Zero-Field ODMR and relaxation of Si-vacancy centers in 6H-SiC

Silicon vacancies in silicon carbide (SiC) have been proposed as interesting candidates for quantum technology applications such as quantum sensing and quantum repeaters. SiC exists in many polytypes with different plane stacking sequences, and in each polytype, the vacancies can occupy a variety of...

Full description

Bibliographic Details
Main Authors: Harpreet Singh, Andrey N Anisimov, Pavel G Baranov, Dieter Suter
Format: Article
Language:English
Published: IOP Publishing 2023-01-01
Series:Materials Research Express
Subjects:
Online Access:https://doi.org/10.1088/2053-1591/ad0935
_version_ 1797627516862595072
author Harpreet Singh
Andrey N Anisimov
Pavel G Baranov
Dieter Suter
author_facet Harpreet Singh
Andrey N Anisimov
Pavel G Baranov
Dieter Suter
author_sort Harpreet Singh
collection DOAJ
description Silicon vacancies in silicon carbide (SiC) have been proposed as interesting candidates for quantum technology applications such as quantum sensing and quantum repeaters. SiC exists in many polytypes with different plane stacking sequences, and in each polytype, the vacancies can occupy a variety of different lattice sites. In this work, we focus on the three important charged silicon vacancies in the 6 H -SiC polytype. We record the photoluminescence and continuous-wave optically detected magnetic resonance (ODMR) spectra at different radio-frequency power levels and different temperatures. We individually select the zero-phonon lines of the different silicon vacancies at low temperatures and record the corresponding ODMR spectra. ODMR allows us to correlate optical and magnetic resonance spectra and thereby separate signals from V _1 and V _3 . The results also explain the observed sign change of the ODMR signal as a function of temperature.
first_indexed 2024-03-11T10:25:24Z
format Article
id doaj.art-1ccff658c15a446eb07a9f4216a2bec7
institution Directory Open Access Journal
issn 2053-1591
language English
last_indexed 2024-03-11T10:25:24Z
publishDate 2023-01-01
publisher IOP Publishing
record_format Article
series Materials Research Express
spelling doaj.art-1ccff658c15a446eb07a9f4216a2bec72023-11-15T13:40:04ZengIOP PublishingMaterials Research Express2053-15912023-01-01101111620110.1088/2053-1591/ad0935Zero-Field ODMR and relaxation of Si-vacancy centers in 6H-SiCHarpreet Singh0https://orcid.org/0000-0002-7505-4850Andrey N Anisimov1https://orcid.org/0000-0003-2171-7943Pavel G Baranov2https://orcid.org/0000-0003-1955-9245Dieter Suter3https://orcid.org/0000-0002-7349-3032Fakultät Physik, Technische Universität Dortmund , D-44221 Dortmund, GermanyFakultät Physik, Technische Universität Dortmund , D-44221 Dortmund, GermanyIoffe Institute , St. Petersburg 194021, RussiaFakultät Physik, Technische Universität Dortmund , D-44221 Dortmund, GermanySilicon vacancies in silicon carbide (SiC) have been proposed as interesting candidates for quantum technology applications such as quantum sensing and quantum repeaters. SiC exists in many polytypes with different plane stacking sequences, and in each polytype, the vacancies can occupy a variety of different lattice sites. In this work, we focus on the three important charged silicon vacancies in the 6 H -SiC polytype. We record the photoluminescence and continuous-wave optically detected magnetic resonance (ODMR) spectra at different radio-frequency power levels and different temperatures. We individually select the zero-phonon lines of the different silicon vacancies at low temperatures and record the corresponding ODMR spectra. ODMR allows us to correlate optical and magnetic resonance spectra and thereby separate signals from V _1 and V _3 . The results also explain the observed sign change of the ODMR signal as a function of temperature.https://doi.org/10.1088/2053-1591/ad0935silicon vacancysilicon carbideODMRtemperature dependend ODMR
spellingShingle Harpreet Singh
Andrey N Anisimov
Pavel G Baranov
Dieter Suter
Zero-Field ODMR and relaxation of Si-vacancy centers in 6H-SiC
Materials Research Express
silicon vacancy
silicon carbide
ODMR
temperature dependend ODMR
title Zero-Field ODMR and relaxation of Si-vacancy centers in 6H-SiC
title_full Zero-Field ODMR and relaxation of Si-vacancy centers in 6H-SiC
title_fullStr Zero-Field ODMR and relaxation of Si-vacancy centers in 6H-SiC
title_full_unstemmed Zero-Field ODMR and relaxation of Si-vacancy centers in 6H-SiC
title_short Zero-Field ODMR and relaxation of Si-vacancy centers in 6H-SiC
title_sort zero field odmr and relaxation of si vacancy centers in 6h sic
topic silicon vacancy
silicon carbide
ODMR
temperature dependend ODMR
url https://doi.org/10.1088/2053-1591/ad0935
work_keys_str_mv AT harpreetsingh zerofieldodmrandrelaxationofsivacancycentersin6hsic
AT andreynanisimov zerofieldodmrandrelaxationofsivacancycentersin6hsic
AT pavelgbaranov zerofieldodmrandrelaxationofsivacancycentersin6hsic
AT dietersuter zerofieldodmrandrelaxationofsivacancycentersin6hsic