Groundwater Contaminant Transport: Prediction Under Uncertainty, With Application to the MADE Transport Experiment

Transport of solutes in porous media at the laboratory scale is governed by an Advection Dispersion Equation (ADE). The advection is by the fluid velocity U and dispersion by DdL = UαdL, where the longitudinal dispersivity αdL is of the order of the pore size. Numerous data revealed that the longitu...

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Main Authors: Aldo Fiori, Antonio Zarlenga, Alberto Bellin, Vladimir Cvetkovic, Gedeon Dagan
Format: Article
Language:English
Published: Frontiers Media S.A. 2019-06-01
Series:Frontiers in Environmental Science
Subjects:
Online Access:https://www.frontiersin.org/article/10.3389/fenvs.2019.00079/full
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author Aldo Fiori
Antonio Zarlenga
Alberto Bellin
Vladimir Cvetkovic
Gedeon Dagan
author_facet Aldo Fiori
Antonio Zarlenga
Alberto Bellin
Vladimir Cvetkovic
Gedeon Dagan
author_sort Aldo Fiori
collection DOAJ
description Transport of solutes in porous media at the laboratory scale is governed by an Advection Dispersion Equation (ADE). The advection is by the fluid velocity U and dispersion by DdL = UαdL, where the longitudinal dispersivity αdL is of the order of the pore size. Numerous data revealed that the longitudinal spreading of plumes at field scale is characterized by macrodispersivity αL, larger than αdL by orders of magnitude. This effect is attributed to heterogeneity of aquifers manifesting in the spatial variability of the logconductivity Y. Modeling Y as a stationary random field and for mean uniform flow (natural gradient), αL could be determined in an analytical form by a first order approximation in σY2 (variance of Y) of the flow and transport equations. Recently, models and numerical simulations for solving transport in highly heterogeneous aquifers (σY2>1), primarily in terms of the mass arrival (the breakthrough curve BTC), were advanced. In all cases ergodicity, which allows to exchange the unknown BTC with the ensemble mean, was assumed to prevail for large plumes, compared to the logconductivity integral scale. Besides, the various statistical parameters characterizing the logconductivity structure as well as the mean flow were assumed to be known deterministically. The present paper investigates the uncertainty of the non-ergodic BTC due to the finiteness of the plume size as well as due to the uncertainty of the various parameters on which the BTC depends. By the use of a simplified transport model we developed in the past (which led to accurate results for ergodic plumes), we were able to get simple results for the variance of the BTC. It depends in an analytical manner on the flow parameters as well as on the dimension of the initial plume relative to the integral scale of logconductivity covariance. The results were applied to the analysis of the uncertainty of the plume spatial distribution of the MADE transport experiment. This was achieved by using the latest, recent, analysis of the MADE aquifer conductivity data.
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spelling doaj.art-0b71fd0f14df45a189814d7e954da92d2022-12-22T01:08:36ZengFrontiers Media S.A.Frontiers in Environmental Science2296-665X2019-06-01710.3389/fenvs.2019.00079442673Groundwater Contaminant Transport: Prediction Under Uncertainty, With Application to the MADE Transport ExperimentAldo Fiori0Antonio Zarlenga1Alberto Bellin2Vladimir Cvetkovic3Gedeon Dagan4Department of Engineering, Roma Tre University, Rome, ItalyDepartment of Engineering, Roma Tre University, Rome, ItalyDepartment of Civil, Environmental and Mechanical Engineering, University of Trento, Trento, ItalyDepartment of Water Resources Engineering, Royal Institute of Technology, Stockholm, SwedenSchool of Mechanical Engineering, Tel Aviv University, Ramat Aviv, IsraelTransport of solutes in porous media at the laboratory scale is governed by an Advection Dispersion Equation (ADE). The advection is by the fluid velocity U and dispersion by DdL = UαdL, where the longitudinal dispersivity αdL is of the order of the pore size. Numerous data revealed that the longitudinal spreading of plumes at field scale is characterized by macrodispersivity αL, larger than αdL by orders of magnitude. This effect is attributed to heterogeneity of aquifers manifesting in the spatial variability of the logconductivity Y. Modeling Y as a stationary random field and for mean uniform flow (natural gradient), αL could be determined in an analytical form by a first order approximation in σY2 (variance of Y) of the flow and transport equations. Recently, models and numerical simulations for solving transport in highly heterogeneous aquifers (σY2>1), primarily in terms of the mass arrival (the breakthrough curve BTC), were advanced. In all cases ergodicity, which allows to exchange the unknown BTC with the ensemble mean, was assumed to prevail for large plumes, compared to the logconductivity integral scale. Besides, the various statistical parameters characterizing the logconductivity structure as well as the mean flow were assumed to be known deterministically. The present paper investigates the uncertainty of the non-ergodic BTC due to the finiteness of the plume size as well as due to the uncertainty of the various parameters on which the BTC depends. By the use of a simplified transport model we developed in the past (which led to accurate results for ergodic plumes), we were able to get simple results for the variance of the BTC. It depends in an analytical manner on the flow parameters as well as on the dimension of the initial plume relative to the integral scale of logconductivity covariance. The results were applied to the analysis of the uncertainty of the plume spatial distribution of the MADE transport experiment. This was achieved by using the latest, recent, analysis of the MADE aquifer conductivity data.https://www.frontiersin.org/article/10.3389/fenvs.2019.00079/fullsolute transportheterogeneous porous formationsbreakthrough curve (BTC)uncertaintyMADE experimentstochastic subsurface hydrology
spellingShingle Aldo Fiori
Antonio Zarlenga
Alberto Bellin
Vladimir Cvetkovic
Gedeon Dagan
Groundwater Contaminant Transport: Prediction Under Uncertainty, With Application to the MADE Transport Experiment
Frontiers in Environmental Science
solute transport
heterogeneous porous formations
breakthrough curve (BTC)
uncertainty
MADE experiment
stochastic subsurface hydrology
title Groundwater Contaminant Transport: Prediction Under Uncertainty, With Application to the MADE Transport Experiment
title_full Groundwater Contaminant Transport: Prediction Under Uncertainty, With Application to the MADE Transport Experiment
title_fullStr Groundwater Contaminant Transport: Prediction Under Uncertainty, With Application to the MADE Transport Experiment
title_full_unstemmed Groundwater Contaminant Transport: Prediction Under Uncertainty, With Application to the MADE Transport Experiment
title_short Groundwater Contaminant Transport: Prediction Under Uncertainty, With Application to the MADE Transport Experiment
title_sort groundwater contaminant transport prediction under uncertainty with application to the made transport experiment
topic solute transport
heterogeneous porous formations
breakthrough curve (BTC)
uncertainty
MADE experiment
stochastic subsurface hydrology
url https://www.frontiersin.org/article/10.3389/fenvs.2019.00079/full
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AT albertobellin groundwatercontaminanttransportpredictionunderuncertaintywithapplicationtothemadetransportexperiment
AT vladimircvetkovic groundwatercontaminanttransportpredictionunderuncertaintywithapplicationtothemadetransportexperiment
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