Advancing high‐performance one‐dimensional Si/carbon anodes: Current status and challenges

Abstract Silicon (Si) anodes, known for their high capacity, confront obstacles such as volume expansion, the solid–electrolyte interface (SEI) formation, and limited cyclability, driving ongoing research for innovative solutions to enhance their performance in next‐generation lithium‐ion batteries...

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Main Authors: Xinyu Chen, Yongbiao Mu, Zifan Liao, Youqi Chu, Shaowei Kang, Bu‐ke Wu, Ruixi Liao, Meisheng Han, Yiju Li, Lin Zeng
Format: Article
Language:English
Published: Wiley 2024-03-01
Series:Carbon Neutralization
Subjects:
Online Access:https://doi.org/10.1002/cnl2.118
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author Xinyu Chen
Yongbiao Mu
Zifan Liao
Youqi Chu
Shaowei Kang
Bu‐ke Wu
Ruixi Liao
Meisheng Han
Yiju Li
Lin Zeng
author_facet Xinyu Chen
Yongbiao Mu
Zifan Liao
Youqi Chu
Shaowei Kang
Bu‐ke Wu
Ruixi Liao
Meisheng Han
Yiju Li
Lin Zeng
author_sort Xinyu Chen
collection DOAJ
description Abstract Silicon (Si) anodes, known for their high capacity, confront obstacles such as volume expansion, the solid–electrolyte interface (SEI) formation, and limited cyclability, driving ongoing research for innovative solutions to enhance their performance in next‐generation lithium‐ion batteries (LIBs). This comprehensive review explores the forefront of one‐dimensional (1D) Si/carbon anodes for high‐performance LIBs. This review delves into cutting‐edge strategies for fabricating 1D Si/carbon structures, such as nanowires, nanotubes, and nanofibers, highlighting their advantages in mitigating volume expansion, enhancing electron/ion transport, and bolstering cycling stability. The review showcases remarkable achievements in 1D Si/carbon anode performance, including exceptional capacity retention, high‐rate capability, and prolonged cycle life. Challenges regarding scalability, cost‐effectiveness, and long‐term stability are addressed, providing insights into the path to commercialization. Additionally, future directions and potential breakthroughs are outlined, guiding researchers and industries toward harnessing the potential of 1D Si/carbon anodes in revolutionizing energy storage.
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spelling doaj.art-1acb9b53304242e884e5ecfef8fc7b212024-03-30T18:01:27ZengWileyCarbon Neutralization2769-33252024-03-013219922110.1002/cnl2.118Advancing high‐performance one‐dimensional Si/carbon anodes: Current status and challengesXinyu Chen0Yongbiao Mu1Zifan Liao2Youqi Chu3Shaowei Kang4Bu‐ke Wu5Ruixi Liao6Meisheng Han7Yiju Li8Lin Zeng9Shenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaShenzhen Key Laboratory of Advanced Energy Storage, Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen ChinaAbstract Silicon (Si) anodes, known for their high capacity, confront obstacles such as volume expansion, the solid–electrolyte interface (SEI) formation, and limited cyclability, driving ongoing research for innovative solutions to enhance their performance in next‐generation lithium‐ion batteries (LIBs). This comprehensive review explores the forefront of one‐dimensional (1D) Si/carbon anodes for high‐performance LIBs. This review delves into cutting‐edge strategies for fabricating 1D Si/carbon structures, such as nanowires, nanotubes, and nanofibers, highlighting their advantages in mitigating volume expansion, enhancing electron/ion transport, and bolstering cycling stability. The review showcases remarkable achievements in 1D Si/carbon anode performance, including exceptional capacity retention, high‐rate capability, and prolonged cycle life. Challenges regarding scalability, cost‐effectiveness, and long‐term stability are addressed, providing insights into the path to commercialization. Additionally, future directions and potential breakthroughs are outlined, guiding researchers and industries toward harnessing the potential of 1D Si/carbon anodes in revolutionizing energy storage.https://doi.org/10.1002/cnl2.1181D Si/carbonhigh‐performancelithium‐ion batteriesSi anodesSi nanosizing
spellingShingle Xinyu Chen
Yongbiao Mu
Zifan Liao
Youqi Chu
Shaowei Kang
Bu‐ke Wu
Ruixi Liao
Meisheng Han
Yiju Li
Lin Zeng
Advancing high‐performance one‐dimensional Si/carbon anodes: Current status and challenges
Carbon Neutralization
1D Si/carbon
high‐performance
lithium‐ion batteries
Si anodes
Si nanosizing
title Advancing high‐performance one‐dimensional Si/carbon anodes: Current status and challenges
title_full Advancing high‐performance one‐dimensional Si/carbon anodes: Current status and challenges
title_fullStr Advancing high‐performance one‐dimensional Si/carbon anodes: Current status and challenges
title_full_unstemmed Advancing high‐performance one‐dimensional Si/carbon anodes: Current status and challenges
title_short Advancing high‐performance one‐dimensional Si/carbon anodes: Current status and challenges
title_sort advancing high performance one dimensional si carbon anodes current status and challenges
topic 1D Si/carbon
high‐performance
lithium‐ion batteries
Si anodes
Si nanosizing
url https://doi.org/10.1002/cnl2.118
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AT youqichu advancinghighperformanceonedimensionalsicarbonanodescurrentstatusandchallenges
AT shaoweikang advancinghighperformanceonedimensionalsicarbonanodescurrentstatusandchallenges
AT bukewu advancinghighperformanceonedimensionalsicarbonanodescurrentstatusandchallenges
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