Progress in electrochemical reduction of CO2 by bimetallic materials with high selectivity

In recent years, the global environmental problems caused by excessive emissions of carbon dioxide(CO2) have become severe gradually, which attract widespread concern all over the world. The electrochemical reduction of CO2 to clean energy and high-value chemicals not only can effectively alleviate...

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Main Authors: WANG Yujing, LIU Man, SI Jianting, ZHANG Ting, REN Geng, CHAI Shouning
Format: Article
Language:zho
Published: Journal of Materials Engineering 2023-04-01
Series:Cailiao gongcheng
Subjects:
Online Access:http://jme.biam.ac.cn/CN/10.11868/j.issn.1001-4381.2021.001122
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author WANG Yujing
LIU Man
SI Jianting
ZHANG Ting
REN Geng
CHAI Shouning
author_facet WANG Yujing
LIU Man
SI Jianting
ZHANG Ting
REN Geng
CHAI Shouning
author_sort WANG Yujing
collection DOAJ
description In recent years, the global environmental problems caused by excessive emissions of carbon dioxide(CO2) have become severe gradually, which attract widespread concern all over the world. The electrochemical reduction of CO2 to clean energy and high-value chemicals not only can effectively alleviate greenhouse effect, but also provide an alternative to solve the energy crisis. The reaction principle of electrochemical reduction of CO2 was briefly described in this review, and some binary metal catalysts with high product selectivity reported in recent years were classified and summarized. The influences of the bimetallic materials physico-chemical properties, including element and composite, atomic ratio, microscopic morphology, particle size, etc. on CO2 reduction performance were reviewed, and the explanation of high selectivity for partial typical catalysts derived from DFT calculation was presented. Finally, the main problems and future research challenges for the selective conversion of CO2 on bimetallic catalysts with high efficiency were also discussed.
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spelling doaj.art-1d1ba8d25e914a30bf70170be2aab70c2023-04-21T06:44:56ZzhoJournal of Materials EngineeringCailiao gongcheng1001-43812023-04-0151411410.11868/j.issn.1001-4381.2021.00112220230401Progress in electrochemical reduction of CO2 by bimetallic materials with high selectivityWANG Yujing0LIU Man1SI Jianting2ZHANG Ting3REN Geng4CHAI Shouning5College of Materials and Chemical Engineering, Xi'an Technological University, Xi'an 710021, ChinaCollege of Materials and Chemical Engineering, Xi'an Technological University, Xi'an 710021, ChinaThe Seventh Division, Institute of Industrial Hygiene of Ordance Industry, Xi'an 710065, ChinaCollege of Materials and Chemical Engineering, Xi'an Technological University, Xi'an 710021, ChinaCollege of Materials and Chemical Engineering, Xi'an Technological University, Xi'an 710021, ChinaSchool of Energy and Power Engineering, Xi'an Jiaotong University, Xi'an 710049, ChinaIn recent years, the global environmental problems caused by excessive emissions of carbon dioxide(CO2) have become severe gradually, which attract widespread concern all over the world. The electrochemical reduction of CO2 to clean energy and high-value chemicals not only can effectively alleviate greenhouse effect, but also provide an alternative to solve the energy crisis. The reaction principle of electrochemical reduction of CO2 was briefly described in this review, and some binary metal catalysts with high product selectivity reported in recent years were classified and summarized. The influences of the bimetallic materials physico-chemical properties, including element and composite, atomic ratio, microscopic morphology, particle size, etc. on CO2 reduction performance were reviewed, and the explanation of high selectivity for partial typical catalysts derived from DFT calculation was presented. Finally, the main problems and future research challenges for the selective conversion of CO2 on bimetallic catalysts with high efficiency were also discussed.http://jme.biam.ac.cn/CN/10.11868/j.issn.1001-4381.2021.001122carbon dioxidealloy materialelectrocatalysisselectivitycatalytic activity
spellingShingle WANG Yujing
LIU Man
SI Jianting
ZHANG Ting
REN Geng
CHAI Shouning
Progress in electrochemical reduction of CO2 by bimetallic materials with high selectivity
Cailiao gongcheng
carbon dioxide
alloy material
electrocatalysis
selectivity
catalytic activity
title Progress in electrochemical reduction of CO2 by bimetallic materials with high selectivity
title_full Progress in electrochemical reduction of CO2 by bimetallic materials with high selectivity
title_fullStr Progress in electrochemical reduction of CO2 by bimetallic materials with high selectivity
title_full_unstemmed Progress in electrochemical reduction of CO2 by bimetallic materials with high selectivity
title_short Progress in electrochemical reduction of CO2 by bimetallic materials with high selectivity
title_sort progress in electrochemical reduction of co2 by bimetallic materials with high selectivity
topic carbon dioxide
alloy material
electrocatalysis
selectivity
catalytic activity
url http://jme.biam.ac.cn/CN/10.11868/j.issn.1001-4381.2021.001122
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AT zhangting progressinelectrochemicalreductionofco2bybimetallicmaterialswithhighselectivity
AT rengeng progressinelectrochemicalreductionofco2bybimetallicmaterialswithhighselectivity
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