Contrasting ice formation in Arctic clouds: surface-coupled vs. surface-decoupled clouds

<p>In the Arctic summer of 2017 (1 June to 16 July) measurements with the OCEANET-Atmosphere facility were performed during the <i>Polarstern</i> cruise PS106. OCEANET comprises amongst other instruments the multiwavelength polarization lidar Polly<span class="inline-formul...

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Main Authors: H. J. Griesche, K. Ohneiser, P. Seifert, M. Radenz, R. Engelmann, A. Ansmann
Format: Article
Language:English
Published: Copernicus Publications 2021-07-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/21/10357/2021/acp-21-10357-2021.pdf
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author H. J. Griesche
K. Ohneiser
P. Seifert
M. Radenz
R. Engelmann
A. Ansmann
author_facet H. J. Griesche
K. Ohneiser
P. Seifert
M. Radenz
R. Engelmann
A. Ansmann
author_sort H. J. Griesche
collection DOAJ
description <p>In the Arctic summer of 2017 (1 June to 16 July) measurements with the OCEANET-Atmosphere facility were performed during the <i>Polarstern</i> cruise PS106. OCEANET comprises amongst other instruments the multiwavelength polarization lidar Polly<span class="inline-formula"><sup>XT</sup></span>_OCEANET and for PS106 was complemented with a vertically pointed 35 <span class="inline-formula">GHz</span> cloud radar. In the scope of the presented study, the influence of cloud height and surface coupling on the probability of clouds to contain and form ice is investigated. Polarimetric lidar data were used for the detection of the cloud base and the identification of the thermodynamic phase. Both radar and lidar were used to detect cloud top. Radiosonde data were used to derive the thermodynamic structure of the atmosphere and the clouds. The analyzed data set shows a significant impact of the surface-coupling state on the probability of ice formation. Surface-coupled clouds were identified by a quasi-constant potential temperature profile from the surface up to liquid layer base. Within the same minimum cloud temperature range, ice-containing clouds have been observed more frequently than surface-decoupled clouds by a factor of up to 6 (temperature intervals between <span class="inline-formula">−</span>7.5 and <span class="inline-formula">−</span>5 <span class="inline-formula"><sup>∘</sup>C</span>, 164 vs. 27 analyzed intervals of 30 <span class="inline-formula">min</span>). The frequency of occurrence of surface-coupled ice-containing clouds was found to be 2–3 times higher (e.g., 82 <span class="inline-formula">%</span> vs. 35 <span class="inline-formula">%</span> between <span class="inline-formula">−</span>7.5 and <span class="inline-formula">−</span>5 <span class="inline-formula"><sup>∘</sup>C</span>). These findings provide evidence that above <span class="inline-formula">−</span>10 <span class="inline-formula"><sup>∘</sup>C</span> heterogeneous ice formation in Arctic mixed-phase clouds occurs by a factor of 2–6 more often when the cloud layer is coupled to the surface. In turn, for minimum cloud temperatures below <span class="inline-formula">−</span>15 <span class="inline-formula"><sup>∘</sup>C</span>, the frequency of ice-containing clouds for coupled and decoupled conditions approached the respective curve for the central European site of Leipzig, Germany (51<span class="inline-formula"><sup>∘</sup></span> N, 12<span class="inline-formula"><sup>∘</sup></span> E). This corroborates the hypothesis that the free-tropospheric ice nucleating particle (INP) reservoir over the Arctic is controlled by continental aerosol. Two sensitivity studies, also using the cloud radar for detection of ice particles and applying a modified coupling state detection, both confirmed the findings, albeit with a lower magnitude. Possible explanations for the observations are discussed by considering recent in situ measurements of INP in the Arctic, of which much higher concentrations were found in the surface-coupled atmosphere in close vicinity to the ice shore.</p>
