Theoretical Investigation of All Optical Switching by Intersystem Crossing

The dynamics of spin flips induced by the femtosecond laser are theoretically investigated in this article. The spin flips in this scenario are attributed to the intersystem crossing (ISC) described within the frame of the Rabi model. This new explanation is a step attempting to explain the mechanis...

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Main Authors: Yuhao Zou, Haiwei Wang, Haozhe Huang, Zhihao Zeng, Kai Wang, Sicong Wang, Xiangping Li, Changsheng Xie
Format: Article
Language:English
Published: MDPI AG 2019-12-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/10/1/128
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author Yuhao Zou
Haiwei Wang
Haozhe Huang
Zhihao Zeng
Kai Wang
Sicong Wang
Xiangping Li
Changsheng Xie
author_facet Yuhao Zou
Haiwei Wang
Haozhe Huang
Zhihao Zeng
Kai Wang
Sicong Wang
Xiangping Li
Changsheng Xie
author_sort Yuhao Zou
collection DOAJ
description The dynamics of spin flips induced by the femtosecond laser are theoretically investigated in this article. The spin flips in this scenario are attributed to the intersystem crossing (ISC) described within the frame of the Rabi model. This new explanation is a step attempting to explain the mechanism of the all-optical magnetic orientation switching in the perspective of the conservation of the angular momentum and breaks of the selection rule, which is ignored in the Raman scattering related explanations. The final spin states discussed herein are closely related to the intensity of the incident laser and the ISC decay rate. The quantitative analysis of the relation between decay rate, temperature and the intensity of the laser is discussed.
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spelling doaj.art-1a34c79f26104ac5b6558bfcb64f8e8f2022-12-22T02:06:27ZengMDPI AGApplied Sciences2076-34172019-12-0110112810.3390/app10010128app10010128Theoretical Investigation of All Optical Switching by Intersystem CrossingYuhao Zou0Haiwei Wang1Haozhe Huang2Zhihao Zeng3Kai Wang4Sicong Wang5Xiangping Li6Changsheng Xie7Wuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaWuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaWuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaWuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaSchool of Physics, Huazhong University of Science and Technology, Wuhan 430074, ChinaGuangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications, Institute of Photonics Technology, Jinan University, Guangzhou 510632, ChinaGuangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications, Institute of Photonics Technology, Jinan University, Guangzhou 510632, ChinaWuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaThe dynamics of spin flips induced by the femtosecond laser are theoretically investigated in this article. The spin flips in this scenario are attributed to the intersystem crossing (ISC) described within the frame of the Rabi model. This new explanation is a step attempting to explain the mechanism of the all-optical magnetic orientation switching in the perspective of the conservation of the angular momentum and breaks of the selection rule, which is ignored in the Raman scattering related explanations. The final spin states discussed herein are closely related to the intensity of the incident laser and the ISC decay rate. The quantitative analysis of the relation between decay rate, temperature and the intensity of the laser is discussed.https://www.mdpi.com/2076-3417/10/1/128intersystem crossingspin-orbit couplingall-optical switchingangular momentum
spellingShingle Yuhao Zou
Haiwei Wang
Haozhe Huang
Zhihao Zeng
Kai Wang
Sicong Wang
Xiangping Li
Changsheng Xie
Theoretical Investigation of All Optical Switching by Intersystem Crossing
Applied Sciences
intersystem crossing
spin-orbit coupling
all-optical switching
angular momentum
title Theoretical Investigation of All Optical Switching by Intersystem Crossing
title_full Theoretical Investigation of All Optical Switching by Intersystem Crossing
title_fullStr Theoretical Investigation of All Optical Switching by Intersystem Crossing
title_full_unstemmed Theoretical Investigation of All Optical Switching by Intersystem Crossing
title_short Theoretical Investigation of All Optical Switching by Intersystem Crossing
title_sort theoretical investigation of all optical switching by intersystem crossing
topic intersystem crossing
spin-orbit coupling
all-optical switching
angular momentum
url https://www.mdpi.com/2076-3417/10/1/128
work_keys_str_mv AT yuhaozou theoreticalinvestigationofallopticalswitchingbyintersystemcrossing
AT haiweiwang theoreticalinvestigationofallopticalswitchingbyintersystemcrossing
AT haozhehuang theoreticalinvestigationofallopticalswitchingbyintersystemcrossing
AT zhihaozeng theoreticalinvestigationofallopticalswitchingbyintersystemcrossing
AT kaiwang theoreticalinvestigationofallopticalswitchingbyintersystemcrossing
AT sicongwang theoreticalinvestigationofallopticalswitchingbyintersystemcrossing
AT xiangpingli theoreticalinvestigationofallopticalswitchingbyintersystemcrossing
AT changshengxie theoreticalinvestigationofallopticalswitchingbyintersystemcrossing