A ZnO Gas Sensor with an Abnormal Response to Hydrogen

ZnO is a commonly used material for hydrogen gas sensors. In this study, a ZnO nanofiber film with a diameter of approximately 60 nm was synthesized by the electrospinning method. Compared to previously reported ZnO hydrogen gas sensors, an abnormal phenomenon was observed here, where the resistance...

Full description

Bibliographic Details
Main Authors: Hao Sun, Yachi Yao, Ruixuan Yang, Zhaonan Yan, Chen Cao, Yanwen Deng, Shengjiang Wu, Shuhai Liu, Qi Xu, Yong Qin
Format: Article
Language:English
Published: MDPI AG 2023-08-01
Series:Energies
Subjects:
Online Access:https://www.mdpi.com/1996-1073/16/15/5847
_version_ 1797586788482547712
author Hao Sun
Yachi Yao
Ruixuan Yang
Zhaonan Yan
Chen Cao
Yanwen Deng
Shengjiang Wu
Shuhai Liu
Qi Xu
Yong Qin
author_facet Hao Sun
Yachi Yao
Ruixuan Yang
Zhaonan Yan
Chen Cao
Yanwen Deng
Shengjiang Wu
Shuhai Liu
Qi Xu
Yong Qin
author_sort Hao Sun
collection DOAJ
description ZnO is a commonly used material for hydrogen gas sensors. In this study, a ZnO nanofiber film with a diameter of approximately 60 nm was synthesized by the electrospinning method. Compared to previously reported ZnO hydrogen gas sensors, an abnormal phenomenon was observed here, where the resistance of the ZnO nanofiber film increased upon exposure to hydrogen gas in the temperature range from 210 °C to 330 °C. The physical mechanism of this phenomenon was explored through microstructure analysis and DFT simulation calculations that showed a total charge transfer of 0.65 e for the hydrogen molecule. This study can push forward the understanding of ZnO hydrogen sensing.
first_indexed 2024-03-11T00:27:02Z
format Article
id doaj.art-167e0b5f091a4fbc83186dfd560e13b3
institution Directory Open Access Journal
issn 1996-1073
language English
last_indexed 2024-03-11T00:27:02Z
publishDate 2023-08-01
publisher MDPI AG
record_format Article
series Energies
spelling doaj.art-167e0b5f091a4fbc83186dfd560e13b32023-11-18T22:53:36ZengMDPI AGEnergies1996-10732023-08-011615584710.3390/en16155847A ZnO Gas Sensor with an Abnormal Response to HydrogenHao Sun0Yachi Yao1Ruixuan Yang2Zhaonan Yan3Chen Cao4Yanwen Deng5Shengjiang Wu6Shuhai Liu7Qi Xu8Yong Qin9Institute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaInstitute of Nanoscience and Nanotechnology, School of Materials and Energy, Lanzhou University, Lanzhou 730000, ChinaZnO is a commonly used material for hydrogen gas sensors. In this study, a ZnO nanofiber film with a diameter of approximately 60 nm was synthesized by the electrospinning method. Compared to previously reported ZnO hydrogen gas sensors, an abnormal phenomenon was observed here, where the resistance of the ZnO nanofiber film increased upon exposure to hydrogen gas in the temperature range from 210 °C to 330 °C. The physical mechanism of this phenomenon was explored through microstructure analysis and DFT simulation calculations that showed a total charge transfer of 0.65 e for the hydrogen molecule. This study can push forward the understanding of ZnO hydrogen sensing.https://www.mdpi.com/1996-1073/16/15/5847ZnO nanofiber filmhydrogen sensorabnormal response
spellingShingle Hao Sun
Yachi Yao
Ruixuan Yang
Zhaonan Yan
Chen Cao
Yanwen Deng
Shengjiang Wu
Shuhai Liu
Qi Xu
Yong Qin
A ZnO Gas Sensor with an Abnormal Response to Hydrogen
Energies
ZnO nanofiber film
hydrogen sensor
abnormal response
title A ZnO Gas Sensor with an Abnormal Response to Hydrogen
title_full A ZnO Gas Sensor with an Abnormal Response to Hydrogen
title_fullStr A ZnO Gas Sensor with an Abnormal Response to Hydrogen
title_full_unstemmed A ZnO Gas Sensor with an Abnormal Response to Hydrogen
title_short A ZnO Gas Sensor with an Abnormal Response to Hydrogen
title_sort zno gas sensor with an abnormal response to hydrogen
topic ZnO nanofiber film
hydrogen sensor
abnormal response
url https://www.mdpi.com/1996-1073/16/15/5847
work_keys_str_mv AT haosun aznogassensorwithanabnormalresponsetohydrogen
AT yachiyao aznogassensorwithanabnormalresponsetohydrogen
AT ruixuanyang aznogassensorwithanabnormalresponsetohydrogen
AT zhaonanyan aznogassensorwithanabnormalresponsetohydrogen
AT chencao aznogassensorwithanabnormalresponsetohydrogen
AT yanwendeng aznogassensorwithanabnormalresponsetohydrogen
AT shengjiangwu aznogassensorwithanabnormalresponsetohydrogen
AT shuhailiu aznogassensorwithanabnormalresponsetohydrogen
AT qixu aznogassensorwithanabnormalresponsetohydrogen
AT yongqin aznogassensorwithanabnormalresponsetohydrogen
AT haosun znogassensorwithanabnormalresponsetohydrogen
AT yachiyao znogassensorwithanabnormalresponsetohydrogen
AT ruixuanyang znogassensorwithanabnormalresponsetohydrogen
AT zhaonanyan znogassensorwithanabnormalresponsetohydrogen
AT chencao znogassensorwithanabnormalresponsetohydrogen
AT yanwendeng znogassensorwithanabnormalresponsetohydrogen
AT shengjiangwu znogassensorwithanabnormalresponsetohydrogen
AT shuhailiu znogassensorwithanabnormalresponsetohydrogen
AT qixu znogassensorwithanabnormalresponsetohydrogen
AT yongqin znogassensorwithanabnormalresponsetohydrogen