The discovery of three-dimensional Van Hove singularity

Abstract Arising from the extreme/saddle point in electronic bands, Van Hove singularity (VHS) manifests divergent density of states (DOS) and induces various new states of matter such as unconventional superconductivity. VHS is believed to exist in one and two dimensions, but rarely found in three...

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Main Authors: Wenbin Wu, Zeping Shi, Mykhaylo Ozerov, Yuhan Du, Yuxiang Wang, Xiao-Sheng Ni, Xianghao Meng, Xiangyu Jiang, Guangyi Wang, Congming Hao, Xinyi Wang, Pengcheng Zhang, Chunhui Pan, Haifeng Pan, Zhenrong Sun, Run Yang, Yang Xu, Yusheng Hou, Zhongbo Yan, Cheng Zhang, Hai-Zhou Lu, Junhao Chu, Xiang Yuan
Format: Article
Language:English
Published: Nature Portfolio 2024-03-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-024-46626-9
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author Wenbin Wu
Zeping Shi
Mykhaylo Ozerov
Yuhan Du
Yuxiang Wang
Xiao-Sheng Ni
Xianghao Meng
Xiangyu Jiang
Guangyi Wang
Congming Hao
Xinyi Wang
Pengcheng Zhang
Chunhui Pan
Haifeng Pan
Zhenrong Sun
Run Yang
Yang Xu
Yusheng Hou
Zhongbo Yan
Cheng Zhang
Hai-Zhou Lu
Junhao Chu
Xiang Yuan
author_facet Wenbin Wu
Zeping Shi
Mykhaylo Ozerov
Yuhan Du
Yuxiang Wang
Xiao-Sheng Ni
Xianghao Meng
Xiangyu Jiang
Guangyi Wang
Congming Hao
Xinyi Wang
Pengcheng Zhang
Chunhui Pan
Haifeng Pan
Zhenrong Sun
Run Yang
Yang Xu
Yusheng Hou
Zhongbo Yan
Cheng Zhang
Hai-Zhou Lu
Junhao Chu
Xiang Yuan
author_sort Wenbin Wu
collection DOAJ
description Abstract Arising from the extreme/saddle point in electronic bands, Van Hove singularity (VHS) manifests divergent density of states (DOS) and induces various new states of matter such as unconventional superconductivity. VHS is believed to exist in one and two dimensions, but rarely found in three dimension (3D). Here, we report the discovery of 3D VHS in a topological magnet EuCd2As2 by magneto-infrared spectroscopy. External magnetic fields effectively control the exchange interaction in EuCd2As2, and shift 3D Weyl bands continuously, leading to the modification of Fermi velocity and energy dispersion. Above the critical field, the 3D VHS forms and is evidenced by the abrupt emergence of inter-band transitions, which can be quantitatively described by the minimal model of Weyl semimetals. Three additional optical transitions are further predicted theoretically and verified in magneto-near-infrared spectra. Our results pave the way to exploring VHS in 3D systems and uncovering the coordination between electronic correlation and the topological phase.
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spelling doaj.art-1d3a73625ece42bf93935cd3a2bd85362024-03-17T12:30:21ZengNature PortfolioNature Communications2041-17232024-03-0115111110.1038/s41467-024-46626-9The discovery of three-dimensional Van Hove singularityWenbin Wu0Zeping Shi1Mykhaylo Ozerov2Yuhan Du3Yuxiang Wang4Xiao-Sheng Ni5Xianghao Meng6Xiangyu Jiang7Guangyi Wang8Congming Hao9Xinyi Wang10Pengcheng Zhang11Chunhui Pan12Haifeng Pan13Zhenrong Sun14Run Yang15Yang Xu16Yusheng Hou17Zhongbo Yan18Cheng Zhang19Hai-Zhou Lu20Junhao Chu21Xiang Yuan22State Key Laboratory of Precision Spectroscopy, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityNational High Magnetic Field Laboratory, Florida State UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityState Key Laboratory of Surface Physics and Institute for Nanoelectronic Devices and Quantum Computing, Fudan UniversityGuangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-Sen UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityMultifunctional Platform for Innovation Precision Machining Center, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityKey Laboratory of Quantum Materials and Devices of Ministry of Education, School of Physics, Southeast UniversityKey Laboratory of Polar Materials and Devices, Ministry of Education, School of Physics and Electronic Science, East China Normal UniversityGuangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-Sen UniversityGuangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-Sen UniversityState Key Laboratory of Surface Physics and Institute for Nanoelectronic Devices and Quantum Computing, Fudan UniversityShenzhen Institute for Quantum Science and Engineering and Department of Physics, Southern University of Science and Technology (SUSTech)Key Laboratory of Polar Materials and Devices, Ministry of Education, School of Physics and Electronic Science, East China Normal UniversityState Key Laboratory of Precision Spectroscopy, East China Normal UniversityAbstract Arising from the extreme/saddle point in electronic bands, Van Hove singularity (VHS) manifests divergent density of states (DOS) and induces various new states of matter such as unconventional superconductivity. VHS is believed to exist in one and two dimensions, but rarely found in three dimension (3D). Here, we report the discovery of 3D VHS in a topological magnet EuCd2As2 by magneto-infrared spectroscopy. External magnetic fields effectively control the exchange interaction in EuCd2As2, and shift 3D Weyl bands continuously, leading to the modification of Fermi velocity and energy dispersion. Above the critical field, the 3D VHS forms and is evidenced by the abrupt emergence of inter-band transitions, which can be quantitatively described by the minimal model of Weyl semimetals. Three additional optical transitions are further predicted theoretically and verified in magneto-near-infrared spectra. Our results pave the way to exploring VHS in 3D systems and uncovering the coordination between electronic correlation and the topological phase.https://doi.org/10.1038/s41467-024-46626-9
spellingShingle Wenbin Wu
Zeping Shi
Mykhaylo Ozerov
Yuhan Du
Yuxiang Wang
Xiao-Sheng Ni
Xianghao Meng
Xiangyu Jiang
Guangyi Wang
Congming Hao
Xinyi Wang
Pengcheng Zhang
Chunhui Pan
Haifeng Pan
Zhenrong Sun
Run Yang
Yang Xu
Yusheng Hou
Zhongbo Yan
Cheng Zhang
Hai-Zhou Lu
Junhao Chu
Xiang Yuan
The discovery of three-dimensional Van Hove singularity
Nature Communications
title The discovery of three-dimensional Van Hove singularity
title_full The discovery of three-dimensional Van Hove singularity
title_fullStr The discovery of three-dimensional Van Hove singularity
title_full_unstemmed The discovery of three-dimensional Van Hove singularity
title_short The discovery of three-dimensional Van Hove singularity
title_sort discovery of three dimensional van hove singularity
url https://doi.org/10.1038/s41467-024-46626-9
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