Engineering Spin States of Isolated Copper Species in a Metal–Organic Framework Improves Urea Electrosynthesis

Engineering Spin States of Isolated Copper Species in a Metal–Organic Framework Improves Urea Electrosynthesis

Highlights The single-atom Cu species with S = 0 spin ground state in CuIII-HHTP have been fabricated. The CuIII-HHTP exhibits remarkable performance with a high urea yield of 7.780 mmol h−1 g−1 with the corresponding Faradaic efficiency of 23.09% at − 0.6 V (vs. RHE). Low spin state and empty ( $${...

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Bibliographic Details
Main Authors: Yuhang Gao, Jingnan Wang, Yijun Yang, Jian Wang, Chuang Zhang, Xi Wang, Jiannian Yao
Format: Article
Language:English
Published: SpringerOpen 2023-06-01
Series:Nano-Micro Letters
Subjects:
Electrocatalysis
Urea synthesis
Metal–organic framework
Spin catalysis
C–N coupling
Online Access:https://doi.org/10.1007/s40820-023-01127-0

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