Ultrafast all-optical manipulation of the charge-density wave in VTe_{2}

The charge-density-wave (CDW) phase in the layered transition-metal dichalcogenide VTe_{2} is strongly coupled to the band inversion involving vanadium and tellurium orbitals. In particular, this coupling leads to a selective disappearance of the Dirac-type states that characterize the normal phase,...

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Bibliographic Details
Main Authors: Manuel Tuniz, Davide Soranzio, Davide Bidoggia, Denny Puntel, Wibke Bronsch, Steven L. Johnson, Maria Peressi, Fulvio Parmigiani, Federico Cilento
Format: Article
Language:English
Published: American Physical Society 2023-12-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.5.043276
Description
Summary:The charge-density-wave (CDW) phase in the layered transition-metal dichalcogenide VTe_{2} is strongly coupled to the band inversion involving vanadium and tellurium orbitals. In particular, this coupling leads to a selective disappearance of the Dirac-type states that characterize the normal phase, when the CDW phase sets in. Here, we investigate the broadband time-resolved reflectivity variations caused by collective and single-particle excitations in the CDW ground state of VTe_{2}. With the aid of density functional perturbation theory simulations we unveil the presence of two collective amplitude modes of the CDW ground state. By applying a double-pulse excitation scheme, we show the possibility to manipulate these modes, gaining insights into the coupling between these two collective excitations and demonstrating a more efficient way to perturb the CDW phase in VTe_{2}.
ISSN:2643-1564