Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols
Long-chain alcohols synthesis from syngas conversion is a promising route for the production of high-value chemicals. Here the authors show that a heterogeneous Fe5C2/Cu catalyst derived from layered double hydroxides precursor exhibits excellent performance with a space time yield of 0.101 g gcat −...
| Main Authors: | , , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2020-01-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-019-13691-4 |
| _version_ | 1828901815187406848 |
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| author | Yinwen Li Wa Gao Mi Peng Junbo Zhang Jialve Sun Yao Xu Song Hong Xi Liu Xingwu Liu Min Wei Bingsen Zhang Ding Ma |
| author_facet | Yinwen Li Wa Gao Mi Peng Junbo Zhang Jialve Sun Yao Xu Song Hong Xi Liu Xingwu Liu Min Wei Bingsen Zhang Ding Ma |
| author_sort | Yinwen Li |
| collection | DOAJ |
| description | Long-chain alcohols synthesis from syngas conversion is a promising route for the production of high-value chemicals. Here the authors show that a heterogeneous Fe5C2/Cu catalyst derived from layered double hydroxides precursor exhibits excellent performance with a space time yield of 0.101 g gcat −1 h−1 at a low pressure of 1 MPa. |
| first_indexed | 2024-12-13T16:05:26Z |
| format | Article |
| id | doaj.art-0d8e2e609cca4ed2a15ee7d91221ae3e |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-12-13T16:05:26Z |
| publishDate | 2020-01-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-0d8e2e609cca4ed2a15ee7d91221ae3e2022-12-21T23:39:03ZengNature PortfolioNature Communications2041-17232020-01-011111810.1038/s41467-019-13691-4Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcoholsYinwen Li0Wa Gao1Mi Peng2Junbo Zhang3Jialve Sun4Yao Xu5Song Hong6Xi Liu7Xingwu Liu8Min Wei9Bingsen Zhang10Ding Ma11State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical TechnologyBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityState Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical TechnologyBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityState Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical TechnologyState Key Laboratory of Coal Conversion, Institute of Coal Chemistry Chinese Academy of Sciences TaiyuanState Key Laboratory of Coal Conversion, Institute of Coal Chemistry Chinese Academy of Sciences TaiyuanState Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical TechnologyShenyang National Laboratory, Institute of Metal Research, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityLong-chain alcohols synthesis from syngas conversion is a promising route for the production of high-value chemicals. Here the authors show that a heterogeneous Fe5C2/Cu catalyst derived from layered double hydroxides precursor exhibits excellent performance with a space time yield of 0.101 g gcat −1 h−1 at a low pressure of 1 MPa.https://doi.org/10.1038/s41467-019-13691-4 |
| spellingShingle | Yinwen Li Wa Gao Mi Peng Junbo Zhang Jialve Sun Yao Xu Song Hong Xi Liu Xingwu Liu Min Wei Bingsen Zhang Ding Ma Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols Nature Communications |
| title | Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols |
| title_full | Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols |
| title_fullStr | Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols |
| title_full_unstemmed | Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols |
| title_short | Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols |
| title_sort | interfacial fe5c2 cu catalysts toward low pressure syngas conversion to long chain alcohols |
| url | https://doi.org/10.1038/s41467-019-13691-4 |
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