A transition of atmospheric emissions of particles and gases from on-road heavy-duty trucks

<p>The transition, in extent and characteristics, of atmospheric emissions caused by the modernization of the heavy-duty on-road fleet was studied utilizing roadside measurements. Emissions of particle number (PN), particle mass (PM), black carbon (BC), nitrogen oxides (<span class="in...

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Main Authors: L. Zhou, Å. M. Hallquist, M. Hallquist, C. M. Salvador, S. M. Gaita, Å. Sjödin, M. Jerksjö, H. Salberg, I. Wängberg, J. Mellqvist, Q. Liu, B. P. Lee, C. K. Chan
Format: Article
Language:English
Published: Copernicus Publications 2020-02-01
Series:Atmospheric Chemistry and Physics
Online Access:https://www.atmos-chem-phys.net/20/1701/2020/acp-20-1701-2020.pdf
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author L. Zhou
Å. M. Hallquist
M. Hallquist
C. M. Salvador
S. M. Gaita
Å. Sjödin
M. Jerksjö
H. Salberg
I. Wängberg
J. Mellqvist
Q. Liu
B. P. Lee
C. K. Chan
author_facet L. Zhou
Å. M. Hallquist
M. Hallquist
C. M. Salvador
S. M. Gaita
Å. Sjödin
M. Jerksjö
H. Salberg
I. Wängberg
J. Mellqvist
Q. Liu
B. P. Lee
C. K. Chan
author_sort L. Zhou
collection DOAJ
description <p>The transition, in extent and characteristics, of atmospheric emissions caused by the modernization of the heavy-duty on-road fleet was studied utilizing roadside measurements. Emissions of particle number (PN), particle mass (PM), black carbon (BC), nitrogen oxides (<span class="inline-formula">NO<sub><i>x</i></sub></span>), carbon monoxide (CO), hydrocarbon (HC), particle size distributions, and particle volatility were measured from 556 individual heavy-duty trucks (HDTs). Substantial reductions in PM, BC, <span class="inline-formula">NO<sub><i>x</i></sub></span>, CO, and to a lesser extent PN were observed from Euro III to Euro VI HDTs by 99&thinsp;%, 98&thinsp;%, 93&thinsp;%, and 57&thinsp;% for the average emission factors of PM, BC, <span class="inline-formula">NO<sub><i>x</i></sub></span>, and CO, respectively. Despite significant total reductions in <span class="inline-formula">NO<sub><i>x</i></sub></span> emissions, the fraction of <span class="inline-formula">NO<sub>2</sub></span> in the <span class="inline-formula">NO<sub><i>x</i></sub></span> emissions increased continuously from Euro IV to Euro VI HDTs. Larger data scattering was evident for PN emissions in comparison to solid particle number (SPN) for Euro VI HDTs, indicating a highly variable fraction of volatile particle components. Particle size distributions of Euro III to enhanced environmentally friendly vehicle (EEV) HDTs were bimodal, whereas those of Euro VI HDTs were nucleation mode dominated. High emitters disproportionately contributed to a large fraction of the total emissions with the highest-emitting 10&thinsp;% of HDTs in each pollutant category being responsible for 65&thinsp;% of total PM, 70&thinsp;% of total PN, and 44&thinsp;% of total <span class="inline-formula">NO<sub><i>x</i></sub></span> emissions. Euro VI HDTs, which accounted for 53&thinsp;% of total kilometres driven by Swedish HDTs, were estimated to only contribute to 2&thinsp;%, 6&thinsp;%, 12&thinsp;%, and 47&thinsp;% of PM, BC, <span class="inline-formula">NO<sub><i>x</i></sub></span>, and PN emissions, respectively. A shift to a fleet dominated by Euro VI HDTs would promote a transition of atmospheric emissions towards low PM, BC, <span class="inline-formula">NO<sub><i>x</i></sub></span>, and CO levels. Nonetheless, reducing PN, SPN, and <span class="inline-formula">NO<sub>2</sub></span> emissions from Euro VI HDTs is still important to improve air quality in urban environments.</p>
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spelling doaj.art-0f097df229034caf801061ac59d22edd2022-12-21T18:58:24ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242020-02-01201701172210.5194/acp-20-1701-2020A transition of atmospheric emissions of particles and gases from on-road heavy-duty trucksL. Zhou0Å. M. Hallquist1M. Hallquist2C. M. Salvador3S. M. Gaita4Å. Sjödin5M. Jerksjö6H. Salberg7I. Wängberg8J. Mellqvist9Q. Liu10B. P. Lee11C. K. Chan12School of Energy and Environment, City University of Hong Kong, Hong Kong, ChinaIVL Swedish Environmental Research Institute, Gothenburg, SwedenDepartment of Chemistry and Molecular Biology, University