Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere

Pollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model....

Full description

Bibliographic Details
Main Authors: F. Ploeger, P. Konopka, K. Walker, M. Riese
Format: Article
Language:English
Published: Copernicus Publications 2017-06-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/17/7055/2017/acp-17-7055-2017.pdf
_version_ 1828772103963279360
author F. Ploeger
P. Konopka
K. Walker
M. Riese
author_facet F. Ploeger
P. Konopka
K. Walker
M. Riese
author_sort F. Ploeger
collection DOAJ
description Pollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model. We show how two main transport pathways from the anticyclone emerge: (i) into the tropical stratosphere (tropical pipe), and (ii) into the Northern Hemisphere (NH) extratropical lower stratosphere. Maximum anticyclone air mass fractions reach around 5 % in the tropical pipe and 15 % in the extratropical lowermost stratosphere over the course of a year. The anticyclone air mass fraction correlates well with satellite hydrogen cyanide (HCN) and carbon monoxide (CO) observations, confirming that pollution is transported deep into the tropical stratosphere from the Asian monsoon anticyclone. Cross-tropopause transport occurs in a vertical chimney, but with the pollutants transported quasi-horizontally along isentropes above the tropopause into the tropics and NH.
first_indexed 2024-12-11T14:38:24Z
format Article
id doaj.art-0adde5846df341028b7fd2c06371da15
institution Directory Open Access Journal
issn 1680-7316
1680-7324
language English
last_indexed 2024-12-11T14:38:24Z
publishDate 2017-06-01
publisher Copernicus Publications
record_format Article
series Atmospheric Chemistry and Physics
spelling doaj.art-0adde5846df341028b7fd2c06371da152022-12-22T01:02:04ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242017-06-01177055706610.5194/acp-17-7055-2017Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphereF. Ploeger0P. Konopka1K. Walker2M. Riese3Institute for Energy and Climate Research: Stratosphere (IEK–7), Forschungszentrum Jülich, Jülich, GermanyInstitute for Energy and Climate Research: Stratosphere (IEK–7), Forschungszentrum Jülich, Jülich, GermanyDepartment of Physics, University of Toronto, Toronto, Ontario, CanadaInstitute for Energy and Climate Research: Stratosphere (IEK–7), Forschungszentrum Jülich, Jülich, GermanyPollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model. We show how two main transport pathways from the anticyclone emerge: (i) into the tropical stratosphere (tropical pipe), and (ii) into the Northern Hemisphere (NH) extratropical lower stratosphere. Maximum anticyclone air mass fractions reach around 5 % in the tropical pipe and 15 % in the extratropical lowermost stratosphere over the course of a year. The anticyclone air mass fraction correlates well with satellite hydrogen cyanide (HCN) and carbon monoxide (CO) observations, confirming that pollution is transported deep into the tropical stratosphere from the Asian monsoon anticyclone. Cross-tropopause transport occurs in a vertical chimney, but with the pollutants transported quasi-horizontally along isentropes above the tropopause into the tropics and NH.http://www.atmos-chem-phys.net/17/7055/2017/acp-17-7055-2017.pdf
spellingShingle F. Ploeger
P. Konopka
K. Walker
M. Riese
Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere
Atmospheric Chemistry and Physics
title Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere
title_full Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere
title_fullStr Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere
title_full_unstemmed Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere
title_short Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere
title_sort quantifying pollution transport from the asian monsoon anticyclone into the lower stratosphere
url http://www.atmos-chem-phys.net/17/7055/2017/acp-17-7055-2017.pdf
work_keys_str_mv AT fploeger quantifyingpollutiontransportfromtheasianmonsoonanticycloneintothelowerstratosphere
AT pkonopka quantifyingpollutiontransportfromtheasianmonsoonanticycloneintothelowerstratosphere
AT kwalker quantifyingpollutiontransportfromtheasianmonsoonanticycloneintothelowerstratosphere
AT mriese quantifyingpollutiontransportfromtheasianmonsoonanticycloneintothelowerstratosphere