A concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometers

An automated function control unit was developed to regularly check the ambient particle number concentration derived from a mobility particle size spectrometer as well as its zero-point behaviour. The function control allows unattended quality assurance experiments at remote air quality monitoring...

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Main Authors: A. Schladitz, M. Merkel, S. Bastian, W. Birmili, K. Weinhold, G. Löschau, A. Wiedensohler
Format: Article
Language:English
Published: Copernicus Publications 2014-04-01
Series:Atmospheric Measurement Techniques
Online Access:http://www.atmos-meas-tech.net/7/1065/2014/amt-7-1065-2014.pdf
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author A. Schladitz
M. Merkel
S. Bastian
W. Birmili
K. Weinhold
G. Löschau
A. Wiedensohler
author_facet A. Schladitz
M. Merkel
S. Bastian
W. Birmili
K. Weinhold
G. Löschau
A. Wiedensohler
author_sort A. Schladitz
collection DOAJ
description An automated function control unit was developed to regularly check the ambient particle number concentration derived from a mobility particle size spectrometer as well as its zero-point behaviour. The function control allows unattended quality assurance experiments at remote air quality monitoring or research stations under field conditions. The automated function control also has the advantage of being able to get a faster system stability response than the recommended on-site comparisons with reference instruments. The method is based on a comparison of the total particle number concentration measured by a mobility particle size spectrometer and a condensation particle counter while removing diffusive particles smaller than 20 nm in diameter. In practice, the small particles are removed by a set of diffusion screens, as traditionally used in a diffusion battery. Another feature of the automated function control is to check the zero-point behaviour of the ambient aerosol passing through a high-efficiency particulate air (HEPA) filter. <br><br> The performance of the function control is illustrated with the aid of a 1-year data set recorded at Annaberg-Buchholz, a station in the Saxon air quality monitoring network. During the period of concern, the total particle number concentration derived from the mobility particle size spectrometer slightly overestimated the particle number concentration recorded by the condensation particle counter by 2 % (grand average). Based on our first year of experience with the function control, we developed tolerance criteria that allow a performance evaluation of a tested mobility particle size spectrometer with respect to the total particle number concentration. We conclude that the automated function control enhances the quality and reliability of unattended long-term particle number size distribution measurements. This will have beneficial effects for intercomparison studies involving different measurement sites, and help provide a higher data accuracy for cohort health and climate research studies.
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spelling doaj.art-10372871ef764d73977333dc21a0242f2022-12-22T02:18:23ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482014-04-01741065107310.5194/amt-7-1065-2014A concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometersA. Schladitz0M. Merkel1S. Bastian2W. Birmili3K. Weinhold4G. Löschau5A. Wiedensohler6Saxon State Office for Environment, Agriculture and Geology (LfULG), Pillnitzer Platz 3, 01326 Dresden, GermanyLeibniz Institute for Tropospheric Research (TROPOS), Permoserstraße 15, 04318 Leipzig, GermanySaxon State Office for Environment, Agriculture and Geology (LfULG), Pillnitzer Platz 3, 01326 Dresden, GermanyLeibniz Institute for Tropospheric Research (TROPOS), Permoserstraße 15, 04318 Leipzig, GermanyLeibniz Institute for Tropospheric Research (TROPOS), Permoserstraße 15, 04318 Leipzig, GermanySaxon State Office for Environment, Agriculture and Geology (LfULG), Pillnitzer Platz 3, 01326 Dresden, GermanyLeibniz Institute for Tropospheric Research (TROPOS), Permoserstraße 15, 04318 Leipzig, GermanyAn automated function control unit was developed to regularly check the ambient particle number concentration derived from a mobility particle size spectrometer as well as its zero-point behaviour. The function control allows unattended quality assurance experiments at remote air quality monitoring or research stations under field conditions. The automated function control also has the advantage of being able to get a faster system stability response than the recommended on-site comparisons with reference instruments. The method is based on a comparison of the total particle number concentration measured by a mobility particle size spectrometer and a condensation particle counter while removing diffusive particles smaller than 20 nm in diameter. In practice, the small particles are removed by a set of diffusion screens, as traditionally used in a diffusion battery. Another feature of the automated function control is to check the zero-point behaviour of the ambient aerosol passing through a high-efficiency particulate air (HEPA) filter. <br><br> The performance of the function control is illustrated with the aid of a 1-year data set recorded at Annaberg-Buchholz, a station in the Saxon air quality monitoring network. During the period of concern, the total particle number concentration derived from the mobility particle size spectrometer slightly overestimated the particle number concentration recorded by the condensation particle counter by 2 % (grand average). Based on our first year of experience with the function control, we developed tolerance criteria that allow a performance evaluation of a tested mobility particle size spectrometer with respect to the total particle number concentration. We conclude that the automated function control enhances the quality and reliability of unattended long-term particle number size distribution measurements. This will have beneficial effects for intercomparison studies involving different measurement sites, and help provide a higher data accuracy for cohort health and climate research studies.http://www.atmos-meas-tech.net/7/1065/2014/amt-7-1065-2014.pdf
spellingShingle A. Schladitz
M. Merkel
S. Bastian
W. Birmili
K. Weinhold
G. Löschau
A. Wiedensohler
A concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometers
Atmospheric Measurement Techniques
title A concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometers
title_full A concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometers
title_fullStr A concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometers
title_full_unstemmed A concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometers
title_short A concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometers
title_sort concept of an automated function control for ambient aerosol measurements using mobility particle size spectrometers
url http://www.atmos-meas-tech.net/7/1065/2014/amt-7-1065-2014.pdf
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