Adsorption Characteristics of Antibiotic Meropenem on Magnetic CoFe2O4@Au Nanoparticles

Adsorption characteristics of the antibiotic meropenem on a novel magnetic material synthesized by surface coating cobalt iron oxide (CFO) with gold nanoparticles (AuNPs) were systematically investigated. The AuNPs can enhance material adsorption capacity by having high affinity towards the thioethe...

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Main Authors: Thi Ngoc Mai Pham, Thi Hieu Hoang, Thu Phuong Nguyen, Quang Khanh Nguyen, Bach Pham, Quoc Anh Hoang, Tien Duc Pham, Thi Anh Huong Nguyen, Anh Tuan Le, Duc Thang Pham
Format: Article
Language:English
Published: SAGE Publications 2022-01-01
Series:Adsorption Science & Technology
Online Access:http://dx.doi.org/10.1155/2022/9759759
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author Thi Ngoc Mai Pham
Thi Hieu Hoang
Thu Phuong Nguyen
Quang Khanh Nguyen
Bach Pham
Quoc Anh Hoang
Tien Duc Pham
Thi Anh Huong Nguyen
Anh Tuan Le
Duc Thang Pham
author_facet Thi Ngoc Mai Pham
Thi Hieu Hoang
Thu Phuong Nguyen
Quang Khanh Nguyen
Bach Pham
Quoc Anh Hoang
Tien Duc Pham
Thi Anh Huong Nguyen
Anh Tuan Le
Duc Thang Pham
author_sort Thi Ngoc Mai Pham
collection DOAJ
description Adsorption characteristics of the antibiotic meropenem on a novel magnetic material synthesized by surface coating cobalt iron oxide (CFO) with gold nanoparticles (AuNPs) were systematically investigated. The AuNPs can enhance material adsorption capacity by having high affinity towards the thioether and amine groups in the meropenem structure. Au coverage on the CFO surface decreased the saturation magnetization from 55.8 emu/g to 48.8 emu/g, still allowing synthesized CFO@Au nanomaterials to be magnetically recoverable. The CFO@Au nanomaterials showed enhanced adsorption capacity of 25.5 mg/g at optimum conditions of pH 4.0 adsorption time 120 min, and adsorbent mass 0.05 g. Adsorption equilibrium was in accordance with a monolayer Langmuir isotherm, while the adsorption kinetics followed pseudo-first-order kinetics and intraparticle diffusion models. This work provides a simple method to prepare a magnetic composite material with high adsorption efficiency for meropenem and probably other thioether-containing substances.
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spelling doaj.art-0c46d5d219ee44db9de792d08075747c2024-03-02T13:35:06ZengSAGE PublicationsAdsorption Science & Technology2048-40382022-01-01202210.1155/2022/9759759Adsorption Characteristics of Antibiotic Meropenem on Magnetic CoFe2O4@Au NanoparticlesThi Ngoc Mai Pham0Thi Hieu Hoang1Thu Phuong Nguyen2Quang Khanh Nguyen3Bach Pham4Quoc Anh Hoang5Tien Duc Pham6Thi Anh Huong Nguyen7Anh Tuan Le8Duc Thang Pham9Faculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryPhenikaa University Nano InstitutePhenikaa University Nano InstituteAdsorption characteristics of the antibiotic meropenem on a novel magnetic material synthesized by surface coating cobalt iron oxide (CFO) with gold nanoparticles (AuNPs) were systematically investigated. The AuNPs can enhance material adsorption capacity by having high affinity towards the thioether and amine groups in the meropenem structure. Au coverage on the CFO surface decreased the saturation magnetization from 55.8 emu/g to 48.8 emu/g, still allowing synthesized CFO@Au nanomaterials to be magnetically recoverable. The CFO@Au nanomaterials showed enhanced adsorption capacity of 25.5 mg/g at optimum conditions of pH 4.0 adsorption time 120 min, and adsorbent mass 0.05 g. Adsorption equilibrium was in accordance with a monolayer Langmuir isotherm, while the adsorption kinetics followed pseudo-first-order kinetics and intraparticle diffusion models. This work provides a simple method to prepare a magnetic composite material with high adsorption efficiency for meropenem and probably other thioether-containing substances.http://dx.doi.org/10.1155/2022/9759759
spellingShingle Thi Ngoc Mai Pham
Thi Hieu Hoang
Thu Phuong Nguyen
Quang Khanh Nguyen
Bach Pham
Quoc Anh Hoang
Tien Duc Pham
Thi Anh Huong Nguyen
Anh Tuan Le
Duc Thang Pham
Adsorption Characteristics of Antibiotic Meropenem on Magnetic CoFe2O4@Au Nanoparticles
Adsorption Science & Technology
title Adsorption Characteristics of Antibiotic Meropenem on Magnetic CoFe2O4@Au Nanoparticles
title_full Adsorption Characteristics of Antibiotic Meropenem on Magnetic CoFe2O4@Au Nanoparticles
title_fullStr Adsorption Characteristics of Antibiotic Meropenem on Magnetic CoFe2O4@Au Nanoparticles
title_full_unstemmed Adsorption Characteristics of Antibiotic Meropenem on Magnetic CoFe2O4@Au Nanoparticles
title_short Adsorption Characteristics of Antibiotic Meropenem on Magnetic CoFe2O4@Au Nanoparticles
title_sort adsorption characteristics of antibiotic meropenem on magnetic cofe2o4 au nanoparticles
url http://dx.doi.org/10.1155/2022/9759759
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