Reduced graphene oxide on silicon-based structure as novel broadband photodetector

Abstract Heterojunction photodetector based on reduced graphene oxide (rGO) has been realized using a spin coating technique. The electrical and optical characterization of bare GO and thermally reduced GO thin films deposited on glass substrate has been carried out. Ultraviolet–visible–infrared tra...

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Main Authors: Carmela Bonavolontà, Antonio Vettoliere, Giuseppe Falco, Carla Aramo, Ivo Rendina, Berardo Ruggiero, Paolo Silvestrini, Massimo Valentino
Format: Article
Language:English
Published: Nature Portfolio 2021-06-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-021-92518-z
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author Carmela Bonavolontà
Antonio Vettoliere
Giuseppe Falco
Carla Aramo
Ivo Rendina
Berardo Ruggiero
Paolo Silvestrini
Massimo Valentino
author_facet Carmela Bonavolontà
Antonio Vettoliere
Giuseppe Falco
Carla Aramo
Ivo Rendina
Berardo Ruggiero
Paolo Silvestrini
Massimo Valentino
author_sort Carmela Bonavolontà
collection DOAJ
description Abstract Heterojunction photodetector based on reduced graphene oxide (rGO) has been realized using a spin coating technique. The electrical and optical characterization of bare GO and thermally reduced GO thin films deposited on glass substrate has been carried out. Ultraviolet–visible–infrared transmittance measurements of the GO and rGO thin films revealed broad absorption range, while the absorbance analysis evaluates rGO band gap of about 2.8 eV. The effect of GO reduction process on the photoresponse capability is reported. The current–voltage characteristics and the responsivity of rGO/n-Si based device have been investigated using laser diode wavelengths from UV up to IR spectral range. An energy band diagram of the heterojunction has been proposed to explain the current versus voltage characteristics. The device demonstrates a photoresponse at a broad spectral range with a maximum responsivity and detectivity of 0.20 A/W and 7 × 1010 cmHz/W, respectively. Notably, the obtained results indicate that the rGO based device can be useful for broadband radiation detection compatible with silicon device technology.
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spelling doaj.art-0eabce4ab5894326b6d54cd501f4a0332022-12-21T23:09:46ZengNature PortfolioScientific Reports2045-23222021-06-0111111010.1038/s41598-021-92518-zReduced graphene oxide on silicon-based structure as novel broadband photodetectorCarmela Bonavolontà0Antonio Vettoliere1Giuseppe Falco2Carla Aramo3Ivo Rendina4Berardo Ruggiero5Paolo Silvestrini6Massimo Valentino7Istituto Scienze Applicate e Sistemi Intelligenti “E. Caianiello” ISASI-CNRIstituto Scienze Applicate e Sistemi Intelligenti “E. Caianiello” ISASI-CNRIstituto Scienze Applicate e Sistemi Intelligenti “E. Caianiello” ISASI-CNRIstituto Nazionale Fisica Nucleare INFN Sez. Napoli Complesso UniversitarioIstituto Scienze Applicate e Sistemi Intelligenti “E. Caianiello” ISASI-CNRIstituto Scienze Applicate e Sistemi Intelligenti “E. Caianiello” ISASI-CNRIstituto Scienze Applicate e Sistemi Intelligenti “E. Caianiello” ISASI-CNRIstituto Scienze Applicate e Sistemi Intelligenti “E. Caianiello” ISASI-CNRAbstract Heterojunction photodetector based on reduced graphene oxide (rGO) has been realized using a spin coating technique. The electrical and optical characterization of bare GO and thermally reduced GO thin films deposited on glass substrate has been carried out. Ultraviolet–visible–infrared transmittance measurements of the GO and rGO thin films revealed broad absorption range, while the absorbance analysis evaluates rGO band gap of about 2.8 eV. The effect of GO reduction process on the photoresponse capability is reported. The current–voltage characteristics and the responsivity of rGO/n-Si based device have been investigated using laser diode wavelengths from UV up to IR spectral range. An energy band diagram of the heterojunction has been proposed to explain the current versus voltage characteristics. The device demonstrates a photoresponse at a broad spectral range with a maximum responsivity and detectivity of 0.20 A/W and 7 × 1010 cmHz/W, respectively. Notably, the obtained results indicate that the rGO based device can be useful for broadband radiation detection compatible with silicon device technology.https://doi.org/10.1038/s41598-021-92518-z
spellingShingle Carmela Bonavolontà
Antonio Vettoliere
Giuseppe Falco
Carla Aramo
Ivo Rendina
Berardo Ruggiero
Paolo Silvestrini
Massimo Valentino
Reduced graphene oxide on silicon-based structure as novel broadband photodetector
Scientific Reports
title Reduced graphene oxide on silicon-based structure as novel broadband photodetector
title_full Reduced graphene oxide on silicon-based structure as novel broadband photodetector
title_fullStr Reduced graphene oxide on silicon-based structure as novel broadband photodetector
title_full_unstemmed Reduced graphene oxide on silicon-based structure as novel broadband photodetector
title_short Reduced graphene oxide on silicon-based structure as novel broadband photodetector
title_sort reduced graphene oxide on silicon based structure as novel broadband photodetector
url https://doi.org/10.1038/s41598-021-92518-z
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