittingscomparabletothebraggstopbandwidths
AT alexeyvkavokin stronglightmattercouplinginmicrocavitiescharacterisedbyrabisplittingscomparabletothebraggstopbandwidths