Prompt fissionγ-ray characteristics from neutron-induced fission on 239Pu and the time-dependence of prompt-γray emission

Recent years have seen an increased interest in prompt fission γ-ray (PFG) measurements motivated by a high priority request of the OECD/NEA for high precision data, mainly for the nuclear fuel isotopes 235U and 239Pu. Our group has conducted a PFG measurement campaign using state-of-the-art lanthan...

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Main Authors: Gatera Angélique, Göök Alf, Hambsch Franz-Josef, Moens André, Oberstedt Andreas, Oberstedt Stephan, Sibbens Goedele, Vanleeuw David, Vidali Marzio
Format: Article
Language:English
Published: EDP Sciences 2018-01-01
Series:EPJ Web of Conferences
Online Access:https://doi.org/10.1051/epjconf/201816900003
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author Gatera Angélique
Göök Alf
Hambsch Franz-Josef
Moens André
Oberstedt Andreas
Oberstedt Stephan
Sibbens Goedele
Vanleeuw David
Vidali Marzio
author_facet Gatera Angélique
Göök Alf
Hambsch Franz-Josef
Moens André
Oberstedt Andreas
Oberstedt Stephan
Sibbens Goedele
Vanleeuw David
Vidali Marzio
author_sort Gatera Angélique
collection DOAJ
description Recent years have seen an increased interest in prompt fission γ-ray (PFG) measurements motivated by a high priority request of the OECD/NEA for high precision data, mainly for the nuclear fuel isotopes 235U and 239Pu. Our group has conducted a PFG measurement campaign using state-of-the-art lanthanum halide detectors for all the main actinides to a precision better than 3%. The experiments were performed in a coincidence setup between a fission trigger and γ-ray detectors. The time-of-flight technique was used to discriminate photons, traveling at the speed of light, and prompt fission neutrons. For a full rejection of all neutrons below 20 MeV, the PFG time window should not be wider than a few nanoseconds. This window includes most PFG, provided that no isomeric states were populated during the de-excitation process. When isomeric states are populated, PFGs can still be emitted up to 1 yus after the instant of fission or later. To study these γ-rays, the detector response to neutrons had to be determined and a correction had to be applied to the γ-ray spectra. The latest results for PFG characteristics from the reaction 239Pu(nth,f) will be presented, together with an analysis of PFGs emitted up to 200 ns after fission in the spontaneous fission of 252Cf as well as for thermal-neutron induced fission on 235U and 239Pu. The results are compared with calculations in the framework of the Hauser-Feshbach Monte Carlo code CGMF and FIFRELIN.
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spelling doaj.art-1667c0ddb68a4305888c532c948892a32022-12-21T22:08:27ZengEDP SciencesEPJ Web of Conferences2100-014X2018-01-011690000310.1051/epjconf/201816900003epjconf_theory42018_00003Prompt fissionγ-ray characteristics from neutron-induced fission on 239Pu and the time-dependence of prompt-γray emissionGatera AngéliqueGöök AlfHambsch Franz-JosefMoens AndréOberstedt AndreasOberstedt StephanSibbens GoedeleVanleeuw DavidVidali MarzioRecent years have seen an increased interest in prompt fission γ-ray (PFG) measurements motivated by a high priority request of the OECD/NEA for high precision data, mainly for the nuclear fuel isotopes 235U and 239Pu. Our group has conducted a PFG measurement campaign using state-of-the-art lanthanum halide detectors for all the main actinides to a precision better than 3%. The experiments were performed in a coincidence setup between a fission trigger and γ-ray detectors. The time-of-flight technique was used to discriminate photons, traveling at the speed of light, and prompt fission neutrons. For a full rejection of all neutrons below 20 MeV, the PFG time window should not be wider than a few nanoseconds. This window includes most PFG, provided that no isomeric states were populated during the de-excitation process. When isomeric states are populated, PFGs can still be emitted up to 1 yus after the instant of fission or later. To study these γ-rays, the detector response to neutrons had to be determined and a correction had to be applied to the γ-ray spectra. The latest results for PFG characteristics from the reaction 239Pu(nth,f) will be presented, together with an analysis of PFGs emitted up to 200 ns after fission in the spontaneous fission of 252Cf as well as for thermal-neutron induced fission on 235U and 239Pu. The results are compared with calculations in the framework of the Hauser-Feshbach Monte Carlo code CGMF and FIFRELIN.https://doi.org/10.1051/epjconf/201816900003
spellingShingle Gatera Angélique
Göök Alf
Hambsch Franz-Josef
Moens André
Oberstedt Andreas
Oberstedt Stephan
Sibbens Goedele
Vanleeuw David
Vidali Marzio
Prompt fissionγ-ray characteristics from neutron-induced fission on 239Pu and the time-dependence of prompt-γray emission
EPJ Web of Conferences
title Prompt fissionγ-ray characteristics from neutron-induced fission on 239Pu and the time-dependence of prompt-γray emission
title_full Prompt fissionγ-ray characteristics from neutron-induced fission on 239Pu and the time-dependence of prompt-γray emission
title_fullStr Prompt fissionγ-ray characteristics from neutron-induced fission on 239Pu and the time-dependence of prompt-γray emission
title_full_unstemmed Prompt fissionγ-ray characteristics from neutron-induced fission on 239Pu and the time-dependence of prompt-γray emission
title_short Prompt fissionγ-ray characteristics from neutron-induced fission on 239Pu and the time-dependence of prompt-γray emission
title_sort prompt fissionγ ray characteristics from neutron induced fission on 239pu and the time dependence of prompt γray emission
url https://doi.org/10.1051/epjconf/201816900003
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