of Gothenburg, Gothenburg, SwedenDepartment of Chemistry and Molecular Biology, University of Gothenburg, Gothenburg, SwedenDepartment of Chemistry and Molecular Biology, University of Gothenburg, Gothenburg, SwedenIVL Swedish Environmental Research Institute, Gothenburg, SwedenIVL Swedish Environmental Research Institute, Gothenburg, SwedenIVL Swedish Environmental Research Institute, Gothenburg, SwedenIVL Swedish Environmental Research Institute, Gothenburg, SwedenEarth and Space Sciences, Chalmers University of Technology, Gothenburg, SwedenSchool of Energy and Environment, City University of Hong Kong, Hong Kong, ChinaSchool of Energy and Environment, City University of Hong Kong, Hong Kong, ChinaSchool of Energy and Environment, City University of Hong Kong, Hong Kong, China<p>The transition, in extent and characteristics, of atmospheric emissions caused by the modernization of the heavy-duty on-road fleet was studied utilizing roadside measurements. Emissions of particle number (PN), particle mass (PM), black carbon (BC), nitrogen oxides (<span class="inline-formula">NO<sub><i>x</i></sub></span>), carbon monoxide (CO), hydrocarbon (HC), particle size distributions, and particle volatility were measured from 556 individual heavy-duty trucks (HDTs). Substantial reductions in PM, BC, <span class="inline-formula">NO<sub><i>x</i></sub></span>, CO, and to a lesser extent PN were observed from Euro III to Euro VI HDTs by 99&thinsp;%, 98&thinsp;%, 93&thinsp;%, and 57&thinsp;% for the average emission factors of PM, BC, <span class="inline-formula">NO<sub><i>x</i></sub></span>, and CO, respectively. Despite significant total reductions in <span class="inline-formula">NO<sub><i>x</i></sub></span> emissions, the fraction of <span class="inline-formula">NO<sub>2</sub></span> in the <span class="inline-formula">NO<sub><i>x</i></sub></span> emissions increased continuously from Euro IV to Euro VI HDTs. Larger data scattering was evident for PN emissions in comparison to solid particle number (SPN) for Euro VI HDTs, indicating a highly variable fraction of volatile particle components. Particle size distributions of Euro III to enhanced environmentally friendly vehicle (EEV) HDTs were bimodal, whereas those of Euro VI HDTs were nucleation mode dominated. High emitters disproportionately contributed to a large fraction of the total emissions with the highest-emitting 10&thinsp;% of HDTs in each pollutant category being responsible for 65&thinsp;% of total PM, 70&thinsp;% of total PN, and 44&thinsp;% of total <span class="inline-formula">NO<sub><i>x</i></sub></span> emissions. Euro VI HDTs, which accounted for 53&thinsp;% of total kilometres driven by Swedish HDTs, were estimated to only contribute to 2&thinsp;%, 6&thinsp;%, 12&thinsp;%, and 47&thinsp;% of PM, BC, <span class="inline-formula">NO<sub><i>x</i></sub></span>, and PN emissions, respectively. A shift to a fleet dominated by Euro VI HDTs would promote a transition of atmospheric emissions towards low PM, BC, <span class="inline-formula">NO<sub><i>x</i></sub></span>, and CO levels. Nonetheless, reducing PN, SPN, and <span class="inline-formula">NO<sub>2</sub></span> emissions from Euro VI HDTs is still important to improve air quality in urban environments.</p>https://www.atmos-chem-phys.net/20/1701/2020/acp-20-1701-2020.pdf
spellingShingle L. Zhou
Å. M. Hallquist
M. Hallquist
C. M. Salvador
S. M. Gaita
Å. Sjödin
M. Jerksjö
H. Salberg
I. Wängberg
J. Mellqvist
Q. Liu
B. P. Lee
C. K. Chan
A transition of atmospheric emissions of particles and gases from on-road heavy-duty trucks
Atmospheric Chemistry and Physics
title A transition of atmospheric emissions of particles and gases from on-road heavy-duty trucks
title_full A transition of atmospheric emissions of particles and gases from on-road heavy-duty trucks
title_fullStr A transition of atmospheric emissions of particles and gases from on-road heavy-duty trucks
title_full_unstemmed A transition of atmospheric emissions of particles and gases from on-road heavy-duty trucks
title_short A transition of atmospheric emissions of particles and gases from on-road heavy-duty trucks
title_sort transition of atmospheric emissions of particles and gases from on road heavy duty trucks
url https://www.atmos-chem-phys.net/20/1701/2020/acp-20-1701-2020.pdf
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