Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathways

The direct carbonation of steel slag has emerged as a promising approach for carbon dioxide (CO2) utilization and sequestration, holding potential for advancing sustainable steel production. Despite considerably high expectations for these cleaner upcycling pathways, their maturity level remains rel...

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Main Authors: Christopher DiGiovanni, Ousmane A. Hisseine, Adedapo Noah Awolayo
Format: Article
Language:English
Published: Elsevier 2024-03-01
Series:Journal of CO2 Utilization
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2212982024000714
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author Christopher DiGiovanni
Ousmane A. Hisseine
Adedapo Noah Awolayo
author_facet Christopher DiGiovanni
Ousmane A. Hisseine
Adedapo Noah Awolayo
author_sort Christopher DiGiovanni
collection DOAJ
description The direct carbonation of steel slag has emerged as a promising approach for carbon dioxide (CO2) utilization and sequestration, holding potential for advancing sustainable steel production. Despite considerably high expectations for these cleaner upcycling pathways, their maturity level remains relatively low and large-scale direct carbonation of steel slag is largely untested. To facilitate steel slag carbonation on a scale necessary for a zero-carbon future economy, this article provides a comprehensive review of fundamental carbonation mechanisms and critical parameters governing the reaction process, including temperature, pressure, reaction time, liquid-to-solid ratio, and CO2 partial pressure. The study critically examines the unique interactions among these process parameters, which can either limit or enhance the process optimization. The spectrum of scientific challenges associated with this pathway, including reaction rate limitations and the carbonated product valorization, particularly as a binder or aggregate in the construction sector, are identified and addressed. These insights aim to enhance the carbonation potential of steel slag for possible cleaner upcycling implementation pathways, ultimately facilitating the development of more efficient and sustainable carbon capture utilization and sequestration (CCUS) technologies. The proposed improvements are expected to be instrumental in promoting sustainable practices, not only to foster the decarbonization of the steelmaking industry but also in aiding other hard-to-abate sectors, such as the cement and concrete industry, in achieving their own decarbonization goals.
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spelling doaj.art-1adbbfe7117b4c29afe28e4e5a34390d2024-03-29T05:50:09ZengElsevierJournal of CO2 Utilization2212-98392024-03-0181102736Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathwaysChristopher DiGiovanni0Ousmane A. Hisseine1Adedapo Noah Awolayo2CanmetMATERIALS, Natural Resources Canada, 183 Longwood Rd S, Hamilton, ON L8P 0A5, Canada; Corresponding author.Department of Civil Engineering, McMaster University, 1280 Main St W, Hamilton, ON L8S 4L8, CanadaDepartment of Civil Engineering, McMaster University, 1280 Main St W, Hamilton, ON L8S 4L8, CanadaThe direct carbonation of steel slag has emerged as a promising approach for carbon dioxide (CO2) utilization and sequestration, holding potential for advancing sustainable steel production. Despite considerably high expectations for these cleaner upcycling pathways, their maturity level remains relatively low and large-scale direct carbonation of steel slag is largely untested. To facilitate steel slag carbonation on a scale necessary for a zero-carbon future economy, this article provides a comprehensive review of fundamental carbonation mechanisms and critical parameters governing the reaction process, including temperature, pressure, reaction time, liquid-to-solid ratio, and CO2 partial pressure. The study critically examines the unique interactions among these process parameters, which can either limit or enhance the process optimization. The spectrum of scientific challenges associated with this pathway, including reaction rate limitations and the carbonated product valorization, particularly as a binder or aggregate in the construction sector, are identified and addressed. These insights aim to enhance the carbonation potential of steel slag for possible cleaner upcycling implementation pathways, ultimately facilitating the development of more efficient and sustainable carbon capture utilization and sequestration (CCUS) technologies. The proposed improvements are expected to be instrumental in promoting sustainable practices, not only to foster the decarbonization of the steelmaking industry but also in aiding other hard-to-abate sectors, such as the cement and concrete industry, in achieving their own decarbonization goals.http://www.sciencedirect.com/science/article/pii/S2212982024000714Carbon capture utilization and sequestrationcarbonationdecarbonizationsteel slag aggregatessteel slagsteelmaking
spellingShingle Christopher DiGiovanni
Ousmane A. Hisseine
Adedapo Noah Awolayo
Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathways
Journal of CO2 Utilization
Carbon capture utilization and sequestration
carbonation
decarbonization
steel slag aggregates
steel slag
steelmaking
title Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathways
title_full Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathways
title_fullStr Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathways
title_full_unstemmed Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathways
title_short Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathways
title_sort carbon dioxide sequestration through steel slag carbonation review of mechanisms process parameters and cleaner upcycling pathways
topic Carbon capture utilization and sequestration
carbonation
decarbonization
steel slag aggregates
steel slag
steelmaking
url http://www.sciencedirect.com/science/article/pii/S2212982024000714
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