Active and fast charge-state switching of single NV centres in diamond by in-plane Al-Schottky junctions

In this paper, we demonstrate an active and fast control of the charge state and hence of the optical and electronic properties of single and near-surface nitrogen-vacancy centres (NV centres) in diamond. This active manipulation is achieved by using a two-dimensional Schottky-diode structure from d...

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Main Authors: Christoph Schreyvogel, Vladimir Polyakov, Sina Burk, Helmut Fedder, Andrej Denisenko, Felipe Fávaro de Oliveira, Ralf Wunderlich, Jan Meijer, Verena Zuerbig, Jörg Wrachtrup, Christoph E. Nebel
Format: Article
Language:English
Published: Beilstein-Institut 2016-11-01
Series:Beilstein Journal of Nanotechnology
Subjects:
Online Access:https://doi.org/10.3762/bjnano.7.165
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author Christoph Schreyvogel
Vladimir Polyakov
Sina Burk
Helmut Fedder
Andrej Denisenko
Felipe Fávaro de Oliveira
Ralf Wunderlich
Jan Meijer
Verena Zuerbig
Jörg Wrachtrup
Christoph E. Nebel
author_facet Christoph Schreyvogel
Vladimir Polyakov
Sina Burk
Helmut Fedder
Andrej Denisenko
Felipe Fávaro de Oliveira
Ralf Wunderlich
Jan Meijer
Verena Zuerbig
Jörg Wrachtrup
Christoph E. Nebel
author_sort Christoph Schreyvogel
collection DOAJ
description In this paper, we demonstrate an active and fast control of the charge state and hence of the optical and electronic properties of single and near-surface nitrogen-vacancy centres (NV centres) in diamond. This active manipulation is achieved by using a two-dimensional Schottky-diode structure from diamond, i.e., by using aluminium as Schottky contact on a hydrogen terminated diamond surface. By changing the applied potential on the Schottky contact, we are able to actively switch single NV centres between all three charge states NV+, NV0 and NV− on a timescale of 10 to 100 ns, corresponding to a switching frequency of 10–100 MHz. This switching frequency is much higher than the hyperfine interaction frequency between an electron spin (of NV−) and a nuclear spin (of 15N or 13C for example) of 2.66 kHz. This high-frequency charge state switching with a planar diode structure would open the door for many quantum optical applications such as a quantum computer with single NVs for quantum information processing as well as single 13C atoms for long-lifetime storage of quantum information. Furthermore, a control of spectral emission properties of single NVs as a single photon emitters – embedded in photonic structures for example – can be realized which would be vital for quantum communication and cryptography.
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spelling doaj.art-1adf8613292c44d39fc4d15ae5b4776c2022-12-22T03:50:53ZengBeilstein-InstitutBeilstein Journal of Nanotechnology2190-42862016-11-01711727173510.3762/bjnano.7.1652190-4286-7-165Active and fast charge-state switching of single NV centres in diamond by in-plane Al-Schottky junctionsChristoph Schreyvogel0Vladimir Polyakov1Sina Burk2Helmut Fedder3Andrej Denisenko4Felipe Fávaro de Oliveira5Ralf Wunderlich6Jan Meijer7Verena Zuerbig8Jörg Wrachtrup9Christoph E. Nebel10Fraunhofer-Institute for Applied Solid State Physics (IAF), 79108 Freiburg, GermanyFraunhofer-Institute for Applied Solid State Physics (IAF), 79108 Freiburg, Germany3rd Institute of Physics, University of Stuttgart, 70569 Stuttgart, Germany3rd Institute of Physics, University of Stuttgart, 70569 Stuttgart, Germany3rd Institute of Physics, University of Stuttgart, 70569 Stuttgart, Germany3rd Institute of Physics, University of Stuttgart, 70569 Stuttgart, GermanyDepartment of Physics and Geoscience, University of Leipzig, 04103 Leipzig, GermanyDepartment of Physics and Geoscience, University of Leipzig, 04103 Leipzig, GermanyFraunhofer-Institute for Applied Solid State Physics (IAF), 79108 Freiburg, Germany3rd Institute of Physics, University of Stuttgart, 70569 Stuttgart, GermanyFraunhofer-Institute for Applied Solid State Physics (IAF), 79108 Freiburg, GermanyIn this paper, we demonstrate an active and fast control of the charge state and hence of the optical and electronic properties of single and near-surface nitrogen-vacancy centres (NV centres) in diamond. This active manipulation is achieved by using a two-dimensional Schottky-diode structure from diamond, i.e., by using aluminium as Schottky contact on a hydrogen terminated diamond surface. By changing the applied potential on the Schottky contact, we are able to actively switch single NV centres between all three charge states NV+, NV0 and NV− on a timescale of 10 to 100 ns, corresponding to a switching frequency of 10–100 MHz. This switching frequency is much higher than the hyperfine interaction frequency between an electron spin (of NV−) and a nuclear spin (of 15N or 13C for example) of 2.66 kHz. This high-frequency charge state switching with a planar diode structure would open the door for many quantum optical applications such as a quantum computer with single NVs for quantum information processing as well as single 13C atoms for long-lifetime storage of quantum information. Furthermore, a control of spectral emission properties of single NVs as a single photon emitters – embedded in photonic structures for example – can be realized which would be vital for quantum communication and cryptography.https://doi.org/10.3762/bjnano.7.165active charge state controldiamondfast charge state switchingNV centretwo-dimensional Schottky diode
spellingShingle Christoph Schreyvogel
Vladimir Polyakov
Sina Burk
Helmut Fedder
Andrej Denisenko
Felipe Fávaro de Oliveira
Ralf Wunderlich
Jan Meijer
Verena Zuerbig
Jörg Wrachtrup
Christoph E. Nebel
Active and fast charge-state switching of single NV centres in diamond by in-plane Al-Schottky junctions
Beilstein Journal of Nanotechnology
active charge state control
diamond
fast charge state switching
NV centre
two-dimensional Schottky diode
title Active and fast charge-state switching of single NV centres in diamond by in-plane Al-Schottky junctions
title_full Active and fast charge-state switching of single NV centres in diamond by in-plane Al-Schottky junctions
title_fullStr Active and fast charge-state switching of single NV centres in diamond by in-plane Al-Schottky junctions
title_full_unstemmed Active and fast charge-state switching of single NV centres in diamond by in-plane Al-Schottky junctions
title_short Active and fast charge-state switching of single NV centres in diamond by in-plane Al-Schottky junctions
title_sort active and fast charge state switching of single nv centres in diamond by in plane al schottky junctions
topic active charge state control
diamond
fast charge state switching
NV centre
two-dimensional Schottky diode
url https://doi.org/10.3762/bjnano.7.165
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