Theoretical Investigation of All Optical Switching by Intersystem Crossing
The dynamics of spin flips induced by the femtosecond laser are theoretically investigated in this article. The spin flips in this scenario are attributed to the intersystem crossing (ISC) described within the frame of the Rabi model. This new explanation is a step attempting to explain the mechanis...
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MDPI AG
2019-12-01
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Online Access: | https://www.mdpi.com/2076-3417/10/1/128 |
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author | Yuhao Zou Haiwei Wang Haozhe Huang Zhihao Zeng Kai Wang Sicong Wang Xiangping Li Changsheng Xie |
author_facet | Yuhao Zou Haiwei Wang Haozhe Huang Zhihao Zeng Kai Wang Sicong Wang Xiangping Li Changsheng Xie |
author_sort | Yuhao Zou |
collection | DOAJ |
description | The dynamics of spin flips induced by the femtosecond laser are theoretically investigated in this article. The spin flips in this scenario are attributed to the intersystem crossing (ISC) described within the frame of the Rabi model. This new explanation is a step attempting to explain the mechanism of the all-optical magnetic orientation switching in the perspective of the conservation of the angular momentum and breaks of the selection rule, which is ignored in the Raman scattering related explanations. The final spin states discussed herein are closely related to the intensity of the incident laser and the ISC decay rate. The quantitative analysis of the relation between decay rate, temperature and the intensity of the laser is discussed. |
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id | doaj.art-1a34c79f26104ac5b6558bfcb64f8e8f |
institution | Directory Open Access Journal |
issn | 2076-3417 |
language | English |
last_indexed | 2024-04-14T07:10:03Z |
publishDate | 2019-12-01 |
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series | Applied Sciences |
spelling | doaj.art-1a34c79f26104ac5b6558bfcb64f8e8f2022-12-22T02:06:27ZengMDPI AGApplied Sciences2076-34172019-12-0110112810.3390/app10010128app10010128Theoretical Investigation of All Optical Switching by Intersystem CrossingYuhao Zou0Haiwei Wang1Haozhe Huang2Zhihao Zeng3Kai Wang4Sicong Wang5Xiangping Li6Changsheng Xie7Wuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaWuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaWuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaWuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaSchool of Physics, Huazhong University of Science and Technology, Wuhan 430074, ChinaGuangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications, Institute of Photonics Technology, Jinan University, Guangzhou 510632, ChinaGuangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications, Institute of Photonics Technology, Jinan University, Guangzhou 510632, ChinaWuhan National Laboratory of Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, ChinaThe dynamics of spin flips induced by the femtosecond laser are theoretically investigated in this article. The spin flips in this scenario are attributed to the intersystem crossing (ISC) described within the frame of the Rabi model. This new explanation is a step attempting to explain the mechanism of the all-optical magnetic orientation switching in the perspective of the conservation of the angular momentum and breaks of the selection rule, which is ignored in the Raman scattering related explanations. The final spin states discussed herein are closely related to the intensity of the incident laser and the ISC decay rate. The quantitative analysis of the relation between decay rate, temperature and the intensity of the laser is discussed.https://www.mdpi.com/2076-3417/10/1/128intersystem crossingspin-orbit couplingall-optical switchingangular momentum |
spellingShingle | Yuhao Zou Haiwei Wang Haozhe Huang Zhihao Zeng Kai Wang Sicong Wang Xiangping Li Changsheng Xie Theoretical Investigation of All Optical Switching by Intersystem Crossing Applied Sciences intersystem crossing spin-orbit coupling all-optical switching angular momentum |
title | Theoretical Investigation of All Optical Switching by Intersystem Crossing |
title_full | Theoretical Investigation of All Optical Switching by Intersystem Crossing |
title_fullStr | Theoretical Investigation of All Optical Switching by Intersystem Crossing |
title_full_unstemmed | Theoretical Investigation of All Optical Switching by Intersystem Crossing |
title_short | Theoretical Investigation of All Optical Switching by Intersystem Crossing |
title_sort | theoretical investigation of all optical switching by intersystem crossing |
topic | intersystem crossing spin-orbit coupling all-optical switching angular momentum |
url | https://www.mdpi.com/2076-3417/10/1/128 |
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