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spelling doaj.art-1a90049c065e4a5f85194a9867061e332022-12-21T22:39:38ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242021-07-0121103571037410.5194/acp-21-10357-2021Contrasting ice formation in Arctic clouds: surface-coupled vs. surface-decoupled cloudsH. J. GriescheK. OhneiserP. SeifertM. RadenzR. EngelmannA. Ansmann<p>In the Arctic summer of 2017 (1 June to 16 July) measurements with the OCEANET-Atmosphere facility were performed during the <i>Polarstern</i> cruise PS106. OCEANET comprises amongst other instruments the multiwavelength polarization lidar Polly<span class="inline-formula"><sup>XT</sup></span>_OCEANET and for PS106 was complemented with a vertically pointed 35 <span class="inline-formula">GHz</span> cloud radar. In the scope of the presented study, the influence of cloud height and surface coupling on the probability of clouds to contain and form ice is investigated. Polarimetric lidar data were used for the detection of the cloud base and the identification of the thermodynamic phase. Both radar and lidar were used to detect cloud top. Radiosonde data were used to derive the thermodynamic structure of the atmosphere and the clouds. The analyzed data set shows a significant impact of the surface-coupling state on the probability of ice formation. Surface-coupled clouds were identified by a quasi-constant potential temperature profile from the surface up to liquid layer base. Within the same minimum cloud temperature range, ice-containing clouds have been observed more frequently than surface-decoupled clouds by a factor of up to 6 (temperature intervals between <span class="inline-formula">−</span>7.5 and <span class="inline-formula">−</span>5 <span class="inline-formula"><sup>∘</sup>C</span>, 164 vs. 27 analyzed intervals of 30 <span class="inline-formula">min</span>). The frequency of occurrence of surface-coupled ice-containing clouds was found to be 2–3 times higher (e.g., 82 <span class="inline-formula">%</span> vs. 35 <span class="inline-formula">%</span> between <span class="inline-formula">−</span>7.5 and <span class="inline-formula">−</span>5 <span class="inline-formula"><sup>∘</sup>C</span>). These findings provide evidence that above <span class="inline-formula">−</span>10 <span class="inline-formula"><sup>∘</sup>C</span> heterogeneous ice formation in Arctic mixed-phase clouds occurs by a factor of 2–6 more often when the cloud layer is coupled to the surface. In turn, for minimum cloud temperatures below <span class="inline-formula">−</span>15 <span class="inline-formula"><sup>∘</sup>C</span>, the frequency of ice-containing clouds for coupled and decoupled conditions approached the respective curve for the central European site of Leipzig, Germany (51<span class="inline-formula"><sup>∘</sup></span> N, 12<span class="inline-formula"><sup>∘</sup></span> E). This corroborates the hypothesis that the free-tropospheric ice nucleating particle (INP) reservoir over the Arctic is controlled by continental aerosol. Two sensitivity studies, also using the cloud radar for detection of ice particles and applying a modified coupling state detection, both confirmed the findings, albeit with a lower magnitude. Possible explanations for the observations are discussed by considering recent in situ measurements of INP in the Arctic, of which much higher concentrations were found in the surface-coupled atmosphere in close vicinity to the ice shore.</p>https://acp.copernicus.org/articles/21/10357/2021/acp-21-10357-2021.pdf
spellingShingle H. J. Griesche
K. Ohneiser
P. Seifert
M. Radenz
R. Engelmann
A. Ansmann
Contrasting ice formation in Arctic clouds: surface-coupled vs. surface-decoupled clouds
Atmospheric Chemistry and Physics
title Contrasting ice formation in Arctic clouds: surface-coupled vs. surface-decoupled clouds
title_full Contrasting ice formation in Arctic clouds: surface-coupled vs. surface-decoupled clouds
title_fullStr Contrasting ice formation in Arctic clouds: surface-coupled vs. surface-decoupled clouds
title_full_unstemmed Contrasting ice formation in Arctic clouds: surface-coupled vs. surface-decoupled clouds
title_short Contrasting ice formation in Arctic clouds: surface-coupled vs. surface-decoupled clouds
title_sort contrasting ice formation in arctic clouds surface coupled vs surface decoupled clouds
url https://acp.copernicus.org/articles/21/10357/2021/acp-21-10357-2021.pdf
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AT kohneiser contrastingiceformationinarcticcloudssurfacecoupledvssurfacedecoupledclouds
AT pseifert contrastingiceformationinarcticcloudssurfacecoupledvssurfacedecoupledclouds
AT mradenz contrastingiceformationinarcticcloudssurfacecoupledvssurfacedecoupledclouds
AT rengelmann contrastingiceformationinarcticcloudssurfacecoupledvssurfacedecoupledclouds
AT aansmann contrastingiceformationinarcticcloudssurfacecoupledvssurfacedecoupledclouds