Ultra‐Thin and Conformable Electrodes Composed of Single‐Walled Carbon Nanotube Networks for Skin‐Contact Dielectric Elastomer Actuators

Abstract Skin‐contact dielectric elastomer actuators (DEAs) consisting of skin‐conformable, stretchable electrodes are fabricated using a roll‐to‐roll‐based gravure coating method. In this method, single‐walled carbon nanotubes (SWCNTs) are continuously applied on a free‐standing ultra‐thin film (na...

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Main Authors: Tatsuhiro Horii, Kei Okada, Toshinori Fujie
Format: Article
Language:English
Published: Wiley-VCH 2023-09-01
Series:Advanced Electronic Materials
Subjects:
Online Access:https://doi.org/10.1002/aelm.202200165
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author Tatsuhiro Horii
Kei Okada
Toshinori Fujie
author_facet Tatsuhiro Horii
Kei Okada
Toshinori Fujie
author_sort Tatsuhiro Horii
collection DOAJ
description Abstract Skin‐contact dielectric elastomer actuators (DEAs) consisting of skin‐conformable, stretchable electrodes are fabricated using a roll‐to‐roll‐based gravure coating method. In this method, single‐walled carbon nanotubes (SWCNTs) are continuously applied on a free‐standing ultra‐thin film (nanosheet) of poly(styrene‐b‐butadiene‐b‐styrene) (SBS) to produce an SWCNT‐SBS nanosheet of 101‐nm thickness. After the first SWCNT coating, the SWCNT‐SBS nanosheet shows a Young's modulus (i.e., 80.9 MPa) comparable to that of the SBS film and a sheet resistance of 4.6 kΩ sq−1. Using the free‐standing SWCNT‐SBS nanosheets as electrodes, a ten‐layered DEA is fabricated without glue or dielectric elastomer precursors on three substrates with different stiffness, namely glass, Ecoflex 00–30, and a urethane elastomer model skin. The low flexural rigidity of the ten‐layered DEA (105 nN m) ensures conformability to the shape of an index finger. Application of an actuation voltage of 2100 V produces a two‐fold larger displacement of the DEA on the Ecoflex 00–30 substrate compared with that on the glass substrate. The ability of the DEA to conform to the surface of skin will enable its application in skin‐contact haptic devices.
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spelling doaj.art-10aad07d0da84e50a7bf9acb3cd467112023-09-12T05:36:18ZengWiley-VCHAdvanced Electronic Materials2199-160X2023-09-0199n/an/a10.1002/aelm.202200165Ultra‐Thin and Conformable Electrodes Composed of Single‐Walled Carbon Nanotube Networks for Skin‐Contact Dielectric Elastomer ActuatorsTatsuhiro Horii0Kei Okada1Toshinori Fujie2School of Life Science and Technology Tokyo Institute of Technology B‐50, 4259 Nagatsuta‐cho Midori‐ku Yokohama 226‐8501 JapanSchool of Life Science and Technology Tokyo Institute of Technology B‐50, 4259 Nagatsuta‐cho Midori‐ku Yokohama 226‐8501 JapanSchool of Life Science and Technology Tokyo Institute of Technology B‐50, 4259 Nagatsuta‐cho Midori‐ku Yokohama 226‐8501 JapanAbstract Skin‐contact dielectric elastomer actuators (DEAs) consisting of skin‐conformable, stretchable electrodes are fabricated using a roll‐to‐roll‐based gravure coating method. In this method, single‐walled carbon nanotubes (SWCNTs) are continuously applied on a free‐standing ultra‐thin film (nanosheet) of poly(styrene‐b‐butadiene‐b‐styrene) (SBS) to produce an SWCNT‐SBS nanosheet of 101‐nm thickness. After the first SWCNT coating, the SWCNT‐SBS nanosheet shows a Young's modulus (i.e., 80.9 MPa) comparable to that of the SBS film and a sheet resistance of 4.6 kΩ sq−1. Using the free‐standing SWCNT‐SBS nanosheets as electrodes, a ten‐layered DEA is fabricated without glue or dielectric elastomer precursors on three substrates with different stiffness, namely glass, Ecoflex 00–30, and a urethane elastomer model skin. The low flexural rigidity of the ten‐layered DEA (105 nN m) ensures conformability to the shape of an index finger. Application of an actuation voltage of 2100 V produces a two‐fold larger displacement of the DEA on the Ecoflex 00–30 substrate compared with that on the glass substrate. The ability of the DEA to conform to the surface of skin will enable its application in skin‐contact haptic devices.https://doi.org/10.1002/aelm.202200165carbon nanotubesdielectric elastomer actuatorsgravure coatingspolymer nanosheetsYoung's modulus
spellingShingle Tatsuhiro Horii
Kei Okada
Toshinori Fujie
Ultra‐Thin and Conformable Electrodes Composed of Single‐Walled Carbon Nanotube Networks for Skin‐Contact Dielectric Elastomer Actuators
Advanced Electronic Materials
carbon nanotubes
dielectric elastomer actuators
gravure coatings
polymer nanosheets
Young's modulus
title Ultra‐Thin and Conformable Electrodes Composed of Single‐Walled Carbon Nanotube Networks for Skin‐Contact Dielectric Elastomer Actuators
title_full Ultra‐Thin and Conformable Electrodes Composed of Single‐Walled Carbon Nanotube Networks for Skin‐Contact Dielectric Elastomer Actuators
title_fullStr Ultra‐Thin and Conformable Electrodes Composed of Single‐Walled Carbon Nanotube Networks for Skin‐Contact Dielectric Elastomer Actuators
title_full_unstemmed Ultra‐Thin and Conformable Electrodes Composed of Single‐Walled Carbon Nanotube Networks for Skin‐Contact Dielectric Elastomer Actuators
title_short Ultra‐Thin and Conformable Electrodes Composed of Single‐Walled Carbon Nanotube Networks for Skin‐Contact Dielectric Elastomer Actuators
title_sort ultra thin and conformable electrodes composed of single walled carbon nanotube networks for skin contact dielectric elastomer actuators
topic carbon nanotubes
dielectric elastomer actuators
gravure coatings
polymer nanosheets
Young's modulus
url https://doi.org/10.1002/aelm.202200165
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