Synthesis of ZnO with Enhanced Photocatalytic Activity: A Novel Approach Using Nanocellulose
Well-crystallized and hexagonal wurtzite ZnO was synthesized with nanocellulose using a facile hydrothermal method. Many highly active (001) facets were retained in the obtained ZnO nanocrystals, presumably due to interaction between the polar facet of ZnO and the nanocellulose. Given its effective...
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Format: | Article |
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North Carolina State University
2016-06-01
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Series: | BioResources |
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Online Access: | http://ojs.cnr.ncsu.edu/index.php/BioRes/article/view/BioRes_11_3_6244_Wei_Synthesis_Photocatalytic_Activity_Nanocellulose |
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author | Guangyu Wei Hong-Fen Zuo Yuan-Ru Guo Qing-Jiang Pan |
author_facet | Guangyu Wei Hong-Fen Zuo Yuan-Ru Guo Qing-Jiang Pan |
author_sort | Guangyu Wei |
collection | DOAJ |
description | Well-crystallized and hexagonal wurtzite ZnO was synthesized with nanocellulose using a facile hydrothermal method. Many highly active (001) facets were retained in the obtained ZnO nanocrystals, presumably due to interaction between the polar facet of ZnO and the nanocellulose. Given its effective surface area, the synthesized ZnO exhibited good photocatalytic activity of degrading methylene blue. Its degradation efficiency reached 94.4% within 30 min (UV irradiation power of 6 W), which was 34% higher than that of Degussa TiO2 P25. The ZnO photocatalyst also exhibited excellent reusability, confirmed by no obvious abatement after its being re-used for 8 cycles. These ZnO nanomaterials were synthesized using renewable nanocellulose derived from cotton. This environmentally friendly and cost-effective approach is anticipated to be applied in the future synthesis of small-sized ZnO photocatalysts. |
first_indexed | 2024-04-13T01:06:14Z |
format | Article |
id | doaj.art-15a72ea440b14cf88ab765a2d940c4e5 |
institution | Directory Open Access Journal |
issn | 1930-2126 1930-2126 |
language | English |
last_indexed | 2024-04-13T01:06:14Z |
publishDate | 2016-06-01 |
publisher | North Carolina State University |
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series | BioResources |
spelling | doaj.art-15a72ea440b14cf88ab765a2d940c4e52022-12-22T03:09:19ZengNorth Carolina State UniversityBioResources1930-21261930-21262016-06-011136244625310.15376/biores.11.3.6244-6253Synthesis of ZnO with Enhanced Photocatalytic Activity: A Novel Approach Using NanocelluloseGuangyu Wei0Hong-Fen Zuo1Yuan-Ru Guo2Qing-Jiang Pan3Heilongjiang University; ChinaNortheast Forestry University; ChinaNortheast Forestry University; ChinaHeilongjiang University; ChinaWell-crystallized and hexagonal wurtzite ZnO was synthesized with nanocellulose using a facile hydrothermal method. Many highly active (001) facets were retained in the obtained ZnO nanocrystals, presumably due to interaction between the polar facet of ZnO and the nanocellulose. Given its effective surface area, the synthesized ZnO exhibited good photocatalytic activity of degrading methylene blue. Its degradation efficiency reached 94.4% within 30 min (UV irradiation power of 6 W), which was 34% higher than that of Degussa TiO2 P25. The ZnO photocatalyst also exhibited excellent reusability, confirmed by no obvious abatement after its being re-used for 8 cycles. These ZnO nanomaterials were synthesized using renewable nanocellulose derived from cotton. This environmentally friendly and cost-effective approach is anticipated to be applied in the future synthesis of small-sized ZnO photocatalysts.http://ojs.cnr.ncsu.edu/index.php/BioRes/article/view/BioRes_11_3_6244_Wei_Synthesis_Photocatalytic_Activity_NanocelluloseNanocrystalline ZnOExposed (001) active facetsNanocelluloseHydrothermalPhotocatalytic activityHydrothermal method |
spellingShingle | Guangyu Wei Hong-Fen Zuo Yuan-Ru Guo Qing-Jiang Pan Synthesis of ZnO with Enhanced Photocatalytic Activity: A Novel Approach Using Nanocellulose BioResources Nanocrystalline ZnO Exposed (001) active facets Nanocellulose Hydrothermal Photocatalytic activity Hydrothermal method |
title | Synthesis of ZnO with Enhanced Photocatalytic Activity: A Novel Approach Using Nanocellulose |
title_full | Synthesis of ZnO with Enhanced Photocatalytic Activity: A Novel Approach Using Nanocellulose |
title_fullStr | Synthesis of ZnO with Enhanced Photocatalytic Activity: A Novel Approach Using Nanocellulose |
title_full_unstemmed | Synthesis of ZnO with Enhanced Photocatalytic Activity: A Novel Approach Using Nanocellulose |
title_short | Synthesis of ZnO with Enhanced Photocatalytic Activity: A Novel Approach Using Nanocellulose |
title_sort | synthesis of zno with enhanced photocatalytic activity a novel approach using nanocellulose |
topic | Nanocrystalline ZnO Exposed (001) active facets Nanocellulose Hydrothermal Photocatalytic activity Hydrothermal method |
url | http://ojs.cnr.ncsu.edu/index.php/BioRes/article/view/BioRes_11_3_6244_Wei_Synthesis_Photocatalytic_Activity_Nanocellulose |
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