Hydrogeochemistry in a relatively unmodified subtropical catchment: Insights regarding the health and aesthetic risks of manganese

Study region: Metal and nutrient concentrations were analysed from freshwater and soil collected from a relatively unmodified ephemeral subtropical catchment in Central Queensland, Australia. Samples were collected quarterly between December 2012 and December 2014. Study focus: There is increasing c...

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Main Authors: Adam K. Rose, Larelle Fabbro, Susan Kinnear
Format: Article
Language:English
Published: Elsevier 2017-10-01
Series:Journal of Hydrology: Regional Studies
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2214581817301453
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author Adam K. Rose
Larelle Fabbro
Susan Kinnear
author_facet Adam K. Rose
Larelle Fabbro
Susan Kinnear
author_sort Adam K. Rose
collection DOAJ
description Study region: Metal and nutrient concentrations were analysed from freshwater and soil collected from a relatively unmodified ephemeral subtropical catchment in Central Queensland, Australia. Samples were collected quarterly between December 2012 and December 2014. Study focus: There is increasing concern about the health effects of manganese in drinking water, prompting interest in understanding manganese dynamics. This study investigated the temporal and spatial patterns of metals and nutrients, as influenced by summer rainfall; and the impacts of those variables on drinking water, associated infrastructure and concomitant health risks. New hydrological insights for region: Results show that the hydrogeochemistry of Baffle Creek was predominantly driven by rain events, with differing responses to varying magnitudes of rain and discharge. Following a flushing event, dissolved aluminium and nitrate increased in the surface and drinking water, whereas manganese and ammonia were undetectable in the drinking water and occurred only in small concentrations in the surface waters. In contrast, when rainfall events occurred without an associated flush, manganese, iron and ammonia concentrations increased in the drinking water. The hydrochemistry of manganese and iron in the supply chain infrastructure was strongly positively correlated with ammonia, and aluminium correlated with nitrate concentrations. Currently the drinking water supply does not pose a threat to chronic manganese exposure for humans, however elevated concentrations are experienced periodically; and may become more problematic under climate change scenarios.
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spelling doaj.art-1a318c5ef7964b87b7b0f010a70a22a22022-12-22T00:03:36ZengElsevierJournal of Hydrology: Regional Studies2214-58182017-10-0113C15216710.1016/j.ejrh.2017.08.008Hydrogeochemistry in a relatively unmodified subtropical catchment: Insights regarding the health and aesthetic risks of manganeseAdam K. Rose0Larelle Fabbro1Susan Kinnear2School of Medical and Applied Sciences, Central Queensland University, North Rockhampton, Queensland, AustraliaSchool of Medical and Applied Sciences, Central Queensland University, North Rockhampton, Queensland, AustraliaResearch Division, Central Queensland University, North Rockhampton, Queensland,, AustraliaStudy region: Metal and nutrient concentrations were analysed from freshwater and soil collected from a relatively unmodified ephemeral subtropical catchment in Central Queensland, Australia. Samples were collected quarterly between December 2012 and December 2014. Study focus: There is increasing concern about the health effects of manganese in drinking water, prompting interest in understanding manganese dynamics. This study investigated the temporal and spatial patterns of metals and nutrients, as influenced by summer rainfall; and the impacts of those variables on drinking water, associated infrastructure and concomitant health risks. New hydrological insights for region: Results show that the hydrogeochemistry of Baffle Creek was predominantly driven by rain events, with differing responses to varying magnitudes of rain and discharge. Following a flushing event, dissolved aluminium and nitrate increased in the surface and drinking water, whereas manganese and ammonia were undetectable in the drinking water and occurred only in small concentrations in the surface waters. In contrast, when rainfall events occurred without an associated flush, manganese, iron and ammonia concentrations increased in the drinking water. The hydrochemistry of manganese and iron in the supply chain infrastructure was strongly positively correlated with ammonia, and aluminium correlated with nitrate concentrations. Currently the drinking water supply does not pose a threat to chronic manganese exposure for humans, however elevated concentrations are experienced periodically; and may become more problematic under climate change scenarios.http://www.sciencedirect.com/science/article/pii/S2214581817301453AustraliaRainfallRunoffDrinkingEphemeralFlood
spellingShingle Adam K. Rose
Larelle Fabbro
Susan Kinnear
Hydrogeochemistry in a relatively unmodified subtropical catchment: Insights regarding the health and aesthetic risks of manganese
Journal of Hydrology: Regional Studies
Australia
Rainfall
Runoff
Drinking
Ephemeral
Flood
title Hydrogeochemistry in a relatively unmodified subtropical catchment: Insights regarding the health and aesthetic risks of manganese
title_full Hydrogeochemistry in a relatively unmodified subtropical catchment: Insights regarding the health and aesthetic risks of manganese
title_fullStr Hydrogeochemistry in a relatively unmodified subtropical catchment: Insights regarding the health and aesthetic risks of manganese
title_full_unstemmed Hydrogeochemistry in a relatively unmodified subtropical catchment: Insights regarding the health and aesthetic risks of manganese
title_short Hydrogeochemistry in a relatively unmodified subtropical catchment: Insights regarding the health and aesthetic risks of manganese
title_sort hydrogeochemistry in a relatively unmodified subtropical catchment insights regarding the health and aesthetic risks of manganese
topic Australia
Rainfall
Runoff
Drinking
Ephemeral
Flood
url http://www.sciencedirect.com/science/article/pii/S2214581817301453
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AT larellefabbro hydrogeochemistryinarelativelyunmodifiedsubtropicalcatchmentinsightsregardingthehealthandaestheticrisksofmanganese
AT susankinnear hydrogeochemistryinarelativelyunmodifiedsubtropicalcatchmentinsightsregardingthehealthandaestheticrisksofmanganese