Simultaneous capturing phonon and electron dynamics in MXenes

How electron energy damp to lattice vibrations (phonons) in MXenes has not yet been unraveled. Here, the authors demonstrate an energy damping channel in which the Ti3C2Tx plasmonic electron energy transfers to coherent phonons by nonthermal electron mediation after Landau damping, without involving...

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Main Authors: Qi Zhang, Jiebo Li, Jiao Wen, Wei Li, Xin Chen, Yifan Zhang, Jingyong Sun, Xin Yan, Mingjun Hu, Guorong Wu, Kaijun Yuan, Hongbo Guo, Xueming Yang
Format: Article
Language:English
Published: Nature Portfolio 2022-12-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-35605-7
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author Qi Zhang
Jiebo Li
Jiao Wen
Wei Li
Xin Chen
Yifan Zhang
Jingyong Sun
Xin Yan
Mingjun Hu
Guorong Wu
Kaijun Yuan
Hongbo Guo
Xueming Yang
author_facet Qi Zhang
Jiebo Li
Jiao Wen
Wei Li
Xin Chen
Yifan Zhang
Jingyong Sun
Xin Yan
Mingjun Hu
Guorong Wu
Kaijun Yuan
Hongbo Guo
Xueming Yang
author_sort Qi Zhang
collection DOAJ
description How electron energy damp to lattice vibrations (phonons) in MXenes has not yet been unraveled. Here, the authors demonstrate an energy damping channel in which the Ti3C2Tx plasmonic electron energy transfers to coherent phonons by nonthermal electron mediation after Landau damping, without involving electron-electron scattering.
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spelling doaj.art-0f0f7f0fb329477ebb2690890970e0452022-12-25T12:21:26ZengNature PortfolioNature Communications2041-17232022-12-0113111010.1038/s41467-022-35605-7Simultaneous capturing phonon and electron dynamics in MXenesQi Zhang0Jiebo Li1Jiao Wen2Wei Li3Xin Chen4Yifan Zhang5Jingyong Sun6Xin Yan7Mingjun Hu8Guorong Wu9Kaijun Yuan10Hongbo Guo11Xueming Yang12State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of SciencesInstitute of Medical Photonics, Beijing Advanced Innovation Center for Biomedical Engineering, School of Biological Science and Medical Engineering, Beihang UniversitySchool of Materials Science and Engineering, Beihang UniversityGuSu Laboratory of MaterialsGuSu Laboratory of MaterialsInstitute of Medical Photonics, Beijing Advanced Innovation Center for Biomedical Engineering, School of Biological Science and Medical Engineering, Beihang UniversitySchool of Materials Science and Engineering, Beihang UniversitySchool of Mechanical Engineering and Automation, Beihang UniversitySchool of Materials Science and Engineering, Beihang UniversityState Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of SciencesState Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of SciencesSchool of Materials Science and Engineering, Beihang UniversityState Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of SciencesHow electron energy damp to lattice vibrations (phonons) in MXenes has not yet been unraveled. Here, the authors demonstrate an energy damping channel in which the Ti3C2Tx plasmonic electron energy transfers to coherent phonons by nonthermal electron mediation after Landau damping, without involving electron-electron scattering.https://doi.org/10.1038/s41467-022-35605-7
spellingShingle Qi Zhang
Jiebo Li
Jiao Wen
Wei Li
Xin Chen
Yifan Zhang
Jingyong Sun
Xin Yan
Mingjun Hu
Guorong Wu
Kaijun Yuan
Hongbo Guo
Xueming Yang
Simultaneous capturing phonon and electron dynamics in MXenes
Nature Communications
title Simultaneous capturing phonon and electron dynamics in MXenes
title_full Simultaneous capturing phonon and electron dynamics in MXenes
title_fullStr Simultaneous capturing phonon and electron dynamics in MXenes
title_full_unstemmed Simultaneous capturing phonon and electron dynamics in MXenes
title_short Simultaneous capturing phonon and electron dynamics in MXenes
title_sort simultaneous capturing phonon and electron dynamics in mxenes
url https://doi.org/10.1038/s41467-022-35605-7
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