Natural oxidase-mimicking copper-organic frameworks for targeted identification of ascorbate in sensitive sweat sensing
Sweat sensors are important in personalized healthcare using natural oxidase to target biomolecules but these reactions are susceptible to external interference. Here, the authors report tryptophan- and histidine-treated copper metal-organic frameworks which show highly selective activity for ascorb...
| Main Authors: | , , , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2023-01-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-022-35721-4 |
| _version_ | 1797958536674672640 |
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| author | Zhengyun Wang Yuchen Huang Kunqi Xu Yanyu Zhong Chaohui He Lipei Jiang Jiankang Sun Zhuang Rao Jiannan Zhu Jing Huang Fei Xiao Hongfang Liu Bao Yu Xia |
| author_facet | Zhengyun Wang Yuchen Huang Kunqi Xu Yanyu Zhong Chaohui He Lipei Jiang Jiankang Sun Zhuang Rao Jiannan Zhu Jing Huang Fei Xiao Hongfang Liu Bao Yu Xia |
| author_sort | Zhengyun Wang |
| collection | DOAJ |
| description | Sweat sensors are important in personalized healthcare using natural oxidase to target biomolecules but these reactions are susceptible to external interference. Here, the authors report tryptophan- and histidine-treated copper metal-organic frameworks which show highly selective activity for ascorbate oxidation and can serve as an efficient ascorbate oxidase-mimicking material in sensitive sweat sensors. |
| first_indexed | 2024-04-11T00:21:30Z |
| format | Article |
| id | doaj.art-12c2b9abec1a479d8f283e6f02b9ac28 |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-04-11T00:21:30Z |
| publishDate | 2023-01-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-12c2b9abec1a479d8f283e6f02b9ac282023-01-08T12:16:25ZengNature PortfolioNature Communications2041-17232023-01-011411910.1038/s41467-022-35721-4Natural oxidase-mimicking copper-organic frameworks for targeted identification of ascorbate in sensitive sweat sensingZhengyun Wang0Yuchen Huang1Kunqi Xu2Yanyu Zhong3Chaohui He4Lipei Jiang5Jiankang Sun6Zhuang Rao7Jiannan Zhu8Jing Huang9Fei Xiao10Hongfang Liu11Bao Yu Xia12Hubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologySecretariat license de chimie, bâtiment 460, Université Paris-saclayKey Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of SciencesHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologyHubei Key Laboratory of Material Chemistry and Service Failure, Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education), Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, School of Chemistry and Chemical Engineering, Huazhong University of Science and TechnologySweat sensors are important in personalized healthcare using natural oxidase to target biomolecules but these reactions are susceptible to external interference. Here, the authors report tryptophan- and histidine-treated copper metal-organic frameworks which show highly selective activity for ascorbate oxidation and can serve as an efficient ascorbate oxidase-mimicking material in sensitive sweat sensors.https://doi.org/10.1038/s41467-022-35721-4 |
| spellingShingle | Zhengyun Wang Yuchen Huang Kunqi Xu Yanyu Zhong Chaohui He Lipei Jiang Jiankang Sun Zhuang Rao Jiannan Zhu Jing Huang Fei Xiao Hongfang Liu Bao Yu Xia Natural oxidase-mimicking copper-organic frameworks for targeted identification of ascorbate in sensitive sweat sensing Nature Communications |
| title | Natural oxidase-mimicking copper-organic frameworks for targeted identification of ascorbate in sensitive sweat sensing |
| title_full | Natural oxidase-mimicking copper-organic frameworks for targeted identification of ascorbate in sensitive sweat sensing |
| title_fullStr | Natural oxidase-mimicking copper-organic frameworks for targeted identification of ascorbate in sensitive sweat sensing |
| title_full_unstemmed | Natural oxidase-mimicking copper-organic frameworks for targeted identification of ascorbate in sensitive sweat sensing |
| title_short | Natural oxidase-mimicking copper-organic frameworks for targeted identification of ascorbate in sensitive sweat sensing |
| title_sort | natural oxidase mimicking copper organic frameworks for targeted identification of ascorbate in sensitive sweat sensing |
| url | https://doi.org/10.1038/s41467-022-35721-4 |
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