Efficient Dye Removal from Real Textile Wastewater Using Orange Seed Powder as Suitable Bio-Adsorbent and Membrane Technology

Textile wastewater is widely produced and its discharge without treatment contributes to environmental pollution. The adsorption process is a suitable and eco-friendly process due to its low initial cost, no formation of degradation products, operation simplicity, insensitivity to toxic compounds, a...

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Main Authors: Miguel A. D. Flores Alarcón, Claudia Revilla Pacheco, Kiara Garcia Bustos, Kevin Tejada Meza, Felix Terán-Hilares, David. A. Pacheco Tanaka, Gilberto J. Colina Andrade, Ruly Terán-Hilares
Format: Article
Language:English
Published: MDPI AG 2022-12-01
Series:Water
Subjects:
Online Access:https://www.mdpi.com/2073-4441/14/24/4104
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author Miguel A. D. Flores Alarcón
Claudia Revilla Pacheco
Kiara Garcia Bustos
Kevin Tejada Meza
Felix Terán-Hilares
David. A. Pacheco Tanaka
Gilberto J. Colina Andrade
Ruly Terán-Hilares
author_facet Miguel A. D. Flores Alarcón
Claudia Revilla Pacheco
Kiara Garcia Bustos
Kevin Tejada Meza
Felix Terán-Hilares
David. A. Pacheco Tanaka
Gilberto J. Colina Andrade
Ruly Terán-Hilares
author_sort Miguel A. D. Flores Alarcón
collection DOAJ
description Textile wastewater is widely produced and its discharge without treatment contributes to environmental pollution. The adsorption process is a suitable and eco-friendly process due to its low initial cost, no formation of degradation products, operation simplicity, insensitivity to toxic compounds, and the possibility of removal from greatly diluted solutions. Orange seed (OS) powder, from which lipids were removed by hexane extraction, was evaluated as a bio-adsorbent to remove dyes from real textile wastewater. In the screening step, pH was a more significant variable (<i>p</i>-value < 0.05) than bio-adsorbent dosage, temperature, stirring speed, and process time. Moreover, under optimized conditions (pH = 2.6, 0.58 g/L from OS powder and 26 °C), more than 95% of the dye was removed from real textile wastewater. Additionally, the dye removal percentage was reduced by only 4% when the volume of textile wastewater was increased from 0.05 L to 10 L. Then, 96% turbidity was removed using a 3 µm tubular ceramic membrane at a pH of 11. Furthermore, the permeate flux through the membrane was kept constant for longer than was observed at low pH (<11). Therefore, the proposed process is an interesting option, due to the fact that orange seeds are currently not valorized and, combined with the membrane process, this could prove a suitable option for the treatment of real textile wastewater.
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spelling doaj.art-115e5ad6f7d74f118766c023046f18b72023-11-24T18:43:02ZengMDPI AGWater2073-44412022-12-011424410410.3390/w14244104Efficient Dye Removal from Real Textile Wastewater Using Orange Seed Powder as Suitable Bio-Adsorbent and Membrane TechnologyMiguel A. D. Flores Alarcón0Claudia Revilla Pacheco1Kiara Garcia Bustos2Kevin Tejada Meza3Felix Terán-Hilares4David. A. Pacheco Tanaka5Gilberto J. Colina Andrade6Ruly Terán-Hilares7Laboratorio de Bioprocesos, Facultad de Ciencias Farmacéuticas, Bioquímicas y Biotecnológicas, Universidad Católica de Santa María—UCSM, Urb. San José s/n—Umacollo, Arequipa 04000, PeruLaboratorio de Bioprocesos, Facultad de Ciencias Farmacéuticas, Bioquímicas y Biotecnológicas, Universidad Católica de Santa María—UCSM, Urb. San José s/n—Umacollo, Arequipa 04000, PeruLaboratorio de Bioprocesos, Facultad de Ciencias Farmacéuticas, Bioquímicas y Biotecnológicas, Universidad Católica de Santa María—UCSM, Urb. San José s/n—Umacollo, Arequipa 04000, PeruLaboratorio de Bioprocesos, Facultad de Ciencias Farmacéuticas, Bioquímicas y Biotecnológicas, Universidad Católica de Santa María—UCSM, Urb. San José s/n—Umacollo, Arequipa 04000, PeruLaboratorio de Investigación Agroindustrial, Universidad Nacional José María Arguedas, Av. 28 de Julio N° 1103, Talavera—Santa Rosa, Andahuaylas 03701, PeruLaboratorio de Bioprocesos, Facultad de Ciencias Farmacéuticas, Bioquímicas y Biotecnológicas, Universidad Católica de Santa María—UCSM, Urb. San José s/n—Umacollo, Arequipa 04000, PeruLaboratorio de Bioprocesos, Facultad de Ciencias Farmacéuticas, Bioquímicas y Biotecnológicas, Universidad Católica de Santa María—UCSM, Urb. San José s/n—Umacollo, Arequipa 04000, PeruLaboratorio de Bioprocesos, Facultad de Ciencias Farmacéuticas, Bioquímicas y Biotecnológicas, Universidad Católica de Santa María—UCSM, Urb. San José s/n—Umacollo, Arequipa 04000, PeruTextile wastewater is widely produced and its discharge without treatment contributes to environmental pollution. The adsorption process is a suitable and eco-friendly process due to its low initial cost, no formation of degradation products, operation simplicity, insensitivity to toxic compounds, and the possibility of removal from greatly diluted solutions. Orange seed (OS) powder, from which lipids were removed by hexane extraction, was evaluated as a bio-adsorbent to remove dyes from real textile wastewater. In the screening step, pH was a more significant variable (<i>p</i>-value < 0.05) than bio-adsorbent dosage, temperature, stirring speed, and process time. Moreover, under optimized conditions (pH = 2.6, 0.58 g/L from OS powder and 26 °C), more than 95% of the dye was removed from real textile wastewater. Additionally, the dye removal percentage was reduced by only 4% when the volume of textile wastewater was increased from 0.05 L to 10 L. Then, 96% turbidity was removed using a 3 µm tubular ceramic membrane at a pH of 11. Furthermore, the permeate flux through the membrane was kept constant for longer than was observed at low pH (<11). Therefore, the proposed process is an interesting option, due to the fact that orange seeds are currently not valorized and, combined with the membrane process, this could prove a suitable option for the treatment of real textile wastewater.https://www.mdpi.com/2073-4441/14/24/4104bio-adsorbentmembranesorange seedstextile wastewaterenvironmental pollution
spellingShingle Miguel A. D. Flores Alarcón
Claudia Revilla Pacheco
Kiara Garcia Bustos
Kevin Tejada Meza
Felix Terán-Hilares
David. A. Pacheco Tanaka
Gilberto J. Colina Andrade
Ruly Terán-Hilares
Efficient Dye Removal from Real Textile Wastewater Using Orange Seed Powder as Suitable Bio-Adsorbent and Membrane Technology
Water
bio-adsorbent
membranes
orange seeds
textile wastewater
environmental pollution
title Efficient Dye Removal from Real Textile Wastewater Using Orange Seed Powder as Suitable Bio-Adsorbent and Membrane Technology
title_full Efficient Dye Removal from Real Textile Wastewater Using Orange Seed Powder as Suitable Bio-Adsorbent and Membrane Technology
title_fullStr Efficient Dye Removal from Real Textile Wastewater Using Orange Seed Powder as Suitable Bio-Adsorbent and Membrane Technology
title_full_unstemmed Efficient Dye Removal from Real Textile Wastewater Using Orange Seed Powder as Suitable Bio-Adsorbent and Membrane Technology
title_short Efficient Dye Removal from Real Textile Wastewater Using Orange Seed Powder as Suitable Bio-Adsorbent and Membrane Technology
title_sort efficient dye removal from real textile wastewater using orange seed powder as suitable bio adsorbent and membrane technology
topic bio-adsorbent
membranes
orange seeds
textile wastewater
environmental pollution
url https://www.mdpi.com/2073-4441/14/24/4104
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